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Tracking saddle-to-scission dynamics using N/Z in projectile breakup reactions SYLVIE HUDAN April 1, 2012

Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

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Page 1: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

Tracking saddle-to-scission dynamics using N/Z in projectile

breakup reactions

SYLVIE HUDANApril 1, 2012

Page 2: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Dynamical Breakup

Montoya et al., PRL73, 3070 (1994); Bocage et al., NPA676, 391 (2000)

Davin et al., PRC65, 064614 (2002); Colin et al., PRC67, 064603 (2003)

McIntosh et al., PRC81, 034603 (2010)

From Colin et al.

Observation of strongly aligned decay in mid-peripheral collisions at intermediate energies with:

Large yieldLarge relative velocity relative to fission

S. Hudan et al., PRC71, 05402 (2006)

Page 3: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Dynamical Breakup

➡ Transiently deformed nuclei➡ Early cluster production

Montoya et al., PRL73, 3070 (1994); Bocage et al., NPA676, 391 (2000)

Davin et al., PRC65, 064614 (2002); Colin et al., PRC67, 064603 (2003)

McIntosh et al., PRC81, 034603 (2010)

From Colin et al.

Observation of strongly aligned decay in mid-peripheral collisions at intermediate energies with:

Large yieldLarge relative velocity relative to fission

S. Hudan et al., PRC71, 05402 (2006)

AMD

Page 4: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Dynamical Breakup

➡ Transiently deformed nuclei➡ Early cluster production

Montoya et al., PRL73, 3070 (1994); Bocage et al., NPA676, 391 (2000)

Davin et al., PRC65, 064614 (2002); Colin et al., PRC67, 064603 (2003)

McIntosh et al., PRC81, 034603 (2010)

From Colin et al.

Observation of strongly aligned decay in mid-peripheral collisions at intermediate energies with:

Large yieldLarge relative velocity relative to fission

S. Hudan et al., PRC71, 05402 (2006)

AMD

What is the isotopic composition of those fragments?

Page 5: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Experimental Setup124Xe 124Sn 112Sn1.30 1.48 1.24

FIRST: T. Paduszynski et al., NIMA 547, 464 (2005)

124(,136)Xe + 112, 124Sn @ 49.2 MeV/AExperiment performed at GANIL (France)

N/Z

Page 6: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

BEAM

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Experimental Setup124Xe 124Sn 112Sn1.30 1.48 1.24

FIRST: T. Paduszynski et al., NIMA 547, 464 (2005)

124(,136)Xe + 112, 124Sn @ 49.2 MeV/AExperiment performed at GANIL (France)

N/Z

Page 7: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

BEAM

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Experimental Setup

• T1: Si-Si-CsI(Tl)- 2.8° ≤ θLab ≤ 6.6°- Z = 1-55; A for Z = 1-14

124Xe 124Sn 112Sn1.30 1.48 1.24

273µm Si(IP) 1001µm Si(IP) 3.3cm CsI(Tl)/PD

48 rings 16 “pies”

48 rings 16 “pies” 16 “pies”

FIRST: T. Paduszynski et al., NIMA 547, 464 (2005)

124(,136)Xe + 112, 124Sn @ 49.2 MeV/AExperiment performed at GANIL (France)

N/Z

Page 8: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

BEAM

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Experimental Setup

• T1: Si-Si-CsI(Tl)- 2.8° ≤ θLab ≤ 6.6°- Z = 1-55; A for Z = 1-14

• T2: Si-CsI(Tl)- 7.3° ≤ θLab ≤ 14.3°- Z = 1-24; A for Z=1-8

124Xe 124Sn 112Sn1.30 1.48 1.24

273µm Si(IP) 1001µm Si(IP) 3.3cm CsI(Tl)/PD

48 rings 16 “pies”

48 rings 16 “pies” 16 “pies”

16 rings (x4 quadrants) 16 “pies”

16 “pies”

3.3 cm CsI(Tl)/PD 500µm Si(IP)

FIRST: T. Paduszynski et al., NIMA 547, 464 (2005)

124(,136)Xe + 112, 124Sn @ 49.2 MeV/AExperiment performed at GANIL (France)

N/Z

Page 9: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

BEAM

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Experimental Setup

• T1: Si-Si-CsI(Tl)- 2.8° ≤ θLab ≤ 6.6°- Z = 1-55; A for Z = 1-14

• T2: Si-CsI(Tl)- 7.3° ≤ θLab ≤ 14.3°- Z = 1-24; A for Z=1-8

• LASSA: 36.4° ≤ θLab ≤ 51.5°• DEMON: n TOF

124Xe 124Sn 112Sn1.30 1.48 1.24

273µm Si(IP) 1001µm Si(IP) 3.3cm CsI(Tl)/PD

48 rings 16 “pies”

48 rings 16 “pies” 16 “pies”

16 rings (x4 quadrants) 16 “pies”

16 “pies”

3.3 cm CsI(Tl)/PD 500µm Si(IP)

FIRST: T. Paduszynski et al., NIMA 547, 464 (2005)

124(,136)Xe + 112, 124Sn @ 49.2 MeV/AExperiment performed at GANIL (France)

N/Z

Page 10: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Aligned Decay Angle between the relative velocity and the fragment “parent” velocity

ZH

ZL

α

TLF*

npvREL

vc.m.

Page 11: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Aligned Decay

• Asymmetric angular distributions• Larger asymmetry for lighter ZL

• Asymmetry persists up to ZL = 18• Similar yield for n-rich target*

Angle between the relative velocity and the fragment “parent” velocity

ZH

ZL

α

TLF*

npvREL

vc.m.

