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·-~
.r, ~
~- Commission of th~ European Communities I ,-
I .i · radiation protection
! : l I j
....... LC') -->< w w (.)
;
RADIOACTIVITY MEASUREMENTS IN EUROPE AFTER THE CHERNOBYL ACCIDENT
Part I: Air
LI8RARY I I
·Report EU~R 12269 EN
Blow-up from microfiche original
..
1989
Commission of the European Communities
radiation protection
RADIOACTIVITY MEASUREMENTS IN EUROPE AFTER THE CHERNOBYL ACCIDENT
Part 1: Air
F. RAES, G. GRAZIANI, L. GROSSI L. MARCIANO, D. PEIRS*, B. PEDERSEN, D. STANNERS, N. ZARIMPAS**
* Grant Holder ** Visiting Scientist
Commission of the European Communities Joint Research Centre
lspra Establishment I- 21020 ISPRA (VA)
Directorate-General Science, Research and Development Joint, Research Centre
EUR 12269 EN
Published by the COMMISSION OF THE EUROPEAN COMMUNITIES
Directorate-General Telecommunications, Information Industries and Innovation
L-2920 LUXEMBOURG
LEGAL NOTICE
Neither the Commission of the European Communities nor any person acting on behalf of the Commission is responsible for the use which might be made of the following
information
Catalogue number: CD-NA-12269-EN-C
© ECSC-EEC-EAEC Brussels - Luxembourg, 1989
1
INTRODUCTION
The data base presented here is being set up primarily for scientific studies such as the validation of long range transport models, physico-chemical behaviour of radionuclides in air, etc.
The data were extracted from the REM Data Bank at the Joint Research Centre of the Commission of the European Communities at Ispra (I) . The data where originally obtained from written reports or were copied directly from tapes ore diskettes into the REM Data Bank. In the latter case, verification with written material was persued. The original sources are given in the references.
In preparing this report, only those data were retained which were fully specified as far as time, location and measuring techniques are concerned, i.e.: beginning and end of sampling, geographical coordinates and types of filters are known.
The full dataset is written on a diskette supplied in the back cover of this report. The diskette is low density (360K) formatted and contains three ASCII files:
CHERNAIR.TXT giving I-131, Cs-134 and Cs-137 concentrations in aerosol particles,
CHERNIOD.TXT giving total I-131 (gas + particles) concentrations,
README.TXT explaining the format of the two previous files.
Fig. 1 and Fig. 2 show the locations covered by CHERNAIR.TXT and CHERNIOD.TXT respectively.
The content of the diskette is visualized in Appendix 1 and Appendix 2, showing figures and tables with time histories of I-131 and Cs-137 in aerosol particles and of total I-131 respectively.
Reading these tables, it should be noted that: - 'HOUR' in the tables is the time of the end of
sampling and is given in hours:minutes. It is not known whether the time is UTC or local time. Hence, if the time given in the report is taken to be UTC, then this time can be up to 3h later than the actual universal time.
- 'DURATION' is the duration of sampling and is given in hours.minutes
- 'LATITUDE' and 'LONGITUDE' are given in degrees.centigrades
2
CEC JRC-ISPRA REM
Fig. 1
Locations for which I-131, cs-134 and/or Cs-137 concentrations of aerosol particles are given.
\
I I ~ I -v I I
~~ I I I I I
i CEC JRC-ISPRA REM
3
I_ ------------------------------------------------------~
Fig. 2
Locations for which total I-131 {gaseous + aerosol fraction) concentrations are given.
5
REFERENCES
* AUSTRIA
'TSCHER: a databank for samples which were measured in Austria following the Chernobyl accident'. Austrian Research Centre Seibersdorf, A-2444 SEIBERSDORF. Contact: Dr. B. Kunsch
'Tschernobyl und die folgen fuer Oesterreich' (1986) Bundesministerium fuer Gesundheit und Umweltschutz
* BELGIUM
Diskette from 'Studiecentrum voor Kernenergie', B-2400 MOL. Contact: Dr. C. Hurtgen.
Diskette from 'Instituut voor Hygiene en Epidemiologie'. B-1050 BRUSSEL. Contact: Dr. H. Versele-Declerq.
'A compendium of the measurements related to the Chernobyl nuclear accident' (1987) Studiecentrum voor Kernenergie MOL, BLG-595
'Radioactivity Monitoring: Results 1986, Draft Report' (1987) Instituut voor Hygiene en Epidemiologie.
* CZECHOSLOVAKIA
'Report on radiation situation in CSSR after Chernobyl accident' (1986) Institute of Hygiene and Epidemiology, Centre of Radiation Hygiene, Prague 10.
* DENMARK
Diskette from Risoe National Laboratories. Postbox 49, 4000 ROSKILDE. Contact: Dr. J. Lippert.
