PAUL SCHERRER INSTITUT Neutron Radiography …indico.ictp.it/event/a04211/session/72/contribution/43/...Paul Scherrer Institut • 5232 Villigen PSI Trieste, Material Sience, 2005PAUL

Paul Scherrer Institut • 5232 Villigen PSI Trieste, Material Sience, 2005

PAUL SCHERRER INSTITUT

Neutron Radiographyand

Tomography

Eberhard H. LehmannPaul Scherrer Institut, CH-5232 VilligenSpallation Neutron Source Division (ASQ)

Neutron Imaging & Activation



Outline (1)

1. How transmission imaging started

2. Neutron interaction, comparison to X-ray

3. What means neutron imaging today

4. Facilities for neutron imaging

5. Detector options for digital neutron imaging

6. Limitations and application range



Outline (2)

7. Specific methods in neutron imaging

8. Principles of neutron tomography

9. Typical applications of neutron imaging

• Science• Industry• Cultural heritage7. Future trends and aspects



How transmission imaging started



First experiments with a new kind of radiationwere performed by Konrad Röntgen in 1895during investigations with cathode-ray tubes.

He found the new ray could pass through mostsubstances casting shadows of solid objects.

In conjunction with a photographic plate, a picture of interior body parts can be obtainedwhen human tissue will be investigated.

X-ray



One of the first experiments late in 1895was a film of a hand of his wife.

The bones and also finger rings delivermuch higher contrast than the softtissue.



Some more exotic applications of X-raytransmission in the earlier period of use.



Such an “open” laboratory wouldn’t be tolerated today due to radiationprotection regulations!



Only few month later (1896)Henri Becquerel discovered the naturalradioactivity when he investigated thefluorescence behavior of uranium saltsand found films blackened through theirlight tight covers.

Gamma radiography became first not aspopular as X-ray one due to the availabilityof the suited source materials.

The discovery of Radium and artificialradioactive gamma sources (Co, Ir, Cs)broadened the application.

During World War II, industrial radiographygrew tremendously as part of the Navy’sshipbuilding and submarine program.

Gamma radiation



Roots of neutron radiographyTaken from C.O. Fischer’s article in WCNR-4

Berlin, 1935 – 1938H. Kallmann & Kuhn with Ra-Be and neutron generator

Berlin until Dec. 1944O. Peter with anaccelerator neutron source

But the real programs with neutrons started after World War II at research reactors

As typical: valves, manometers, injectors



From X-rays to neutrons



Nuclear Interactions

• X-rays interact with the electron shell of the atoms by Compton scattering, photo-effect and pair-production

• Thermal neutrons interact with the atomic nuclei by collision (elastic and inelastic scattering), capture and (seldom) fission



1a 2a 3b 4b 5b 6b 7b 1b 2b 3a 4a 5a 6a 7a 0H He

Li Be B C N O F Ne

Na Mg Al Si P S Cl Ar

K Ca Sc Ti V Cr Mn Fe Co Ni Cu Zn Ga Ge As Se Br Kr

Rb Sr Y Zr Nb Mo Tc Ru Rh Pd Ag Cd In Sn Sb Te I Xe

Cs Ba La Hf Ta W Re Os Ir Pt Au Hg Tl Pb Bi Po At Rn

Fr Ra Ac Rf Ha

Ce Pr Nd Pm Sm Eu Gd Tb Dy Ho Er Tm Yb Lu

Th Pa U Np Pu Am Cm Bk Cf Es Fm Md No

8

*Lanthanides

**Actinides

Periodisches System der Elemente



Attenuation coefficients with X-ray [cm?¹]

1a 2a 3b 4b 5b 6b 7b 8 1b 2b 3a 4a 5a 6a 7a 0 H He

0.02 0.02Li Be B C N O F Ne

0.06 0.22 0.28 0.27 0.11 0.16 0.14 0.17Na Mg Al Si P S Cl Ar

0.13 0.24 0.38 0.33 0.25 0.30 0.23 0.20K Ca Sc Ti V Cr Mn Fe Co Ni Cu Zn Ga Ge As Se Br Kr

