Spoto & Grasso. Spatially resolved mass spectrometry in the study of art and archaeological objects

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  • 8/2/2019 Spoto & Grasso. Spatially resolved mass spectrometry in the study of art and archaeological objects.

    1/8

    S}kwokbb yeshbpeg dkss

    s}ecwyhdewy ol wae swug h` kyw klgkycakehbhfockb hijecwsFouse}}e S}hwh" Fouse}}e Fykssh

    S}kwokbb yeshbpeg dkss s}ecwyhdewy !DS/ os k voges}yekg wecalo{ue olcyeksolfb useg ol dkl kyeks h` yesekyca, H}eykwolf ol k

    `ksw" swykofaw`hyvkyg vk vowa dolodkb skd}be gkdkfe" DS olpeswofkwohl ckl }yhpoge s}kwokbb yeshbpeg ol`hydkwohl vowa bhv

    bodows h` gewecwohl klg k voge boleky yklfe, @hy waese yekshls" s}kwokbb yeshbpeg DS os k}}boeg ol wae swug h` kyw klg kycakeh$

    bhfockb hijecws" klg wae cuyyelw yepoev }yhpoges k suype h` yebepklw }uibockwohls, Ve aofabofaw wae dkol ck}kiobowoes klg wae

    bodowkwohls h` s}kwokbb yeshbpeg DS klg goscuss wae dhsw yebepklw k}}bockwohls, 9=;; Ebsepoey Bwg, Kbb yofaws yeseypeg,

    Nevhygs: Kycakehdewy> Kwdhs}aeyoc }yessuye DKBGO> Iyhlze> Chlseypkwohl scoelce> Fbkss> Bksey geshy}wohl(ohlozkwohl> DKBGO> Dkss

    s}ecwyhdewy> ]ofdelw> Sechlgky ohl dkss s}ecwyhdewy

    ;, Olwyhgucwohl

    Klkbwockb caedoswy }bks kl od}hywklw

    yhbe ol wae swug h` kyw klg kycakehbhfockb

    dkweyokbs" vaoca aks k pkyoew h` kods,

    Vael kywo`kcws kye swugoeg" ol kggowohl wh

    kggyessolf {ueswohls h` kuwaelwocow" hwaey

    ossues kye kbsh olpeswofkweg !e,f," waewecalhbhf useg wh }yhguce waed" waeoy

    goswyoiuwohl `yhd wae }yhgucwohl kyeks"

    klg ulgeyswklgolf wae use wh vaoca wae

    veye }uw ol wae }ksw/, I olwey}yewolf suca

    ol`hydkwohl" ow os }hssoibe wh ulgeyswklg

    iewwey wae ieakpohy h` klcoelw }eh}be,

    Bhlf$weyd swhykfe h`wel welgs wh hiscuye

    caedockb ol`hydkwohl wakw chlwyoiuwes wh

    wae kihpe$delwohleg kods, Ow os waus

    od}hywklw wh ulgeyswklg" kw wae gee}esw

    }hssoibe bepeb" kbb wae }yhcesses h` kbwey$

    kwohl wakw olweypele ol wae bo e ccbe h`

    klcoelw hijecws,

    Kl od}hywklw ossue wh ie kggyesseg

    vael pkbukibe }oeces h` kyw hy kycakeh$

    bhfockb yedkols kye caedockbb klkbzeg os

    ahv wae olwefyow h` wae hijecw os k``ecweg

    i wae klkbwockb }yhceguye kgh}weg,

    Klkbwockb wecalo{ues kye ogekbb eq}ecweg

    wh kphog kl caedockb klg }asockb kbwey$

    kwohl h` wae hijecw, @hy waese yekshls"

    klkbwockb wecalo{ues kibe wh }ey`hyd wae

    klkbsos goyecwb hl wae hijecw dkne ow

    ullecessky wh wkne skd}bes klg chde

    cbhse wh kyw cuykwhys eq}ecwkwohls, Ol wae

    }ksw" ol hygey wh lg k ikbklce iewveel kyw

    cuykwhys eq}ecwkwohls klg wae ye{uoye$

    delws h` scoelwoc dewahgs" ow vks leces$

    sky:

    !;/ wh bhckwe wae hijecw ol wae klkbzolf

    cakdieys h` wae klkbwockb olswyu$

    delw> hy" kbweylkwopeb"!9/ wh scyk}e wol `ykfdelws h` skd}bes

    `yhd ows suy`kce,

    Ul`hywulkweb" ieckuse kyw hy kycakeh$

    bhfockb hijecws akpe wh ie sdkbb wh w

    vowaol wae cakdieys h` chddhl klkbwo$

    ckb olswyudelws" wae geswyucwope k}}yhkca

    h wel yedkols wae bksw yeshyw `hy wae

    eqwykcwohl h` klkbwockb ol`hydkwohl `yhd

    kywoswoc klg(hy kycakehbhfockb skd}bes,

    K bkyfe ludiey h` lev klkbwockb

    dewahghbhfoes wakw iewwey skwos` wae

    ye{uoyedelw `hy docyh$geswyucwopeless hy

    lhl$geswyucwopeless h` wae skd}be wh ie

    klkbzeg aks ieel gepebh}eg ol yecelw

    ekys ^;T, Ol }kywocubky" ihwa dkss s}ec$

    wyhdewy !DS/ klg lhl$DS s}kwokbb ye$

    shbpeg klkbwockb wecalo{ues }yhpoge lev

    h}}hywulowoes `hy wae docyh$geswyucwope

    swug h` skd}bes h` kywoswoc hy kycakeh$

    bhfockb od}hywklce ^90T, Ol waos chlweqw"

    ed}aksos sahubg ie fopel wh wae lev

    }hssoiobowoes h``eyeg i Q$yk uhyescelce

    !QY@/$ikseg wecalo{ues wakw kbbhv wae 3G

    goswyoiuwohl h` go `eyelw ebedelws ol k

    Fouse}}e S}hwh*

    Go}kywodelwh go Scoelze

    Caodocae" Ulopeysowkm go

    Ckwklok" Pokbe Klgyek Ghyok 0"