'Slutrapportering af Risoes maeleprogram (Fase III) i forbindelse med Chernobylulykken' A. Aarkorg (1987) Risoe National Laboratories.
* FEDERAL REPUBLIC OF GERMANY
'Bericht des Deutschen Wetterdienstes ueber die Auswirkungen des Reaktorunfalles in der UdSSR auf den Radioaktivitaetsgehalt von Luft und Niederschlag der Bundesrepublik Deutschland'
6
'Auswirkungen des Reaktorunfalls in Tschernobyl auf die Bundesrepublik Deutschland' (1987) Veroeffentlichungen der Strahlenschutzkommission Band 7. Gustav Fischer Verlag, Stuttgart New York.
'Ergebnisse von Radioactivitaetmessungen nach dem Reaktorunfall in Tschernobyl' I. Winkelmann et al. (1986) Institut fur Stralenhygiene des BGA, Neuherberg, ISH-HEFT 99
'Die Radioaktivitaet der bodennahen Luft der Bundesrepublik Deutschland im Zeitraum 29.4 - 10.05.1986' (1986) W. Weiss et al. Institut fuer Atmosphaerische Radioaktivitaet, Freiburg.
'Der Reaktorunfall von Tschernobyl' L.A. Koenig et al. (1986) Kernforschungszentrum Karlsruhe, KfK 4115.
Personal communication with Dr. H. Bonka from 'Lehrgebiet Strahlenschutz in der Kerntechnik Rhein.-Westf. Technische Hochschule, Aachen'
Personal ~ommunication with Dr. A. Reiniking from 'Isotopenlaboratourium der Universitaet Goettingen.
* FRANCE
Tape from "Institut de Protection et de Suret~ Nucleaire" CEA Fontenay-aux-Roses. Contact: Dr. D. Robeau.
'L'accident de Tchernobyl, revision 3' (1986) rapport IPSN 2/86.
'Tableaux Mensuels des Mesures, Mai 1986' (1986) Service Central de Protection centre les Rayonnements Ionisants. B.P. 78110 Le Vesinet.
* GREECE
Diskette from Nuclear Research Centre "Democritus", 15310 Aghia Paraskevi Attikis, ATHENS. Contact: Dr. P. Kritidis CEC Contract No RCN EN 8705893M
'The consequences of the Chernobyl nuclear accident in Greece' (1986). Greek Atomic Energy Commission, Nuclear Research Centre "Democritus", DEMO 86/4.
* HUNGARY
7
'Monitoring the radiation consequences due to the disaster at the Chernobyl nuclear facility from april 28 to june 12, 1986' A. Andrasi et al. (1986) Central Research Institute for Physics, Budapest, KFKI-1986-49/K
* FINLAND
'Airborne radioactivity in Finland after the Chernobyl accident in 1986' (1987) Finnish Centre for Radiation and Nuclear Safety STUK-A56.
* ITALY
'Misure effettuate nell'anno 1986 dai laboratori dell'ENEA su campioni ambientali e della catena alimentare in seguito all'incidente di chernobyl' (1989) ENEA Vol 1 (Saluggia)
'Misure effettuate nell'anno 1986 dai laboratori dell'ENEA su campioni ambientali e della catena alimentare in seguito all'incidente di chernobyl' (1989) ENEA Vol 2 (Bologna)
'Misure effettuate nell'anno 1986 dai laboratori dell'ENEA su campioni ambientali e della catena alimentare in seguito all'incidente di chernobyl' (1989) ENEA Vol 3 (Bologna)
'Misure effettuate nell'anno 1986 dai laboratori dell'ENEA su campioni ambientali e della catena alimentare in seguito all'incidente di chernobyl' (1989) ENEA Vol 5 (Casaccia)
'Misure effettuate nell'anno 1986 dai laboratori dell'ENEA su campioni ambientali e della catena alimentare in seguito all'incidente di chernobyl' (1989) ENEA Vol 6 (Casaccia)
'Misure effettuate nell'anno 1986 dai laboratori dell'ENEA su campioni ambientali e della catena alimentare in seguito all'incidente di chernobyl' (1989) ENEA Vol 9 (Trisaia)
* IRELAND
Personal contact with J. Cunningham from Nuclear Energy Board, Clonskeagh Road, DUBLIN 14.
'Chernobyl, its effect on Ireland' (1987) Nuclear Energy Board.