0.14 0.26 0.48 0.73 1.04 1.29 1.32 1.57 1.78 1.96 1.97 1.64 1.42 1.33 1.50 1.23 0.90 0.73Rb Sr Y Zr Nb Mo Tc Ru Rh Pd Ag Cd In Sn Sb Te I Xe

0.47 0.86 1.61 2.47 3.43 4.29 5.06 5.71 6.08 6.13 5.67 4.84 4.31 3.98 4.28 4.06 3.45 2.53Cs Ba La Hf Ta W Re Os Ir Pt Au Hg Tl Pb Bi Po At Rn

1.42 2.73 5.04 19.70 25.47 30.49 34.47 37.92 39.01 38.61 35.94 25.88 23.23 22.81 20.28 20.22 9.77Fr Ra Ac Rf Ha 11.80 24.47


Lanthanides 5.79 6.23 6.46 7.33 7.68 5.66 8.69 9.46 10.17 10.91 11.70 12.49 9.32 14.07 Th Pa U Np Pu Am Cm Bk Vf Es Fm Md No Lr

*Actinides 28.95 39.65 49.08 x-ray Legend Attenuation coefficient [cm?¹] = sp.gr. * μ/δ sp.gr.: Handbook of Chemistry and Physics, 56th Edition 1975-1976. μ/δ: J. H. Hubbell+ and S. M. Seltzer Ionizing Radiation Division, Physics Laboratory National Institute of Standards and Technology Gaithersburg, MD 20899,

http://physics.nist.gov/PhysRefData/XrayMassCoef/tab3.html.

X-ray



Attenuation coefficients with neutrons [cm?¹]

1a 2a 3b 4b 5b 6b 7b 8 1b 2b 3a 4a 5a 6a 7a 0 H He

3.44 0.02Li Be B C N O F Ne

3.30 0.79 101.60 0.56 0.43 0.17 0.20 0.10Na Mg Al Si P S Cl Ar

0.09 0.15 0.10 0.11 0.12 0.06 1.33 0.03K Ca Sc Ti V Cr Mn Fe Co Ni Cu Zn Ga Ge As Se Br Kr

0.06 0.08 2.00 0.60 0.72 0.54 1.21 1.19 3.92 2.05 1.07 0.35 0.49 0.47 0.67 0.73 0.24 0.61Rb Sr Y Zr Nb Mo Tc Ru Rh Pd Ag Cd In Sn Sb Te I Xe

0.08 0.14 0.27 0.29 0.40 0.52 1.76 0.58 10.88 0.78 4.04 115.11 7.58 0.21 0.30 0.25 0.23 0.43Cs Ba La Hf Ta W Re Os Ir Pt Au Hg Tl Pb Bi Po At Rn

0.29 0.07 0.52 4.99 1.49 1.47 6.85 2.24 30.46 1.46 6.23 16.21 0.47 0.38 0.27 Fr Ra Ac Rf Ha 0.34


*Lanthanides 0.14 0.41 1.87 5.72 171.47 94.58 1479.04 0.93 32.42 2.25 5.48 3.53 1.40 2.75 Th Pa U Np Pu Am Cm Bk Cf Es Fm Md No Lr

**Actinides 0.59 8.46 0.82 9.80 50.20 2.86 neut. Legend

σ-total * sp.gr. * 0.6023 Attenuation coefficient [cm?¹] = at.wt. σ-total: JEF Report 14, TABLE OF SIMPLE INTEGRAL NEUTRON CROSS SECTION DATA FROM JEF-2.2, ENDF/B-VI, JENDL-3.2, BROND-2 AND CENDL-2,

AEN NEA, 1994. and Special Feature: Neutron scattering lengths and cross sections, Varley F. Sears, AECL Research, Chalk River Laboratories Chalk River, Ontario, Canada KOJ

1JO, Neutron News, Vol. 3, 1992, http://www.ncnr.nist.gov/resources/n-lengths/list.html. sp.gr.: Handbook of Chemistry and Physics, 56th Edition 1975-1976. at.wt.: Handbook of Chemistry and Physics, 56th Edition 1975-1976.

thermal neutrons



Comparison between the interaction probabilitiesfor (thermal) neutrons and x-ray

The deviations in the cross-sections are especially high for:A: light materials like hydrogen B: especially strong neutron absorbers Gd, Cd, Dy, In C: heavy materials like Pb, Bi, U , Th