*: Backward enhancement observed in Sn+Ni for change of target and projectile

P. Russotto et al., PRC 81, 064605 (2010)

Page 12: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Isotopic Composition vs Rotation Angle

• Backward emission neutron-rich relative to forward emission

• Fragment neutron content enhanced for larger alignment

• No visible target effect of the relative neutron composition

Page 13: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Relative Velocity Dependence

90°-180°66°-90°37°-66°0°-37°

Page 14: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Relative Velocity Dependence• ⟨N⟩/Z decreases with vREL for forward decay (Coulomb effect)

• ⟨N⟩/Z increases with vREL for backward decay

90°-180°66°-90°37°-66°0°-37°

Page 15: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Relative Velocity Dependence• ⟨N⟩/Z decreases with vREL for forward decay (Coulomb effect)

• ⟨N⟩/Z increases with vREL for backward decay

• All backward decays show the same dependence with vREL

90°-180°66°-90°37°-66°0°-37°

Page 16: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Relative Velocity Dependence

More aligned decay with higher vREL ⇒ observed angular dependence

• ⟨N⟩/Z decreases with vREL for forward decay (Coulomb effect)

• ⟨N⟩/Z increases with vREL for backward decay

• All backward decays show the same dependence with vREL

90°-180°66°-90°37°-66°0°-37°

Page 17: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Time Extraction

t = 0

Page 18: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

• The rotation angle can be related to time via the rotational frequency ω:

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Time Extraction

t =α

ω

t = 0

Page 19: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

• The rotation angle can be related to time via the rotational frequency ω:

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Time Extraction

t =α

ω

t

t = 0

Page 20: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

• The rotation angle can be related to time via the rotational frequency ω:

•ω in the range 0.7-0.6 1021 rad/s corresponding to based on previous studies*.

� ≈ 40�

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Time Extraction

t =α

ω

*: G. Casini et al., PRL 71, 2567 (1993)

t = T/4

t = 0

Page 21: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

• The rotation angle can be related to time via the rotational frequency ω:

•ω in the range 0.7-0.6 1021 rad/s corresponding to based on previous studies*.

• The correlation between <vREL> and the rotation angle is monotonous (5th degree polynom parametrization).

� ≈ 40�

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Time Extraction

t =α

ω

*: G. Casini et al., PRL 71, 2567 (1993)

t = T/4

t = 0

Page 22: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

• The rotation angle can be related to time via the rotational frequency ω:

•ω in the range 0.7-0.6 1021 rad/s corresponding to based on previous studies*.

• The correlation between <vREL> and the rotation angle is monotonous (5th degree polynom parametrization).

vREL ⇒ angle ⇒ time

� ≈ 40�

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Time Extraction

t =α

ω

*: G. Casini et al., PRL 71, 2567 (1993)

t = T/4

t = 0

Page 23: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

N/Z Time Dependence

66°-90° 37°-66°0°-37°

1 zs = 10-21 s

Page 24: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

N/Z Time Dependence

• ZL = 4• Strong time dependence• Two components

66°-90° 37°-66°0°-37°

1 zs = 10-21 s

Page 25: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

N/Z Time Dependence

• ZL = 4• Strong time dependence• Two components

• ZL = 5,6• Time dependence not as pronounced as for ZL = 4

66°-90° 37°-66°0°-37°

1 zs = 10-21 s

Page 26: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

N/Z Time Dependence

• ZL = 4• Strong time dependence• Two components

• ZL = 5,6• Time dependence not as pronounced as for ZL = 4

• ZL = 8• Similar dependence for both short and long times

66°-90° 37°-66°0°-37°

1 zs = 10-21 s

Page 27: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Conclusions

Page 28: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

ConclusionsThe ⟨N⟩/Z of fragments emitted in dynamical decay is correlated with the rotation angle.Different vREL dependence are observed for forward and backward emission.For backward decays, ⟨N⟩/Z increases with vREL with a similar magnitude for all angles.Evolution of ⟨N⟩/Z over 2-3 zs (600-900 fm/c)

Page 29: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

ConclusionsThe ⟨N⟩/Z of fragments emitted in dynamical decay is correlated with the rotation angle.Different vREL dependence are observed for forward and backward emission.For backward decays, ⟨N⟩/Z increases with vREL with a similar magnitude for all angles.Evolution of ⟨N⟩/Z over 2-3 zs (600-900 fm/c)

Difference in ⟨N⟩/Z time dependence for different ZL may be related to differences in the initial di-nuclear configuration (different position relative to saddle and scission points).In the future, use of damped reactions at radioactive beam facilities?

Page 30: Tracking saddle-to-scission dynamics using N/Z in ...nuchem.iucf.indiana.edu/Presentations/SylvieHudan_APS2012.pdfSylvie Hudan, APS April Meeting 2012 April 1, 2012 Dynamical Breakup

April 1, 2012Sylvie Hudan, APS April Meeting 2012

Collaboration and AcknowledgementsIndiana University: A.B. McIntosh, S. Hudan, J. Black, D. Mercier, C.J. Metelko, R. Yanez, R.T. de Souza

GANIL: A. Chbihi

GSI: S. Bianchin, C. Schwarz, W. Trautmann

Université Laval, Québec: M.O. Frégeau, J. Gauthier, J. Moisan, R. Roy

WMU: M. Famiano

Thanks to:• The support of the GANIL staff and facility• The DEMON collaboration

This work was supported by the DOE Office of Science under the Grant No. DEFG02-88ER-40404