* the NETHERLANDS
Diskette from 'Rijksinstituut voor Volksgezondheid en Milieu' Postbox 1, 3720 BA BILTHOVEN. Contact: Dr. R. Blaauwboer
8
CEC contract No RCN EN 8704692M
'Werkdocumenten, gebruikt bij het opstellen van het CCRX-rapport "De radioactieve besmetting in Nederland ten gevolge van het kernreactorongeval in Tsjernobyl"' Dee! 1. ( 198 6)
* NORWAY
'Tsjernobyl-ulykken' (1987) Norges Offentlige Utredninger NOU 1987:1
* SPAIN
'Informe sobre las consecuencias radiologicas en Espana del accidente de la C.N. de Chernobyl' Consejo de Seguridad Nuclear CSN/IPR/3/86 Julio 1986
* SWEDEN
'Radioactive particulates in air and precipitation in sweden, second quarter 1986' L.-E. De Geer et al. FOA report C 20629-9.2.
* SWITZERLAND
'Radioaktivitaetsmessungen in der Schweiz nach Tschernobyl und ihre wissenschaftliche interpretation" Band 1 (1986) Proceedings meeting, Bern, 20-22 Ooctober 1986.
* UNITED KINGDOM
Magnetic tape from the National Radiological Protection Board, HARWELL, Didcot OXON OX 11 ORA. Contact: Mrs. J. Brown CEC contract No 3087-86-12 ED ISP GB
'Environmental radioactivity measurements at BNL during the year following the Chernobyl accident' R. Hancock et al. (1987). Central Electricity Generating Board, Berkeley. TPRD/B/0968/R87.
'Chernobyl and Scotland - Results of analyses carried out by NRPB Scottish Centre' (1987) D.M. Smith. NRPB-M142
'Observations on radioactivity from the Chernobyl accident' R.S. Cambray et al. (1987) United Kingdom Atomic Energy Authority, AERE R 12462.
9
APPENDIX 1
Concentration of I-131 and Cs-137 in aerosol particles
E+.3
E+2
,.,......,
1'
0 E
""-... cr
E+l
(l)
...
_ z 0 E+
O .-
--I- <:
e::::
I- z w
E-1
u z 0 u ,....
. E
-2
-
E-3
-
E-4
-
27
29
AP
R I
I_
. ... ,.--
.---
-
.---
-
3
II~-I<')~
I~'
L
--
,_
1--
-
5 7
I I
I
9 1
1
I i ; ; i I I l j I i l I ~ I i l ! .-
--I I ;
-
I 13
15
19
86
(' <
--1
~ 7
t-t
R I
') 0
~
[+3
___
____
__ ::
'_:_
_·--
-~-~
~' ~----------------,
E+2
E -t
1 -
E+O
-E-
1
r--
E-2
-
r--
--
E--
3 -
--
-·
ItT
E
-4-.
......
-n-
. ' I
I I
I I
I
27
29
3 5
7 9
11
13
15
AP
PIL
t\A
A. v
1
98
6
.......
0
AER
OSO
L PA
RTI
CLE
S M
EASU
RIN
G
UN
ITS
=
BQ
/M3
LATI
TUD
E LO
NG
TITU
DE
DENM
ARK
RIS
OE
55
. 70
000
12
.07
00
0
DA
TE
HOUR
D
UR
ATI
ON
I-
13
1
CS
-134
C
S-1
37
86
/04
/27
2
4:0
0
24
.00
1
. 00
0000
0
.24
00
00
8
6/0
4/2
8
24
:00
2
4.0
0
0.0
04
60
0
0.0
00
54
0
0.0
00
98
0
86
/04
/29
1
2:0
0
12
.00
0