AB

C



Comparison of transmission images

X-ray neutron

high contrast for metals metals are more transparentno contrast for plastics high contrast for plastics

HARD DRIVE



source collimator object detector

Simplified setup of a radiography facility

***never forget the shielding around ***



Neutron sources

• Research reactor (ILL, FRM-2,...)• Spallation sources (ISIS, SINQ, SNS,...)• Radioactive nuclides (Cf, Ra-Be, Sb-Be)• Accelerator sources (D-D, D-T reactions)



Properties of neutron sourcesfor imaging purpose

Source type nuclear reactor neutron generator spallation source radio isotope

Reaction fission D-T fusion spallation by protons gamma-n-reaction

used material U-235 deuterium, tritium high mass nuclides Sb, Be

gain: primary neutron intensity [1/s]

1.00E+16 4.00E+11 1.00E+15 1.00E+08

beam intensity[cm-2 s-1] 106 to 109 105 106 to n*107 103

neutron energyfast, thermal and

cold fast, thermal fast, thermal and cold 24 keV, thermal

limitation of use burn up life time tube target life time half life Sb-124

typical operation cycle 1 month 1000 h 1 year 0,5 year

costs of the facility high medium very high low



Neutron energies• high energy neutrons (E > 100 MeV)• fast neutrons (from fission process): E ~ 1 MeV• epithermal neutrons: E > 1eV• thermal neutrons: E ~ 25 meV• cold neutrons: E ~ 4 meV• ultra-cold neutrons: E ~ 100 neV

15 orders of magnitude in energy



Neutron energies• high energy neutrons (E > 100 MeV)• fast neutrons (from fission process): E ~ 1 MeV• epithermal neutrons: E > 1eV• thermal neutrons: E ~ 25 meV• cold neutrons: E ~ 4 meV• ultra-cold neutrons: E ~ 100 neV

15 orders of magnitude in energy



0.0E+00

2.0E+02

4.0E+02

6.0E+02

8.0E+02

1.0E+03

1.00E-06 1.00E-03 1.00E+00 1.00E+03 1.00E+06 1.00E+09

neutron energy [eV]

inte

nsity

[rel

. uni

ts]

Fission SpectrumThermal MaxwellianSb-BeCold Source SpectrumB-10 cross-section



Collimation• to generate a quasi-parallel, clean beam• by selection of suited neutrons• collimation ratio: L(collator length)/D(aperture

diameter) – typically several 100• by filtering (against gamma radiation,

against neutrons of different energies)• to limit the radiation level at the detector

position



The Neutron Radiography Station NEUTRA for thermal neutrons

ca. 10 m



0.0E+00

2.0E+02

4.0E+02

6.0E+02

8.0E+02

1.0E+03

1.00E-06 1.00E-03 1.00E+00 1.00E+03 1.00E+06 1.00E+09

neutron energy [eV]

inte

nsity

[rel

. uni

ts]

Fission SpectrumThermal MaxwellianSb-BeCold Source SpectrumB-10 cross-section



The Neutron Radiography Station ICON for cold neutrons

In use since May 2005In use since May 2005



ICON beam line @ SINQ

micro-tomographysetup

position for theobservation of extended objects



Properties of the neutron radiography stations at PSI

325mean energy [meV]

coldthermalspectrum

8 – 30 cmdep. on the chosen aperture

∅ 15 – 40 cm beam size

Up to ~1000dep. on the chosen aperture

250 – 550collimation ratio L/D

> 5·1063·106 - 2·107neutron flux density [cm-2 s-1]

ICON(under construction)

NEUTRA(operational since 1997)

Facility



neutron detection for imaging

• no direct neutron detection possible

• a secondary nuclear process is needed(capture, fission, collision)

• main neutron imaging processes are using:scintillationphoto-luminiscence by secondary particles + β, γnuclear track detectionchemical excitationcollection of charge in semiconductors from Gd conversion



Capture reactions for thermal neutrons

3He + 1n 3He + 1p + 0.77 MeV

6Li + 1n 3H + 4He + 4.79 MeV

10B + 1n 7Li + 4He + 2.78 MeV (7%)7Li* + 4He + 2.30 MeV (93%)

