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Yb:CaF Yb:CaF 2 2 Diode-Pumped Regenerative Diode-Pumped Regenerative Amplifier: Study and Optimization of Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st October 2010 S. Ricaud 1,4 , F. Druon 1 , D. N. Papadopoulos 1,2 , P. Camy 3 , J. L. Doualan 3 , R. Moncorgé 3 , M. Delaigue 4 , Y. Zaouter 4 , A. Courjaud 4 , P. Georges 1 and E. Mottay 4 1 Laboratoire Charles Fabry de l'Institut d'Optique (LCFIO), Palaiseau, France 2 Institut de la Lumière Extrême (ILE), Palaiseau, France 3 Centre de recherche sur les Ions, les Matériaux et la Photonique (CIMAP), Caen, France 4 Amplitude Systèmes, Pessac, France [email protected]

Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

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Page 1: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

Yb:CaFYb:CaF22 Diode-Pumped Regenerative Diode-Pumped Regenerative Amplifier: Study and Optimization of Amplifier: Study and Optimization of

Pulse Duration Versus Repetition RatePulse Duration Versus Repetition Rate

ICUIL, Watkins Glen, 26th September-1st October 2010

S. Ricaud1,4, F. Druon1, D. N. Papadopoulos1,2, P. Camy3, J. L. Doualan3, R. Moncorgé3, M. Delaigue4, Y. Zaouter4,

A. Courjaud4, P. Georges1 and E. Mottay4

1 Laboratoire Charles Fabry de l'Institut d'Optique (LCFIO), Palaiseau, France2 Institut de la Lumière Extrême (ILE), Palaiseau, France

3 Centre de recherche sur les Ions, les Matériaux et la Photonique (CIMAP), Caen, France

4 Amplitude Systèmes, Pessac, France

[email protected]

Page 2: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

2ICUIL 2010, Watkins Glen 2

OutlineOutline

• Yb3+:CaF2 crystal- Spectroscopy- Thermal properties

• Ultrashort amplifier- Experimental setup- Q-switch regime- Regenerative amplifier configuration

• Conclusion

Page 3: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

3ICUIL 2010, Watkins Glen 3

OutlineOutline

• Yb3+:CaF2 crystal- Spectroscopy- Thermal properties

• Ultrashort amplifier- Experimental setup- Q-switch regime- Regenerative amplifier configuration

• Conclusion

Page 4: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

4ICUIL 2010, Watkins Glen 4

““A new old laser material A new old laser material ””

First ceramic and diode-pumped solid-state lasers were based on CaF2 host matrix !!!

(Artist representation)

R. J. Keyes, et al. “Injection Luminescent pumping of CaF2:U3+ with GaAs diode lasers”Appl. Phys. Lett. 4 pp 50-51. (1964).

S.E. Hatch, et al.  “Hot-pressed polycrystalline CaF2:Dy2+ laser ” Appl. Phys. Lett. 5 pp 153-154. (1964)

M. Siebold, et al.“Yb:CaF2 – A New Old Laser Material”Appl. Phys. B (2009).

Doped Yb:CaF2 up to ϕ200 mm

(Korth GmbH)

V. Petit, et al.“CW and tunable laser operation of Yb3+ doped CaF2”Appl. Phys. B (2004).

Page 5: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

5ICUIL 2010, Watkins Glen 5

SpectroscopySpectroscopy

Broad absorption and fluorescence spectra

ClustersCrystalline reorganization

Charge compensation

YbYb3+3+CaCa2+2+

Hexameric cluster

V. Petit et al (Appl. Phys. B, 2004)

• Diode pumping• Tunability / ultrashort pulses• Long emission lifetime (2.4 ms)

Page 6: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

6ICUIL 2010, Watkins Glen 6

Thermal propertiesThermal properties

Undoped crystal~ 2.7%-Yb-doped

crystal

Thermal conductivity (W.m-

1.K-1)9.7 6

Thermo-optic coefficient (10-

6 K-1)- 17.8 - 11.3

S-FAP

YAG

Y2O3

LSOKGW

glass

YVO4

YSOBOYS

SrF2

CaF2

CALGO

SYS

Favorabledirections

Page 7: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

7ICUIL 2010, Watkins Glen 7

Potential laser materialPotential laser material

- Smooth optical bands-Relatively large cross sections-Cryo-cooled perspective

Femtosecond pulses (**)

- High thermal conductivity- High quality crystal with very- Low parasitic nonradiative effect

Energetic pulses (*) - Long fluorescence lifetime (2.4 ms)- High quality crystal with large diameter

*M.Siebold et al "Terawatt diode-pumped Yb:CaF2 laser”, Opt. Letters 33(23), 2770–2772 (2008)

**F. Friebel et al "Diode-pumped 99 fs Yb:CaF2 oscillator”, Opt. Letters 34(9), 1474–1476 (2009)

***J. Boudeile et al "Thermal behaviour of ytterbium-doped fluorite crystals under high power pumping”, Opt. Express 16, 10098-10109 (2008)