.01
47
00
0
.00
43
00
0
.00
74
00
8
6/0
4/2
9
24
:00
1
2.0
0
0.0
00
61
0
0.0
00
09
0
86
/04
/30
2
4:0
0
24
.00
0
.00
07
50
0
.00
01
00
0
.00
02
80
8
6/0
5/0
1
24
:00
2
4.0
0
0.0
00
53
0
0.0
00
20
0
86
/05
/02
2
4:0
0
24
.00
0
.01
76
00
0
.00
02
20
8
6/0
5/0
3
24
:00
2
4.0
0
0.2
23
90
0
0.0
02
12
0
0.0
03
56
0
86
/05
/04
1
2:0
0
12
.00
0
.41
00
00
0
.01
42
00
0
.02
27
00
8
6/0
5/0
4
24
:00
1
2.0
0
0.2
64
30
3
0.0
14
34
2
0.0
23
96
6
86
/05
/05
1
2:0
0
12
.00
0
.36
20
00
0
.00
96
50
0
.01
54
40
8
6/0
5/0
5
24
:00
1
2.0
0
0.2
80
00
0
0.0
04
60
0
0.0
07
41
0
86
/05
/06
1
2:0
0
12
.00
0
.33
40
00
0
.00
73
00
0
.01
24
00
8
6/0
5/0
6
24
:00
1
2.0
0
0.1
64
00
0
0.0
03
90
0
0.0
06
40
0
86
/05
/07
2
4:0
0
24
.00
0
.49
60
00
0
.08
24
00
0
.15
44
00
8
6/0
5/1
1
24
:00
9
6.0
0
0.0
17
90
2
0.0
07
96
4
0.0
14
44
9
86
/05
/13
2
4:0
0
48
.00
0
.00
42
99
0
.00
04
64
0
.00
07
39
8
6/0
5/1
4
24
:00
2
4.0
0
0.0
08
25
2
0.0
01
23
6
0.0
02
27
2
86
/05
/15
2
4:0
0
24
.00
0
.00
32
45
0
.00
04
87
0
.00
08
81
8
6/0
5/1
6
24
:00
2
4.0
0
0.0
01
50
5
0.0
00
16
9
0.0
00
29
2
86
/05
/17
2
4:0
0
24
.00
0
.00
27
72
0
.00
04
51
0
.00
07
83
8
6/0
5/1
8
24
:00
2
4.0
0
0.0
01
66
4
0.0
00
38
8
0.0
00
74
5
86
/05
/19
2
4:0
0
24
.00
0
.00
22
48
0
.00
13
67
0
.00
24
21
8
6/0
5/2
0
24
:00
2
4.0
0
0.0
02
50
7
0.0
01
43
9
0.0
02
59
9
86
/05
/21
2
4:0
0
24
.00
0
.00
20
07
0
.00
07
83
0
.00
13
23
8
6/0
5/2
2
24
:00
2
4.0
0
0.0
02
81
0
0.0
01
02
2
0.0
01
77
3
86
/05
/25
2
4:0
0
72
.00
0
.00
18
05
0
.00
12
21
0
.00
22
75
8
6/0
5/2
6
24
:00
2
4.0
0
0.0
01
02
9
0.0
00
74
9
0.0
01
30
0
86
/05
/27
2
4:0
0
24
.00
0
.00
05
17
0
.00
03
15
0
.00
05
94
8
6/0
5/2
8
24
:00
2
4.0
0
0.0
00
48
2
0.0
00
19
6
0.0
00
33
0
86
/05
/29
2
4:0
0
24
.00
0
.00
05
33
0
.00
01
46
0
.00
03
30
z 0 I
<{
cr:
1- z w
u z 0 u
Et3
E+2
E+l
EtO
E-1
E-2
E-3
E-4
1-13
1
TTTJ
TTT,
-rro
27
29
APR
IL
I I
I
**
AACH
EN
(OW
O)
....---
....-
-
~ 1
-- 1
-t-
f.-
-f.-
--
~
I I
I I
I I
I I
rp rp
T
f
3 5
7 9
11
MAY
E+
JI
E+2
Etl
EtO
E-1
::-2
E-3
T{
TIT
jTT
Tfl
l q
E -4
13
15
CS
-137
I T
19
86
A
PRIL
*-*
AACH
EN
(OW
D)
1-
....--
-
1--
f.-
-
f-
.---
I--
1-
I I
1 I
I I
I I
I I
I
3 5
7 9
11
MAY
I I
I
13
15
19
86
......
N
AER
OSO
L PA
RTI
CLE
S M
EASU
RIN
G
UN
ITS
= B
Q/M
3 LA
TITU
DE
LON
GTI
TUD
E FE
DER
AL
REP
UB
LI
AA
CHEN
( D
WD)
50
. 76
000
6.1
00
00
DA
TE
HOUR
D
UR
ATI
ON
I-
13
1
CS
-134
C
S-1
37
86
/05
/02
0
8:0
0
24
.00
1.
905
000
0.5
92
00
0
1.