155Gd + 1n 156Gd + γ´s + CE´s (7.9 MeV)

157Gd + 1n 158Gd + γ´s + CE´s (8.5 MeV)

235U, 239Pu 1n fission products + 80 MeV



Properties of neutron detection materials

reaction σn [barn] particle energy [MeV]

natural content enrichment price [US$ 2000]3He(n,p) 5333 p: 0.57 3H: 0.2 0.00014% 90 dm-3

6Li(n,α) 940 α: 2.05 3H: 2.74 7.5% 95% 1.5 g-1 6Li Metall10B(n,α) 3837 α: 1.47 7Li: 0.83 19.8% 99% 12 g-1 10B2O3

155Gd(n,γ ) 60900 CE,s: 0.039 - 0.25 14.8%157Gd(n,γ ) 254000 CE´s: 0.029 - 0.23 15.7% 86% 8000 g-1 Gd2O3natGd(n,γ ) 48890 100% 1.5 g-1 Gd2O3

235U(n,f) 583 80 total 0.72%239Pu(n,f) 748 80 total 0



detector systemx-ray film and

transmission light scanner

scintillator + CCD-camera imaging plates amorph silicon

flat panel

max. spatial resolution [μm]

20 - 50 100 - 500 25 - 100 127 - 750

typical exposure time for suitable image

5 min 10 s 20 s 10s

detector area (typical) 18 cm x 24 cm 25 cm x 25 cm 20 cm x 40 cm 30 cm x 40 cm

number of pixels per line 4000 1000 6000 1750

dynamic range 102 (non-linear) 105 (linear) 105 (linear) 103 (non-linear)

digital format 8 bit 16 bit 16 bit 12 bit

Detectors for digital imaging with neutrons



1.00E-03

1.00E-02

1.00E-01

1.00E+00

1.00E+01

0.0001 0.001 0.01 0.1 1 10 100 1000 10000 100000 1000000

time resolution [s]

spat

ial r

esol

utio

n [m

m]

X-ray film+ converter

track etchfoils

Neutron detectors for imaging

Situation about 10 years agoSituation about 10 years ago



1.00E-03

1.00E-02

1.00E-01

1.00E+00

1.00E+01

0.0001 0.001 0.01 0.1 1 10 100 1000 10000 100000 1000000

time resolution [s]

spat

ial r

esol

utio

n [m

m]


track etchfoils

CCD camera+ scintillator

n-imaging plates

amorphous-Siflat panel

CMOSpixel detector

intensifiedreal-timecamera


Present situationPresent situation



1.00E-03

1.00E-02

1.00E-01

1.00E+00

1.00E+01

0.0001 0.001 0.01 0.1 1 10 100 1000 10000 100000 1000000

time resolution [s]

spat

ial r

esol

utio

n [m

m]


track etchfoils

CCD camera+ scintillator

n-imaging plates

amorphous-Siflat panel

CMOSpixel detector

intensifiedreal-timecamera

more neutrons

detectordevelopment!!!




CCD-camera• neutrons are hitting the

scintillator and the emitted light will be detected by the high sensitive camera.

This design has become a commonone is many labs

This design has become a commonone is many labs



Neutron Imaging with a PILATUS -Module

CMOSChip

Silicon Sensor

IndiumBump

Gd Converter

Aluminisationp+

n+

Thermal neutrons

e- +

GlobalTresh

Tresholdcorrection

CSAmp

CompBumpPad

DOUTAOUT

GateRowsel

PixselPixsel Colsel

-

+

Cal1.7fF

Analog Block Digital Block

15 bit SRcounter

Φ12

ClockGen

ExtClock

Ext/CompClock

&

Principle

Pixel Electronics Features

• No dark current

• No readout-noise

• Fast Gate: 100μs …secs

• Read-out time: 6.7ms



transmission image by neutronsFoto of the array in a box

active area: 3.5 cm * 8 cm



1.00E-06 1.00E-05 1.00E-04 1.00E-03 1.00E-02 1.00E-01 1.00E+00

neutron

SLS

dimensions [m]

Comparison to Synchrotron Radiation Imaging

Detection lower limit: spatial resolution (by the detector)Detection upper limit: object size (beam size, transmission)

Different, but overlapping working area



Options for neutron imagingavailable at PSI

Radiography with high spatial resolutionTomography on different size scale (4 cm to 40 cm)real-time imaging (up to 30 frames/sec. or triggered mode)Phase contrast neutron imagingLaminographyX-ray enhanced neutron imagingLater: energy selective neutron imagingLater: micro-tomography with neutrons



The Principles of Neutron Tomography

B. Schillinger



1. Introduction

- A radiography picture is a shadow image of the investigated sample.