High average power pulses (***)

•Yb:CaF2 based HEC-DPSSL broadband CPA pump for the ILE front end OPCPA system

•Diode-pumped regenerative amplifier

Page 8: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

8ICUIL 2010, Watkins Glen 8

OutlineOutline

• Yb3+:CaF2 crystal- Spectroscopy- Thermal properties

• Ultrashort amplifier- Experimental setup- Q-switch regime- Regenerative amplifier configuration

• Conclusion

Page 9: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

9ICUIL 2010, Watkins Glen 9

Experimental setupExperimental setup

Diode-pumped CPA laser chain

Page 10: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

10ICUIL 2010, Watkins Glen 10

Q-switch regime (non injected)Q-switch regime (non injected)

In Q-switch regime : - maximal output energy 1.8 mJ at 100 Hz- maximal average power : 850 mW above 800 Hz- maximal spectral bandwidth : 16 nm centered at 1040 nm at 500 Hz

Normalized output pulse spectrum at

500 Hz

Optimal repetition rate energy/power : 500 Hz (fluo lifetime 2.4 ms)

Optimization of the injection spectrum : broadband oscillator centered around 1043 nm (Yb:GALGO)

Page 11: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

11ICUIL 2010, Watkins Glen 11

- Maximum energy plateau up to 300 Hz : 1.6 mJ / 700 µJ (uncompressed / compressed)

- Higher repetition rate : 10 kHz 1.4W / 0.6W (uncompressed / compressed)

Beam profile : Gaussian shape with M2 < 1.1

Regenerative amplifier configurationRegenerative amplifier configuration

Page 12: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

12ICUIL 2010, Watkins Glen 12

Spectral Spectral bandwidthbandwidth

15 nm

Spectral shaping depending on repetition rate and extraction time

Low Δn, maximal gain ~ 1045 nmHigh Δn, maximal gain ~ 1035 nm

Spectral bandwidth up to 15 nm (below 1 kHz)

500 Hz repetition rate for different time of extraction: 1.35 µs, 300 µJ (red curve)1.7 µs, 620 µJ (blue curve)2.2 µs, 580 µJ (green curve)Short dash curve : oscillator spectrum

Page 13: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

13ICUIL 2010, Watkins Glen 13

SHG FROG trace at 500 HzSHG FROG trace at 500 Hz

At 500 Hz repetition rate : - pulse duration : 178 fs >90% temp. Strehl ratio >95% main peak - pulse energy : 1.4 mJ before compression

620 µJ after compression - optical-to-optical efficiency : 4.5 % Measured Retrieved

178 fs8.5 nm

15 nm

Page 14: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

14ICUIL 2010, Watkins Glen 14

Pulse duration vs rep. ratePulse duration vs rep. rate

-Up to 1 kHz : pulse duration below 200 fs

- 10 kHz : 400 fs, narrower spectrum shifted at 1045 nm

S. RICAUD et al“Short pulse and high repetition rate diode-pumped Yb:CaF2 regenerative amplifier”Optics Letters, Vol. 35, Issue 14, pp. 2415-2417 (July 2010)

Page 15: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

15ICUIL 2010, Watkins Glen 15

OutlineOutline

• Yb3+:CaF2 crystal- Spectroscopy- Thermal properties

• Ultrashort amplifier- Experimental setup- Q-switch regime- Regenerative amplifier configuration

• Conclusion

Page 16: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

16ICUIL 2010, Watkins Glen 16

ConclusionConclusion

- Diode-pumped room-temperature regenerative Yb:CaF2 amplifier operating at low and high repetition rate.

- Short pulses up to 1 kHz repetition rate (178 fs at 500 Hz).

- Maximum extracted energy : 1.6 mJ / 0.7 mJ (before / after compression).

- Highest average power : 1.4 W / 0.6 W (before / after compression).

- Optical to optical efficiency ranging from 5 to 10%.

…Potential for sub-100 fs pulses with spectral shaping and high order phase control …cryo-cooled setup (oscillator), multipass booster (200mJ/100Hz)

Page 17: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

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Thank you !!!

Page 18: Yb:CaF 2 Diode-Pumped Regenerative Amplifier: Study and Optimization of Pulse Duration Versus Repetition Rate ICUIL, Watkins Glen, 26 th September-1 st

18ICUIL 2010, Watkins Glen 18

1.1 % defect (992 nm) demonstrated(despite dichroic mirror)

1030 nm 1034 nm

Laser diode245 W @ 979 nm

Ø=400µm

Yb:CaF2

Dichroic mirror

50 mm triplets Mirror

R=800mm

OC

P

P

Pre

f

Spectrometer

CCD

Leak

Prism

Spectrometer

Experimental small signal gain: max 3.1Population Inversion =0.42.

DPSSL cryo Yb:CaFDPSSL cryo Yb:CaF22