1840
00
86
/05
/03
0
8:0
0
24
.00
2
.25
70
00
0
.59
20
00
1
. 22
1000
8
6/0
5/0
4
08
:00
2
4.0
0
0.6
84
00
0
0.2
00
00
0
0.4
11
00
0
86
/05
/05
0
8:0
0
24
.00
0
.07
40
00
0
.01
80
00
8
6/0
5/0
6
08
:00
2
4.0
0
0.0
54
00
0
0.0
22
00
0
0.0
44
00
0
86
/05
/07
0
8:0
0
24
.00
0
.04
00
00
0
.00
81
00
0
.01
50
00
8
6/0
5/0
8
08
:00
2
4.0
0
0.0
08
50
0
0.0
01
20
0
0.0
02
40
0
86
/05
/09
0
8:0
0
24
.00
0
.00
67
00
0
.00
05
00
0
.00
12
00
8
6/0
5/1
0
08
:00
2
4.0
0
0.0
05
20
0
0.0
00
70
0
86
/05
/11
0
8:0
0
24
.00
0
.00
63
00
0
.00
07
00
0
.00
26
00
8
6/0
5/1
2
08
:00
2
4.0
0
0.0
06
00
0
0.0
01
00
0
0.0
01
50
0
86
/05
/19
0
8:0
0
24
.00
0
.00
29
00
0
.00
08
20
0
.00
15
40
8
6/0
5/2
6
08
:00
2
4.0
0
0.0
01
70
0
0.0
00
77
0
z 0
1-<( 0::: 1-z w u z 0 u
14
CS-137 ** AACHEN (RWTH) [+3~----------------------------------~
1
1
EtO i 1
i ~
~ I
E-1 l 1 1 1 1 I I
E-2 l l j
i E-3 ~
i j
i E-4 l•••t'''l'''l'''l'''l'' I' I
2 7 29 3
APRIL MAY
,, I' I I' 'I' 'I" I" I" I"'
5 7 9 11 13 15
1986
AER
OSO
L PA
RTI
CLE
S
FED
ERA
L R
EPU
BLI
DA
TE
HOUR
86
/05
/01
1
7:4
5
86
/05
/02
08
: 15
8
6/0
5/0
2
12
:39
8
6/0
5/0
2
14
:52
8
6/0
5/0
2
17
:25
8
6/0
5/0
2
19
:45
8
6/0
5/0
3
08
:21
8
6/0
5/0
3
11:
19
86
/05
/03
1
3:3
0
86
/05
/03
1
6:0
0
86
/05
/03
1
8:3
5
86
/05
/03
2
1:5
4
86
/05
/04
1
5:0
0
86
/05
/05
0
9:2
5
86
/05
/06
19
: 10
8
6/0
5/0
7
09
:40
8
6/0
5/0
7
18
:00
8
6/0
5/0
8
07
:30
8
6/0
5/0
9
08
:45
8
6/0
5/1
0
10
:00
8
6/0
5/1
1
17
:45
8
6/0
5/1
2
18
:30
8
6/0
5/1
3
19
:00
MEA
SURI
NG
U
NIT
S =
BQ
/M3
AA
CHEN
(R
WTH
)
DU
RA
TIO
N
I-1
31
8.5
5
13
.30
2
.00
2
.00
2
.00
2
.00
1
2.0
0
2.0
0
2.0
0
2.0
0
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00
0
0.3
00
00
0
0.0
30
00
0
0.0
09
70
0
0.0
02
50
0
0.0
02
00
0
0.0
02
20
0
LON
GTI
TUD
E 1
4.4
16
66
CS
-137
23
.00
00
00
2
0.0
00
00
0
23
.00
00
00
9.
700
000
1. 7
0000
0 1.
000
000
0. 1
5000
0 0
.06
00
00
1.
200
000
7.9
00
00
0
3.6
00
00
0
1. 4
0000
0 0
.90
00
00
0
.80
00
00
0
.20
00
00
0
.80
00
00
0
.80
00
00
0.
700
000
0.0
50
00
0
0.0
21
00
0
<
0.0
05
20
0
0.0
04
30
0
0.0
04
70
0
N ......
(J1
E+J
I -1
3 1
**
U
ST
I N
.L.
-
Et2
,........,
I"')
E
"-.._
E
t1
cr
m
'--"
r-
z 0 E
tO
I-
<{
0:::
I- z
t-
w
[-1
u z 0 u
E-2
E-3
I I
I I
I I
'I
E·-
4 I
I I
I I
I 'I
27
29
3 5
7 9
APR
IL
MAY
-··
I I
1 1
I I
'I
c s --1
3 7
E
t3------·-
E+2
E + 1
-
EtO
E-1
E-2
E-3
E -4
1'
...-
rr'T
TT
I
13
15
21
2~
19
86
A
PRIL
**
US
TI
N.L
.
.--:-
t-
I I
I I
I I
I I
I I
I I
I f
5 7
9 1
1 13
15
MAY
19
86
AER
OSO
L PA
RTI
CLE
S M
EASU
RIN
G
UN
ITS
= B
Q/M
3 LA
TITU
DE
LON
GTI
TUD
E CZ
ECH
OSL
OV
AK
IA
UST
I N
. L.
50
.68
33
3
14
.00
00
0
DA
TE
HO
UR
DU
RATI
ON
I-
13
1
CS
-134
C
S-1
37
86
/05
/01
0
5:0
0
24
.00
5
.24
00
00
1
.40
00
00
2
.60
00
00
8
6/0
5/0
2
05
:00
2
4.0
0
4.8
10
00
0
1.
4300
00
2.6
00
00
0
86
/05
/03
0
5:0
0
24
.00
0.
196
000
0.0
13
00
0
0.0
19
00
0
86
/05
/04
0
5:0
0
24
.00
1.
300
000
0.5
02
00
0
0.9
31
00
0
86
/05
/05
0
5:0
0
24
.00
1.