- Information about the internal distribution of the attenuation coefficient within the sample along beam direction is lost in the single projection.

- If the sample is rotated and many different views are taken, a tomographicreconstruction of that internal distribution can be performed.

- Mathematical models assume either a perfect parallel beam or a perfect point source.

- Neither case is exactly given for neutron tomography.

- It is therefore of great importance to shape the beam as to approximate ideal beam geometry best as possible.



Beam geometries for tomography

Fan beam geometry

This applies for a standard setup with an X-ray tube and a line detector.The projection of the sample is magnified.Reconstruction is done in an even plane.




Cone beam geometry

Applies for a point source (LinAc, X-ray tube) and a two-dimensional detector.

The projection of the sample is magnified.

Reconstruction must be done in a 3D-Matrix.




Parallel beam geometry

The simplest case - applies for a synchrotron light source and a lineor 2D-detector.

There is no magnification.

For neutrons, none of the cases is really true, we try to approximate parallel beam geometry as good as possible.



2. The tomography principle

2.1 Projection and Radon Transform

The following assumptions are made:

- the examined object is penetrated by a bundle of parallel rays. The procedure can be described in a plane (x,y).

- The beam is attenuated by the two-dimensional attenuation coefficient Σ(x,y).

- Scattered neutrons do not hit the detector, so scattering looks like absorption.

- The beam is mono-energetic.



Each detector element is hit by a number of neutrons

with N0= number of incident neutrons and the linear attenuation coefficient Σ(x,y) at position (x,y).

Integration is performed along the straight beam path s through the plane.

eNN pathbeam

dsyx⋅= ∫Σ−

0),(



Projection Pθ(t) of a two-dimensional slice and the position of its Fourier transform Pθ(ω) in frequency domain.



We can give the projection of the two-dimensional slice as a one-dimensional function of the variable t perpendicular to the rays:

∫Σ=),(

),()(tray

dsyxtpθ

θ

∫∫+∞

∞−

+∞

∞−

Σ−+= dxdyyxtyx ),()sincos( θθδ

θθ sincos yxtwith +=

This is the Radon Transform .



It can be derived from measurement as

)()(

ln)(0 t

tt

NNp θ

θ−=

For parallel beam geometry, an angular range of 0 to 180° it is sufficient.

The integration causes the loss of the spatial information aboutthe distribution of Σ(x,y) along the ray path.

But as each ray represents an independent measurement, the spatial information perpendicular to the ray direction

(i.e. in direction θ,t) is still present.



2.2 The Fourier Slice Theorem

The one-dimensional Fourier-Transform of the projection Pθ(ω) is

dtt epP ti∫+∞

∞−

−= ωπ

θθ ω 2)()(

and the two-dimensional Fourier-Transform S(u,v) of the slice to be reconstructed is:

dxdyyxvu eS vyuxi∫∫+∞

∞−

+−+∞

∞−

Σ= )(2),(),( π



These combined deliver the Fourier Slice Theorem:

),()sin,cos()( θωθωθωωθ SSP ≡=

Which can be worded as:

“The one-dimensional Fourier Transform Pθ(ω) of a parallel projection of a distribution μ(x,y),

taken under an angle θ, is identical with a single line within the two-dimensional Fourier Transform S(u,v)

of the distribution Σ(x,y) that encloses the angle θ with the u-axis.”



For reminder, again the representation in the spatialand in the Fourier Domain:



In theory, it would be possible to fill the entire Fourier spaceby measuring an infinite number of projections and then to obtain the distribution μ(x,y) by a two-dimensional Fourier back-transform of S(u,v):

dvduvuSyx e vyuxi∫∫+∞

∞−

++∞

∞−

=Σ )(2),(),( π



2.3 Filtered Back-projection

In reality, the number of rays and the number of projections is limited. The function S(u,v) is known only at a few points on radial lines.

