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M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade do Porto, Portugal, [email protected] Purely elastic instabilities in a cross Purely elastic instabilities in a cross - - slot flow slot flow A. Afonso Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade do Porto, Portugal, [email protected] F. T. Pinho Escola de Engenharia, Universidade do Minho, Portugal, [email protected] CEFT, Faculdade de Engenharia Universidade do Porto, Portugal, [email protected] The Society of Rheology 79 th annual meeting, 7 th to 11 th October 2007 Salt Lake City, USA P. J. Oliveira Departamento de Eng. Electromecânica, Universidade da Beira Interior, Covilhã, Portugal, [email protected] R. J. Poole Dept. Engineering, Mechanical Engineering, University of Liverpool Liverpool L69 3GH, UK, [email protected], [email protected]

Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

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Page 1: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

M. A. AlvesDepartamento de Engenharia Química, CEFT, Faculdade de Engenharia da

Universidade do Porto, Portugal, [email protected]

Purely elastic instabilities in a crossPurely elastic instabilities in a cross--slot flowslot flow

A. AfonsoDepartamento de Engenharia Química, CEFT, Faculdade de Engenharia da

Universidade do Porto, Portugal, [email protected]

F. T. PinhoEscola de Engenharia, Universidade do Minho, Portugal, [email protected]

CEFT, Faculdade de Engenharia Universidade do Porto, Portugal, [email protected]

The Society of Rheology 79th annual meeting, 7th to 11th October 2007Salt Lake City, USA

P. J. OliveiraDepartamento de Eng. Electromecânica, Universidade da Beira Interior,

Covilhã, Portugal, [email protected]

R. J. PooleDept. Engineering, Mechanical Engineering, University of Liverpool

Liverpool L69 3GH, UK, [email protected], [email protected]

Page 2: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Outline

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

• Motivation and previous work (UCM)

• Governing equations/numerical method

• Effect of solvent viscosity (Oldroyd-B) and inertia

• Effect of extensional viscosity (PTT)

• Conclusions

Page 3: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Motivation

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Arratia et al, Physical Review Letters 96, 144502 (2006)

Microfluidic flow in a “cross channel” geometry

650 µm

500 µm

Newtonian:

Re < 10-2

PAA Boger fluid:

Re < 10-2 (De=4.5)

Page 4: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Motivation and Previous work

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Poole, Alves and Oliveira, accepted in Physical Review Letters (2007)

Successfully used a numerical technique with a simple

viscoelastic constitutive equation (UCM) to model this steady

asymmetry under creeping-flow conditions.

Newtonian De=0.45

Page 5: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Motivation and Previous work

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Poole, Alves and Oliveira, accepted in Physical Review Letters (2007)

Successfully used a numerical technique with a simple

viscoelastic constitutive equation (UCM) to model this steady

asymmetry under creeping-flow conditions.

De = 0De = 0 .1De = 0 .2De = 0 .3De = 0 .31De = 0 .315De = 0 .32De = 0 .33De = 0 .34De = 0 .35De = 0 .36De = 0 .37De = 0 .38De = 0 .39De = 0 .40De = 0 .41De = 0 .42De = 0 .43De = 0 .44De = 0 .45

Streamlines →

Page 6: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Motivation and Previous work

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Poole, Alves and Oliveira, accepted in Physical Review Letters (2007)

Purely-elastic: inertia decreases the degree of asymmetry and

stabilizes the flow

De

DQ

0.25 0.3 0.35 0.4 0.45-1

-0.75

-0.5

-0.25

0

0.25

0.5

0.75

1

Re = 0

Re = 1

Re = 2

Re = 5

DQ = A (De - DeCR)0.5

Qq

1

q2

q1

q2 Q

Q

Q

Q

qq

qq

qqDQ 12

12

12−

=+−

=

DQ=0 → symmetric

DQ=±1 → completely asymmetric

Flow asymmetry:

Page 7: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Motivation and Previous work

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Afonso, Alves, Pinho and Oliveira, XV IWNMNNF, Rhodes (2007)

Secondary instability in which the flow becomes unsteady and

fluctuates non-periodically in time.

UCM model

De=1.0

→Re=1.0

Page 8: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Governing equations

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

( ) ( ) ( )TDf

Dtλ − ∇ − ∇ =

Au A A u A

( ) ( ) ( )TDf

D tλ − ∇ − ∇ =

Au A A u A

(Mass conservation)

(Momentum conservation)

(Constitutive equation, based on the conformation tensor, A)

•Incompressible Viscoelastic fluid

( ),

( ) ( ),

(tr )( ),

f

Y

= −− −

A I

A A I

A A I

• Examples: Upper Convected Maxwell - UCM (ββββ=0)

Oldroyd-B (0<ββββ<1)

Phan-Thien and Tanner (0<ββββ<1), with

( )( )

1 tr 3(tr )

exp tr 3Y

εε

+ −= −

AA

A

(linear)

(exponential)

s s

o s P

η ηβ

η η η≡ =

+0=⋅∇ u

g

Page 9: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Numerical method - brief description

• Finite-Volume Method

Oliveira, Pinho and Pinto (1998)

Oliveira and Pinho (1999)

• Structured, collocated and non-orthogonal meshes.

