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Text optional: Institutsname � Prof. Dr. Hans Mustermann � www.fzd.de � Mitglied der Leibniz-Gemeinschaft
Seite 3
Stand-alone
Target Chamber(s)
Helmholtz Beamline at European XFELLaser Options:
~1 Hz PW, 150J/150 fs~1 Hz PW, 30 J/30 fs~few kJ, ~ns (shock driver)
Seite 4
Helmholtz Beamline at European XFEL: Scientific Motivation
Exciting new science opportunities will be enabled by combining European XFEL with ultra-intense and high-power lasers
• Unique science with XFEL + Laser - strong field QED, e.g., vacuum birefringence
• Laser Pump + XFEL Probe- highest quality x-ray probing (imaging, spectroscopy, FR,…) of:
WDM, HEDP, high pressures, shocks, laser-plasma,damage processes, dynamics in materials, chemistry, biology
- making use of laser-generated ions, x-rays, bremsstrahlung γ’s, HHG
• XFEL Pump + Laser Probe -multi-species probing (protons, fs-electrons, γ’s, HHG …)
• Spin-offs- e.g., high-field X-ray Magnetic Circular Dichroism with small pulsed magnets- single-shot implementation of conventional synchrotron techniques
Seite 5
Workshop GOALS
• Identify the unique and high-value Scientific Opportunities enabled by the “Helmholtz Beamline at the European XFEL”
• Assess the technical requirements: - PW & kJ laser systems- XFEL beam parameters- Measurement techniques & detectors- HED endstation
• Build the Community of future Users, and establish a “User Consortium” for the program and instrument development
Seite 6
Outline
• Overview of proposed Helmholtz Beamline at European XFEL
• Sample Experiments from the HZDR Science Program
• Program Development Path
• Specific Workshop Tasks
Text optional: Institutsname � Prof. Dr. Hans Mustermann � www.fzd.de � Mitglied der Leibniz-Gemeinschaft
20112010 2012 2013 2014 2015
Zentrum HSQ
Future Directions: Center for High Power Radiation Sources (HSQ)
Text optional: Institutsname � Prof. Dr. Hans Mustermann � www.fzd.de � Mitglied der Leibniz-Gemeinschaft
ELBE SRF e-linac
(40 MeV, ps, 13 MHz)
SRF photo gun (nC)
PW DPSSL area
Ti:Sa
Dual approach:
• Ti:Sapphire PW-class laser (~30J in 30fs, now 4J in 30fs)
• Diode pumped solid state PW laser (~150J in 150 fs, few Hz)
ELBE & Petawatt Laser Developments
Petawatt, Energy-Efficient Laser for Optical Plasma Experiments
Seite 9
Proposed Helmholtz Beamlines at XFEL & FAIR
• HZDR Center for High Power Radiation Sources (2009-2014), in construction
- R&D on combining Ultra-intense High-power Lasers with Accelerators- ultrafast diagnostics, fs-synchronization, high gradient accelerators (…with DESY)
- Technology prototyping for Helmholtz Strategic Infrastructures (2015- )
• Helmholtz Beamline at European XFEL
• ~1 Hz PW + kJ/ns-beams
• Laser-pump / XFEL-probe
• up to 1013 ph/pulse, ~100 fs, coherent
� true single-shot experiments
• strong-field QED, dynamic damage, WDM, HEDP, excited-state chemistry…
• Helmholtz Beamline with High-Power Lasers at FAIR
XFEL
Beam
Seite 10
Additional research topics for Helmholtz Beamline at XFEL
effects and problems to be investigated:
- deformation of light cone, birefringence, polarization effects - nonpertubative QFT in strong laser fields - photon-photon scattering - electron-positron pair creation (in vacuum), ...
Avetissian [14]: 10 W/cmPopov [15]: 10 W/cm
2
27 2
18
e-
e+
nγ
absorptive: pair production
Strong-field Physics: High-pressure Physics:
• Vacuum birefringence:
Th. Heinzl, R. Sauerbrey, et al., Opt.