Measured values in frequency domain



•These points must be interpolated to a quadratic mesh.

•With increasing radial distance, the density of measured values decreases, and interpolation incertainty increases.

•A simple reconstruction can be performed by simply summing up the two-dimensional Fourier Transforms of the single lines.

•Because of the linearity of the Fourier Transform, this can be done either in spatial or in frequency domain.

•But as the density of measured values decreases towards high frequencies, the high frequencies do not get enough weight, and the reconstructed image appears smoothed or smeared.



Each of k projections over 180° must deliver the information for a "cake slice" of width 2π|ω|/k.

But as it delivers only a single line, it is weighted with a ramp filter of height 2π|ω|/k, so that the new wedge has the same "mass” as the cake slice.

required, real and filtered representation of the data in frequency domain



The filter |ω| can be obtained mathematically exact by transformation to polar coordinates in frequency space. Then we obtain

θθθωωθω

θωωθω

ωππ

θθωππ

sincos||),(

||),(),(

0

2

0

0

)sincos(2

0

yxtwithddS

ddSyx

e

eti

yxi

+==

=Σ

∫∫

∫∫∞+

+∞+

If we now substitute the one-dimensional Fourier Transform Pθ(ω) of the projection at angle θ for the two-dimensional Fourier Transform S(ω,θ), we obtain

ωωωθθθ

θθθωωω

ωπ

θθ

π

θ

ωπ

θ

π

dtwithdyx

yxtwithddyx

ePQQ

ePti

ti

∫∫

∫∫∞+

+∞

=+=

+=⎥⎦

⎤⎢⎣

⎡=Σ

0

2

0

0

2

0

||)()()sincos(

sincos||)(),(

This Equation describes a filter operation with the filter |ω|.



Qθ(t) is called "filtered projection”.

These filtered projections are "back-projected" onto the reconstruction field: Each filtered projections Qθ(t) contributes the same value to all points of the reconstruction field along the original ray.The filtered back-projection is being "smeared" along the original ray path across the reconstruction field.



The filtered back-projection is being "smeared" along the original ray path across the reconstruction field.

Back-projection of filtered data



The maximum spatial frequency is given by Nyquists theorem by the distance T between two detector elements as

T212

max⋅= πω



The simple multiplication of Pθ(ω) by ω in the frequency domain can be replaced by a convolution of pθ(t) with the Fourier Transform of |ω| in the spatial domain:

Frequency domain Frequency domain spatial domainFrequency domain Spatial domain

w (frequency) or t (distance)

The ideal filter |ω| in spatial and frequency domain



•Difficulties with the ideal filter |ω| occur with noisy data, as noise consists mainly of high frequencies, which are much enhanced by this filter. •The ideal filter is therefore often replaced by special filter functions that decrease again towards high frequencies.•For neutrons, the inherent beam unsharpness (see below) often attenuates most high frequencies towards the Nyquist limit.

The ideal filter |ω| and some alternative functions



2.4 Number of projections

The number of projections should be in the same order as the number of rays in one projection. For M projections with N rays over 180° , the angular increment δbetween two consecutive projections is given in Fourier space as

Mπδ =

For distance T between two neighboring rays, the highest measured spatial frequency ωmax in the projection is given by Nyquist's Theorem as

T21

max=ω



This is the radius of a disk in the frequency domain that contains all measured values. The distance d between two consecutive values on the circle is:

MTd πδω 2

1max =⋅=

Density of measured values in frequency domain



For N measured values for each projection in spatial domain, there are also N measured values for each measured line in the frequency domain, so that the distance ε between two consecutive measured values on a radial line (or diameter) in frequency domain is given as

TNN12 max ==

ωε

For the worst azimuthal resolution in frequency domain to match the radial resolution, we must demand:

TNMT1

21

≈π



For practical neutron radiography, most detector systems cannot - at least for sub-millimeter resolution - measure down to the nominal Nyquist resolution given by their pixel size.

The greatest limiting factor is almost always the geometry of the neutron beam and its deviation from the ideal parallel ray model.