• Discretization (formally 2nd order)

• Diffusive terms: central differences (CDS)

• Advective terms, high resolution scheme: CUBISTA

Alves, Pinho and Oliveira (2003)

• Dependent variables evaluated at cell centers;

• Special formulations for cell-face velocities and stresses;

Page 10: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Computational domain, boundary conditions

Qq

1

q2

q1

q2

Q

Q

Q

20D

D

20D

20D

20D

Q=UD

De=λU/D

Inlet Boundary Conditions:

Fully-developed u(y) and ττττ(y)

Outlet Boundary Conditions:

0=∂∂ yφ

Page 11: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Effect of mesh refinement

0.01

0.02

(∆xMIN)/D

7680612 801M1

30360650 601M2

DOFNC

x/D

y/D

-1 -0.5 0 0.5 1-1

-0.5

0

0.5

1

Page 12: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Effect of mesh refinement (Oldroyd-B, ββββ=1/9, De=0.35 and Re=0)

* * * * * * * * * * * * **

**

**

**

** * *

**

**

**

**

* * * * * * * * * * * * *

* * * * * * **

**

*

*

*

*

*

**

* * * **

**

* * * **

*

*

*

*

*

**

**

* * * * * * *

x/D

u/U

Txx

-1 -0.5 0 0.5 1

-1.5

-1

-0.5

0

0.5

1

1.5

-2.5

-2

-1.5

-1

-0.5

0

0.01

0.02

(∆xMIN)/D

7680612 801M1

30360650 601M2

DOFNC

Page 13: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Oldroyd-B Results – ββββ effect

• Effect of increasing solvent viscosity (creeping flow)

De

DQ

0.3 0.4 0.5 0.6 0.7-1

-0.75

-0.5

-0.25

0

0.25

0.5

0.75

1

ββββ=0ββββ=1/9

ββββ=2/9

ββββ=3/9

Increase of critical DeCR

For ββββ>3/9 flow became asymmetricunsteady;

Page 14: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Oldroyd-B Results – ββββ effect

• Streamlines (creeping flow and ββββ=1/9)

Page 15: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Oldroyd-B Results – Inertia effect

• Effect of increasing Reynolds number (ββββ=1/9)

Increase of critical DeCR

Decrease in degree of asymmetry;

For Re>2, asymmetricunsteady flow.

De

DQ

0.3 0.4 0.5 0.6 0.7-1

-0.75

-0.5

-0.25

0

0.25

0.5

0.75

1

Re=0

Re=1

Re=2

Re=3

Re=4

DQ

0.71

0.72

Page 16: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Oldroyd-B Results – Inertia effect (streamlines)-REMOVE

•Re.vs.De map (ββββ=1/9)

De

Re

0.3 0.4 0.5 0.60

1

2

3

4

Symmetric

Steady Asymmetric

Unsteady Asymmetric

Page 17: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

De

DQ

0.5 1 1.5 2 2.5 3-1

-0.75

-0.5

-0.25

0

0.25

0.5

0.75

1

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

PTT Results

•Effect of varying ε ε ε ε parameter in PTT model (creeping flow

and ββββ=1/9)εεεε=0

εεεε=0.02εεεε=0.04 εεεε=0.06

εεεε=0.08

Increase of critical DeCR

Decrease in degree of

asymmetry (εεεε<0.04);

Increase in degree of asymmetry and in maximum De

(εεεε>0.04);

For εεεε>0.08, asymmetricstable flow disappears.

Page 18: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

PTT Results

• εεεε .vs.De stability map (Creeping flow and ββββ=1/9)

De

ε

1 2 30

0.05

0.1

Symmetric

Steady Asymmetric

Unsteady Asymmetric

Page 19: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

PTT Results

• Streamlines (creeping flow, εεεε=0.02 and ββββ=1/9)

Page 20: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Conclusions

• Increasing the solvent viscosity (increasing β) increases the critical De. For β>2/9 the first steady instability disappears and the flow becomes unsteady (but still asymmetric);

• Increasing the level of inertia (increasing Re) shifts the onset of the instability to higher De and decreases the degree of asymmetry. Essentially inertia appears to stabilize the flow.

•For the PTT model, decreasing the extensional viscosity(increasing ε) increases the critical De.

•We propose that this flow would make a good “benchmark” case for purely-elastic instabilities

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007

Page 21: Purely elastic instabilities in a cross -slot flowwebx.ubi.pt/~pjpo/SOR2007b.pdf · M. A. Alves Departamento de Engenharia Química, CEFT, Faculdade de Engenharia da Universidade

Acknowledgments

• Fundação para a Ciência e Tecnologia:

•PROJECT: BD/28288/2007

• Fundação Luso-Americana:

•PROJECT: 544/2007

• The Society of Rheology:

•Student Travel Grant

R. J. Poole, M.A. Alves, A. Afonso, F.T. Pinho and P.J. Oliveira, 79th SoR Meeting, 2007