320
000
0.5
60
00
0
1. 0
4000
0
z 0 I
<(
cr
1- z w
u z 0 (_)
E+
3r-
__
_ I_-
_1_3
_1 __
_ *_* _
_ B_U_D_A_P_E_S_~T __
____
____
~
E+2
E + 1
-
.---
r-
,_
..--
-r--
E+O
.--
t-
1-
E-1
-r---
t--
E-2
E-3
E-4
1
I I
I l
l I
I I
I rr
rr
rorT
"'T
'
27
29
3 5
7 9
11
13
15
AP
RIL
M
AY
19
86
E+3
,..--_
c_s -
1 3
7
**
BUD
APE
ST
--
E+2
E + 1
-
E+O
r-
.---
r--
.--
1--
r-
1--
1--
E-1
~
E-2
E-3
E-4
r
I I
l T
I
I l
I I
'I
l I
I I
I
'2 7
2 9
3 5
7 9
1 1
13
15
AP
RIL
M
AY
19
86
AER
OSO
L PA
RTI
CLE
S M
EASU
RIN
G
UN
ITS
= B
Q/M
3 LA
TITU
DE
LON
GTI
TUD
E HU
NGAR
Y B
UD
APE
ST
47
.50
00
0
19.
1000
0
DA
TE
HOUR
D
URA
TIO
N
I-1
31
C
S-1
34
CS
-137
86
/04
/29
0
8:0
0
24
.00
0
.00
05
00
0
.00
00
50
8
6/0
4/3
0
08
:00
2
4.0
0
0.9
00
00
0
0. 1
6000
0 0
.30
00
00
8
6/0
5/0
1
08
:00
2
4.0
0
1.
9000
00
0.3
00
00
0
0.6
50
00
0
86
/05
/02
0
8:0
0
24
.00
4.
100
000
0.8
00
00
0
1.4
00
00
0
86
/05
/03
0
8:0
0
24
.00
0.
750
000
0. 1
3000
0 0
.26
00
00
8
6/0
5/0
4
08
:00
2
4.0
0
1.
6000
00
0.3
40
00
0
0.6
20
00
0
86
/05
/05
0
8:0
0
24
.00
0
.42
00
00
0
.05
00
00
0
.09
00
00
8
6/0
5/0
6
08
:00
2
4.0
0
0.4
40
00
0
0.0
56
00
0
0. 1
0000
0 8
6/0
5/0
7
08
:00
2
4.0
0
3.7
00
00
0
0.5
80
00
0
1.
2000
00
86
/05
/08
0
8:0
0
24
.00
2
.20
00
00
0
.33
00
00
0
.69
00
00
8
6/0
5/0
9
08
:00
2
4.0
0
0. 7
5000
0 o.
1400
00
0.2
90
00
0
86
/05
/10
0
8:0
0
24
.00
0
.05
40
00
0
.00
60
00
0
.00
90
00
8
6/0
5/1
1
08
:00
2
4.0
0
0.0
51
00
0
0.0
06
00
0
0.0
10
00
0
220
221
APPENDIX 2
Concentration of total I-131 (gas + aerosol particles)
222
T 0 TAL
Et3 1-131 ** AACHEN (RWTH)
E+2
---. 1'0 E
""' Etl r-
CY r-co '-./
z 0 E+O r-
I-<:( ~
0::: .--
I-z w E-1 (_)
~
z 0
r-.--
u ,__ r-
I--
E-2
E-3
E·-4 I I I I I 'I I I 'I r I I 'I 'I 'I 'I I'" I
27 29 3 7 9 I 1 13 15
APRIL MAY 1986
GA
S +
AER
OSO
L PA
RTI
CLE
S M
EASU
RIN
G
UN
ITS
= B
Q/M
3
FED
ERA
L R
EPU
BLI
A
ACH
EN
(RW
TH)
DA
TE
HOUR
D
UR
ATI
ON
I-
13
1
86
/05
/01
1
7:4
5
8.5
5
1. 0
0000
0 8
6/0
5/0
2
08:
15
13
.30
1
1.0
00
00
0
86
/05
/02
1
2:3
9
2.0
0
18
.00
00
00
8
6/0
5/0
2
14
:52
2
.00
1
2.0
00
00
0
86
/05
/02
1
7:2
5
2.0
0
7.8
00
00
0
86
/05
/02
1
9:4
5
2.0
0
8.2
00
00
0
86
/05
/03
0
8:2
1
12
.00
6
.80
00
00
8
6/0
5/0
3
11:
19
2.0
0
5.2
00
00
0
86
/05
/03
1
3:3
0
2.0
0
7.9
00
00
0
86
/05
/03
1
6:0
0
2.0
0
7. 7
0000
0 8
6/0
5/0
3
18
:35
2
.00
4
.50
00
00
8
6/0
5/0
3
21
:53
2
.00
3
.80
00
00
8
6/0
5/0
4
10
:00
11
. 30
0
.53
00
00
8
6/0
5/0
4
15
:00
4
.00
0
.36
00
00
8
6/0
5/0
4
19
:50
4
.00
0
.39
00
00
8
6/0
5/0
5
09
:25
1
2.4
0
0.4
00
00
0
86
/05
/06
19
: 10
8
.00
0
.44
00
00
8
6/0
5/0
7
09
:40
14
. 10
0.