Commun. 267, 318 (2006)
� talks by G. Paulus, I. Uschmann
� Material under extreme conditions
� Need well-characterized samples
Void growth in shocked Al� later fracture
Seite 13
Stand-alone
Target Chamber(s)
Helmholtz Beamline at European XFELLaser Options:
~1 Hz PW, 150J/150 fs~1 Hz PW, 30 J/30 fs~few kJ, ~ns (shock driver)
Seite 14
XFEL beam parameters
XFEL.EU TN-2011-001
Layout of the X-Ray Systems at the European XFEL14 April 2011Th. Tschentscherfor the European XFEL project team
Seite 15
Helmholtz Beamline at European XFEL: Scientific Motivation
• Unique science enabled by combining European XFEL with ultra-intense lasers
- strong field QED, e.g., vacuum birefringence
• Highest quality x-ray probing of laser-driven experiments - isochorically heated matter (laser-ions, self- & externally-magnetized targets, interface collisional heating, laser-ablation-driven shocks)- ion induced damage in materials- time-resolved spectroscopy of excited-state chemical pathways- extreme fields & currents in ultra-intense laser-matter interaction- high pressure phenomena in laser-driven shocks- multi-view tomography, multi-frame imaging spectroscopy
• Add laser-based multi-species probing to XFEL experiments - proton radiography, fs-electron diffraction, hard bremsstrahlung,…
• Spin-offs- e.g., high-field X-ray Magnetic Circular Dichroism with small pulsed magnets- single-shot implementation of conventional synchrotron techniques
Seite 16
Outline
• Overview of proposed Helmholtz Beamline at European XFEL
• Sample Experiments from the HZDR Science Program
1. Excited-state chemistry of Actinides
2. Dynamics of ion-induced materials damage
3. Electron transport and ionization dynamics in laser-driven solids
• Program Development Path
• Specific Workshop Tasks
Seite 17
Laser+Accelerator: applications in sub-ps X-ray „pump-probe“
• Material modification by intense ion pulses (energy transfer, melting, recrystallization)• Warm-dense matter (WDM) by laser-ion isochoric heating• Extreme fields and current densities in high-energy density plasmas (HEDP)• Excited-state actinide chemistry
2) Synchronized X-ray pulse:
(HSQ: ~3x107 photons/keV, ~ps)
(XFEL: ~1012 ph/pulse, 0.1%, ~150 fs, coh.)
1) Sample modification:
Laser-ions, shock,
photochemical…
0.0
2ps
1ps
5ps
Seite 18
ICS
Photon flux for Pump-Probe:
“pink” photons per pulse per keV
(i.e., broad bandwidth)
XFEL: few 1012 (~100 fs)
LCLS: few 1010 (~200 fs)
(not implemented)
ESRF: few 1010 (~100 ps)
Inverse Compton: ~107 – 109 (~1 ps)
Broad-band sources X-ray backlighting sources
Seite 19
Excited-state chemistry
� S. Tsushima, K. Fahmy et al.
absorption
intersystem crossinginternal conversion
singlet
triplet
U
O
O175pm
175pm
U
O
O179pm
196pm
singlet
U(VI)
H
U(V)
U(VI) + U(IV)
disproportionation
• solubility depends on redox state
• redox state can be changed by excited-state chemistry (Arnold et al. Nature 451, 315, 2008)
• prospects for actinide extraction, fixation(S. Tsushima, Inorg. Chem. 48, 4846, 2009)
GOAL: Predictive understanding
of excited-state actinide chemistry
by validation of time-dependent
DFT dynamics
U-O bond length difference
� time-resolved EXAFS
Seite 20
Time-Resolved EXAFS
UO22+
*UO22+
UOOH2+
( )2/1
2
00
2
)(/)]()([)(
−=
−=
III
III
L
e
L
EEk
EEEk
m
h
µµµχ
Nnet = 485±182*
pulsed laser (400-500nm)
U: LIII 17.2 keV
X-ray
XFEL “pink”: 1011 ph in 1 keV (~5%)
Nnet = 160 (±3.3) x 103 (2% rms)
Seite 21
Dynamics of particle-induced damage
GOAL: Predictive understanding of ion-
induced damage, by experimental bench-
marking & validation of MD calculations of
full dynamics
• Fast neutron damage
• Ion implantation damage
Ion-induced damage:
• knock-ion cascade
• local melt
• refreezing
• residual defects
• also, electronic heating
(electron-phonon coupling)
� M. Posselt et al (HZDR)� A. Froideval et al (PSI)
XFEL
Beam
Seite 22
Staged approach:
• fs time-resolved ion melt (long term)
• ps time-resolved refreezing (mid term)
time-resolved surface meltRousse et al, Nature 410 65 (2001)Siders et al, Science 286, 1340 (1999)
Systematics:
ion-flux dependence
metal vs. dielectric vs. amorphous
projectile dependence (e.g., p vs. Si) time-resolved lattice expansionRose-Petruch et al,, Nature 398 310 (1999)h
� requires to distinguish ion-induced melt
from electron-induced melt
• electron heating – thermal expansion
(near term)
� talk by M. Posselt, Monday p.m.