2π

≈=NM

raysofNumbersprojectionofNumber



Camera Control System Control Volume Reconstruction Visualisation

beamshutter

beammonitor

rotatingdesk



Sequence for the neutron tomography reconstruction

Acquisition of N+1 projections of the object rotated in N steps over 180°around its vertical axis

Spot filtering and normalization, determination of the centre of rotation

Building of the sinogram = rearrangement of the projection values for onesingle slice

Reconstruction according to the “Filtered back-projection” algorithm

Results as a three-dimensional matrix of attenuation coefficients Σ(x,y.z)





Non-invasive investigation of objects from cultural heritage

example:

bronze sculpture“The Sun”made by Jaohan Gregor van der Schardt

height: 45.7 cm

tomography set produced intwo separate runs-data unified





Time dependent investigations with neutrons

• the opportunity to make time dependent investigationsis limited by the beam intensity and the detector efficiency

• In the case of repetitive processes, triggered optionsand superposition of frames can be exploited

• It is to optimise between image quality and time resolution



Piston movementof a running motorcarengine

obtained at 1000 rpm





Resin injection intoa wooden sample:

Leaf 15 cm long

direct run



referenced to original state

Resin injection intoa wooden sample:

Leaf 15 cm long



Energy selective NR investigations

• Using a turbine type selector

• Using a beam line on a pulsed neutron source with the TOF option

• To cut out parts of the spectrum by absorbers



Experiments at the Bragg edges of the materials

cold spectrumpreferred !



Experiment 1:

neutron energy selector at the PGAneutron guide 15 of SINQwork was done as collaboration betweenUni Fribourg, PSI (CH) and TU Munich (D)



Application of referencing

Image at: 6.9Å 3.2Å division

Example: spark plug, N. Kardjilov (TUM)

Steel becomes transparent, electrodes more clearly visible



The Neutron Radiography Station NEUTRA for thermal neutrons

ca. 10 m

X-ray option



Example for a comparison

End-connector of aHe-3 counter

measured with Imaging Platesunder similar conditions

neutron X-ray

•Check of the He-3 gas content with n•Status of the wire connection with X



Applications of neutron imaging(selected cases)

• All cases where organic liquids are involved• Adhesive connections, especially in metals• Explosives detection • Inspection of nuclear fuel• Hydride accumulation, corrosion of metals• In-situ diagnostic of processes, e.g. electric fuel cells• Analysis of museums objects (unique samples!)• Biologic tests (in-situ root growing)• Standard NDT (turbine blades, casting pieces, …)



Inspection of a motorcar door with neutrons

►the metallic parts are transparent►the adhesive bounds can be inspected easily

photograph neutron image



0

10000

20000

30000

40000

50000

0 20 40 60 80 100 120 140 160distance [mm]

transmission [rel. units]

2,34%

3,5%

4.74%

3,5% + 3,95% Gd

enrichment

Determination of the U-235 content (enrichment) in nuclear fuel elements



“Mercur from Uster”

Roman bronze sculpture

Taken from the Swiss National Museum, Zurich

Due to the high leadcontent, neutron imagingis advantageously applied



Facility utilization NEUTRA 2004

research34%

material testing40%

methodical development

11%

detector tests15%



Methods

NEURAP

Radiography

Tomography

Laminography

Auto-radiography

others

Realtime



Detectors

ANDOR62%Pi-max

4%

PaxScan1%

n-IP25%

g-IP6%

PILATUS-N0%

others2%


PAUL SCHERRER INSTITUTUser countries

Schweiz

Schweiz (PSI)

Deutschland

Österreich

Japan

USA

Tschechien

Dänemark

Korea

Without any user support for traveling and accommodation until now!



Conclusions• Neutron imaging methods are established at PSI

and used for many interesting applications in science and technology

• There has been a strong progress on the detector side which makes the method more attractive and diverse in applications

• There is potential for several new options to improve the methodology (especially at new sources)

• An easy access to the facility will help to attract industrial (commercial) partners

• A network of the NR facilities will improve the flexibility and the interaction between the partners, maybe with the help of NMI3!?



Further information can be found at:

http://neutra.web.psi.ch/

Documents

PAUL SCHERRER INSTITUT Neutron Radiography …indico.ictp.it/event/a04211/session/72/contribution/43/...Paul Scherrer Institut • 5232 Villigen PSI Trieste, Material Sience, 2005PAUL