130
000
86
/05
/07
1
8:0
0
8.0
0
0.0
80
00
0
86
/05
/08
0
7:3
0
13
.00
0
.05
00
00
8
6/0
5/0
9
08
:45
1
5.0
0
0.0
40
00
0
86
/05
/10
1
0:0
0
25
.00
0
.03
00
00
8
6/0
5/1
1
17
:45
3
1.3
0
0.0
20
00
0
86
/05
/12
1
8:3
0
24
.30
0
.03
00
00
8
6/0
5/1
3
19
:00
2
4.0
0
0.0
20
00
0
LATI
TUD
E 50
. 76
000
CS
-134
LON
GTI
TUD
E 6.
100
00 .
CS
-137
N
N w
224
T 0 TAL
Et3 I -13 1 ** BERLIN-WEST (WABOLU)
E+2
,..,.-... I")
E '-.. Etl o-
co ..._., ...--
z 0 EtO ~ <( 0:::: ~ z w E-1 u r- r-
z 0 u
E-2 -
E-3 r-
E-4 I I I l I I I I I 'T I I I I I I I I 'I
27 29 3 7 9 11 13 15
APRIL MAY 1986
GAS
+ A
ERO
SOL
PAR
TIC
LES
MEA
SURI
NG
U
NIT
S =
B
Q/M
3
FED
ERA
L R
EPU
BLI
B
ERLI
N-W
EST
(WA
BOLU
)
DA
TE
HOUR
D
URA
TIO
N
I-1
31
86
/04
/29
1
4:2
0
24.
16
0.0
70
00
0
86
/04
/30
0
8:2
1
18
.01
3.
100
000
86
/04
/30
1
0:5
0
2.2
9
13
.00
00
00
8
6/0
4/3
0
13
:23
2
.33
2
0.0
00
00
0
86
/04
/30
1
5:0
8
1.
43
14
.00
00
00
8
6/0
4/3
0
16
:45
1
. 35
3
.00
00
00
8
6/0
4/3
0
18
:45
2
.00
0
.60
00
00
8
6/0
5/0
1
07
:40
1
2.5
5
<
0. 1
0000
0 8
6/0
5/0
1
12
:00
4
.20
<
0.
100
000
86
/05
/01
1
7:5
0
5.5
0
<
0. 1
0000
0 8
6/0
5/0
2
05
:50
1
2.0
0
<
0. 1
0000
0
LATI
TUD
E 5
2.3
30
00
CS
-134
LON
GTI
TUD
E 1
3.4
20
00
CS
-137
N
N
V
l
226
T 0 T A L
I -1 31 ** KARLSRUHE
E+2
---I"') r-
E ........_
o- E+1 1-
(l) 1-c--...._,.
,-
z 0
EtO -
l--<( c:r: I- 1-
z r-
w E-1 u -
1- 1-z 1-~--
0 u
E-2
E-3
E-4 I I I I I I I I I I I I, T I, I I I I I
27 29 7 9 1 1 13 15
.APRIL MAY 1986
GA
S +
AER
OSO
L PA
RTI
CLE
S M
EASU
RIN
G
UN
ITS
= B
Q/M
3
FED
ERA
L R
EPU
BLI
K
ARL
SRU
HE
DA
TE
HOUR
D
URA
TIO
N
I-1
31
86
/04
/30
1
7:0
0
24
.00
0.
180
000
86
/05
/01
1
1:0
0
18
.00
0
.08
40
00
8
6/0
5/0
1
17
:00
6
.00
2
0.0
00
00
0
86
/05
/02
1
1:0
0
18
.00
2
4.0
00
00
0
86
/05
/02
1
7:0
0
6.0
0
30
.00
00
00
8
6/0
5/0
3
11
:00
1
8.0
0
10
.50
00
00
8
6/0
5/0
3
17
:00
6
.00
9
.60
00
00
8
6/0
5/0
4
11
:00
1
8.0
0
5. 7
0000
0 8
6/0
5/0
4
17
:00
6
.00
1
. 40
0000
8
6/0
5/0
5
11
:00
1
8.0
0
4. 7
0000
0 8
6/0
5/0
5
17
:00
6
.00
2.