Dynamics of particle-induced damage
Seite 23
1013 A/cm2, > 1000 T, 1013 V/m, ~keV solid density
Extreme Ex
Electron transport & strong fields in laser-driven targets
Extreme current densities, magnetized current filaments, and strong quasi-static magnetic fields in ultra-intense laser-matter interactions
Current filamentation
Quasistatic 5000 T fields in shaped targets, electron transport inhibition, enhanced heating
J. Rassuchine et al, PRE 79, 036408 (2009)
Important for:
Laser-ion accelerationIsochoric heatingFast Ignitor physicsLaser-plasma x-ray sourcesMagnetized HEDP
Seite 24
Extreme Ex5000 Tesla quasi-static field � x-ray Faraday rotation imaging
dzBnKze∫≈∆ 2λϕ
with K= 2.629×10-13 M.K.S. units.
LCLS-Matter in Extreme Conditions (HEDP) concept paper (04.2009):
“Relativistic electron transport, isochoric heating, and multi-MG magnetization in solid density plasma” T.E. Cowan, M.S. Wei et al., (HZDR, UCSD, LANL, LLNL)
Concept – image B-fields by x-ray Faraday rotation
Channel-cut Si cyrstals: I. Uschmann et al, HI-Jena
Seite 25
Channel cut Si 400 crystal
Realization – use channel-cut Bragg crystal polarimeter
I. Uschmann et al, “Determination of high purity polarization state of x-rays,” ESRF expt. (2010)
(5 x 10-10 polarization)
Seite 26
2D space-resolved x-ray absorption spectroscopy
7400 7600 7800 8000 8200
0
200
400
600
800
1000
1200
B-like
Mg-like
F-like
Be-like
Inte
nsity (
a.u
.)
Energy in 5th Order Diffraction (eV)
L-Shell (1st order),
Kß (6th order)
O-like
Self emission spectroscopy ∆t ~ 5-10 ps
Bulk electron temperature Tbulk ( x, y, t )
Space-averaged spectrum
with D. Thorn, T. Stoehlker (HI-Jena, GSI), M. Harmond, S. Toleikis (DESY)
Electron transport & ionization dynamics
Seite 27
Laser Isochoric Heating
Interface shock heating in heterogenous solid targetsSentoku et al., Phys. Plasmas 14, 122701 (2007)
Isochoric heating with laser-accelerated protonsPatel et al., Phys. Rev. Lett. 91, 125004 (2003)
Self-generated magnetic confinementRassuchine et al., PRE 79, 036408 (2009) Pulsed external ~MG magnetic transport inhibition
Bakeman et al., Megagauss XI (2007) http://conferences.theiet.org/mg-xi/mgxi-final-
v7.0.pdf
Electrostatic hot electron confinement using reduced-mass targets
Perez et al., Phys. Rev. Lett. 104, 085001 (2010)
Seite 28
Helmholtz Beamline at European XFEL: Scientific Motivation
• Unique science enabled by combining European XFEL with ultra-intense lasers
- strong field QED, e.g., vacuum birefringence
• Highest quality x-ray probing of laser-driven experiments- isochorically heated matter (laser-ions, self- & externally-magnetized targets, interface collisional heating, laser-ablation-driven shocks)- ion induced damage in materials- time-resolved spectroscopy of excited-state chemical pathways- extreme fields & currents in ultra-intense laser-matter interaction- high pressure phenomena in laser-driven shocks- multi-view tomography, multi-frame imaging spectroscopy
• New laser-based multi-species probes for XFEL experiments - proton radiography, fs-electron diffraction, hard bremsstrahlung,…
• Spin-offs- e.g., high-field X-ray Magnetic Circular Dichroism with small pulsed magnets- single-shot implementation of conventional synchrotron techniques
Seite 29
Outline
• Overview of proposed Helmholtz Beamline at European XFEL
• Sample Experiments from the HZDR Science Program
• Program Development Path
• Specific Workshop Tasks
Seite 30
Program Development Path (I)
• Broad and Strong Scientific Case- must compete with other research areas (e.g., Energy, Health) for strategic infrastructure investment in Helmholtz Association (HGF)