750
000
86
/05
/06
1
1:0
0
18
.00
2
.85
00
00
8
6/0
5/0
6
17
:00
6
.00
2
.95
00
00
8
6/0
5/0
7
11
:00
1
8.0
0
1.
5000
00
86
/05
/07
1
7:0
0
6.0
0
0.3
70
00
0
86
/05
/08
1
1:0
0
18
.00
0
.22
00
00
8
6/0
5/0
9
11
:00
2
4.0
0
o. 13
0000
8
6/0
5/1
0
11
:00
2
4.0
0
0.0
81
00
0
86
/05
/11
1
1:0
0
24
.00
0
.06
50
00
8
6/0
5/1
2
11
:00
2
4.0
0
0.0
59
00
0
86
/05
/14
1
1:0
0
48
.00
0
.09
40
00
8
6/0
5/1
6
11
:00
4
8.0
0
0.0
54
00
0
86
/05
/18
1
1:0
0
48
.00
0
.02
00
00
LATI
TUD
E 4
9.0
00
00
CS
-134
LON
GTI
TUD
E 8
.67
00
0
CS
-137
N
N
-.....,
J
228
T 0 TAL
I -1 3 1 ** NEUHERBERG E+3 ------------
E+2
,........ .--I") 1-
E ~ E+l --o-
m 1-
""-/ r-
z -0 E+O -t-<:( er:: t-z Ld E-1 (_)
r---1-
z .--0 u
E-2
E-3
!:-4 • I I I I I I I I I I I I I I I I I I
27 29 3 5 7 9 1 1 13 15
APRIL MAY 1986
GAS
+ A
ERO
SOL
PAR
TIC
LES
MEA
SURI
NG
U
NIT
S =
BQ
/M3
FED
ERA
L R
EPU
BLI
N
EUH
ERBE
RG
DA
TE
HOUR
D
UR
ATI
ON
I-
13
1
86
/04
/30
1
0:0
0
20.
15
3. 1
0000
0 8
6/0
4/3
0
14
:30
4
.00
5
2.0
00
00
0
86
/04
/30
18
: 15
3.
15
33
.60
00
00
8
6/0
5/0
1
11
:45
1
7.0
5
29
.80
00
00
8
6/0
5/0
1
18
:00
6.
10
48
.00
00
00
8
6/0
5/0
1
20:
10
2. 1
0 3
8.2
00
00
0
86
/05
/02
0
9:0
0
12
.50
2
3.9
00
00
0
86
/05
/02
1
0:0
0
1.
00
16
.20
00
00
8
6/0
5/0
2
21
:55
8
.40
12
. 70
0000
8
6/0
5/0
3
15
:40
1
7.3
5
10
.40
00
00
8
6/0
5/0
4
16:
15
24
.35
5.
700
000
86
/05
/05
1
9:4
5
27
.25
3
.47
00
00
8
6/0
5/0
6
09
:20
1
3.3
5
1. 6
1000
0 8
6/0
5/0
7
17
:00
3
1.3
0
2.6
40
00
0
86
/05
/08
1
3:0
0
20
.00
0
.98
00
00
8
6/0
5/0
9
18
:00
2
9.0
0
0. 1
0900
0 8
6/0
5/1
0
19
:00
2
4.2
0
0. 1
2300
0 8
6/0
5/1
1
16:
10
21
.05
0
.09
40
00
8
6/0
5/1
2
19
:30
27
. 10
0
.02
89
00
8
6/0
5/1
3
16
:40
2
1.0
0
0.0
56
60
0
86
/05
/15
1
6:2
0
47
.30
0
.02
43
00
8
6/0
5/2
1
13
:00
1
40
.40
0
.01
38
60
LATI
TUD
E 48
. 13
000
CS
-134
LON
GTI
TUD
E 1
1.5
80
00
CS
-137
N
N
1..0
230
T 0 T A L
1-131 ** SACLAY E + .3 r------------------------ -------- ---------------
E+2
r--... I")
E ............ E+l cr m .....__-
-z 0 EtO ...__ <:(
IY' r- .-
z ,_ Ld E-1
1-
(_)
z 0 C..)
E-2-
E-3
[ --4 +r-r-rrl 'I"'T"''"'"''I........-rliM""T"r"'I"T'T'TI...-.J.r, lr"T'11 rln-rl-,1,-r.l-.lrnl.-.lr-rrr"n I.,..,T J.,-.-,-1 rLn-T-1-r'rnl-,ln-1,.-,J,.,.--.-rrr 1.,..,1 rT"I'"'!"'"I ~,TTT1
27 29 3 ~ 7 9 11 1.3 15
APRIL MAY 1986
GAS
+ A
ERO
SOL
PAR
TIC
LES
MEA
SURI
NG
U
NIT
S =
BQ
/M3
LATI
TUD
E LO
NG
TITU
DE
FRA
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