• Alleinstellungsmerkmal (Unique Selling Point)- complementarity to other EU projects, especially:
Helmholtz Beamline for High Intensity Lasers at FAIR, Extreme Light Infrastructure (ELI)
- relation to int’l projects: LCLS, SCSS, SwissFEL, ILE, NIF, LMJ, MaRIE
e.g., among fel peers, EuroXFEL has higher rep-rate, & high-power lasers
• Documentation- Conceptual Design & Science “white book”
� contributions beginning with this Workshop
Seite 31
Program Development Path (II)
• Communicating our plans to European XFEL, GmbH- Expression of Interest for User Consortium submitted 15.06.11
- Presentation to XFEL SAC, 29.09.11� preliminary technical requirements (laser)� identify community of users
• Next Steps:- Collaborations for developing HED Endstation
- Support opportunities for collaboratorsex. BMBF Verbundforschung (Rostock, TU-Dresden, FSU Jena, TU-Darmstadt…)
- Towards a technical design:- review of laser & x-ray requirements - identify technical challenges (e.g., synch, spectrum, seeding?) & decision points- broadening the scientific case - possible technical contributions from international partners
Seite 32
Outline
• Overview of proposed Helmholtz Beamline at European XFEL
• Sample Experiments from the HZDR Science Program
• Program Development Path
• Specific Workshop Tasks
Seite 33
Specific Workshop Tasks (I): Key Questions
• What Science are you proposing?
- Is it uniquely suited for Ultra-intense or High-power Lasers at the European XFEL?- What scientific question(s) can be pursued?- Is it a Flagship experiment? A major improvement on experiments done elsewhere? Or a unique or innovative technique?
• What are the technical requirements?
- Laser pulse energy, duration, intensity, contrast, rep-rate- Laser-generated secondary beams or radiation- Diagnostics for laser pulse & secondary beams
- X-ray photon energy, spectral width (narrow or “pink”), polarization- Per-pulse photon number; multi-views or multi-frames? - Focusing requirement- Special synchronization issues- X-ray beam diagnostics
Seite 34
• Are additional developments required?- Multi-view x-ray split & delay- “Pink beam” x-ray optics- External or self-seeding for x-ray pulse stabilization- Implementation of conventional techniques to single-shot operation- Pulsed high-fields
• Is there a defined development path?- Feasibility studies- Prototype development- Staged experiments at existing facilities (synchrotrons, FLASH, LCLS)
• What is the scientific, technical team?- Established collaborations- Theory & modeling support- Open to additional collaborators?
Specific Workshop Tasks (II): Key Questions
Seite 35
Specific Workshop Tasks (III): Scientific Case
• Workshop Presentations- talks will be posted on Workshop website (exclude proprietary info)- we can print slides for Poster Boards to stimulate discussion & exchange
- Key points will summarized by Workshop Topic Organizers
• Scientific Case documentation- Indicate your interest to contribute to the Scientific Case document
- Are you willing to assist the editorial team?
-Provide a draft “place holder” text and figure(s)
• User Consortia- Indicate your interest to contribute to HED instrument development
- Submit a Letter of Intent to Collaborate on the HGF Beamline at the European XFEL (deadline: 19 September)
Seite 36
Workshop GOALS
• Identify the unique and high-value Scientific Opportunities enabled by the “Helmholtz Beamline at the European XFEL”
• Assess the technical requirements: - PW & kJ laser systems- XFEL beam parameters- Measurement techniques & detectors- HED endstation
• Build the Community of future Users, and establish a “User Consortium” for the program and instrument development