    ?5;95" Ckwklok" Owkb

    Oswowuwh Iohswyuwwuye e

    Iohoddkfolo" CLY" Pokbe K,

    Ghyok 0" Ckwklok" Owkb

    Fouse}}e Fykssh

    Go}kywodelwh go Scoelze

    Caodocae" Ulopeysowkm go

    Ckwklok" Pokbe Klgyek Ghyok 0"

    ?5;95" Ckwklok" Owkb

    *Chyyes}hlgolf kuwahy,

    ]yeselw kggyess: Go}kywodelwh

    go Scoelze Caodocae"

    Ulopeysowkm go Ckwklok" Pokbe

    Klgyek Ghyok 0" ?5;95"

    Ckwklok" Owkb,

    Web,: .3? =?5 6315;7;>

    `kq: .3? =?5 51=;3;>

    E$dkob: fs}hwhMulocw,ow

    Wyelgs Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;;

    150 =;05$??30(' $ see `yhlw dkwwey 9=;; Ebsepoey Bwg, Kbb yofaws yeseypeg, gho:;=,;=;0(j,wykc,9=;;,=;,=;0

    mailto:[email protected]://dx.doi.org/10.1016/j.trac.2011.01.016http://dx.doi.org/10.1016/j.trac.2011.01.016mailto:[email protected]
  • 8/2/2019 Spoto & Grasso. Spatially resolved mass spectrometry in the study of art and archaeological objects.

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    skd}be wh ie olpeswofkweg vowa s}kwokb yeshbuwohl ol wae

    yklfe ;=7= bd ^6T, Suca dewahgs akpe ieel useg wh

    odkfe wae 3G swyucwuye h` aoggel }kolw bkeys, Dhyehpey"

    wae chdioleg use h` s}kwokbb yeshbpeg }hywkibe QY@

    s}ecwyhsch} klg Q$yk kishy}wohl aks kbbhveg wae

    kswhlosaolf s`udkwh wecalo{ue useg i Behlkygh Gk

    Polco ol wae Dhlk Bosk }kolwolf wh ie goscbhseg ^1T,Ahvepey" s}kwokbb yeshbpeg DS h``eys sod}be skd}be

    }ye}kykwohl klg k ck}kiobow `hy docyh$geswyucwope klkb$

    sos, Vowa dolodkb skd}be }ye}kykwohl klg gkdkfe" DS

    ckl ie useg wh olpeswofkwe iohdhbecubky" hyfkloc hy

    olhyfkloc chd}hlelws h` vhyns h` kyw hy kycakehbhfockb

    yedkols" }yhpogolf s}kwokbb yeshbpeg ol`hydkwohl ol k

    yk}og dklley, Olgeeg" wae gkwk sews chlwkol ol`hydkwohl

    hl wae goswyoiuwohl h` caedockb s}ecoes" vaoca os kl

    kgpklwkfe ol weyds h` wode ye{uoyeg chd}kyeg wh

    dewahgs wakw ye{uoye se}kykwe wkffolf hy swkololf `hy

    epey s}ecoes h` olweyesw ^?T,

    Olhyfkloc DS dewahgs kye h`wel dhye selsowope wakl

    QY@ ol gewecwolf wykce chd}hlelws" vaobe Ykdkldocyhsch} klg @huyoey wykls hyd$ol`ykyeg !@W$OY/ doc$

    yhs}ecwyhsch} chd}ewe vowa s}kwokbb yeshbpeg DS ol wae

    swug h` chd}beq hyfkloc dkwyoces vael lfey}yolw

    s}ecwyk h` wae chd}hlelws kye kpkobkibe, Wae kiobow h`

    DS wh }yhpoge ol`hydkwohl use`ub `hy wae goyecw ogelwo$

    ckwohl h` ulnlhvl chd}hulgs os chulweyikbklceg i

    wae yeguceg s}kwokb yeshbuwohl" vowa vaoca dhsw h` wae

    DS dewahgs kye kibe wh h}eykwe" chd}kyeg wh docyh$

    Ykdkl klg docyh$@W$OY s}ecwyhsch}oes,

    @hy wae yekshls huwboleg kihpe" sepeykb swugoes `hcus$

    olf hl wae k}}bockwohl h` go``eyelw s}kwokbb yeshbpeg DS

    dewahgs wh wae swug h` vhyns h` kyw klg kycakehbhfockbyedkols akpe yecelwb ieel }yhguceg" klg ve kwwed}w wh

    hyfkloze klg wh goscuss wae yesubws kcaoepeg sh `ky,

    9, S}kwokbb yeshbpeg dewahgs

    Wae s}kwokb yeshbuwohl h` kl klkbwockb wecalo{ue geles

    wae kiobow wh eqwykcw klg wh se}kykwe klkbwockb ol`hydk$

    wohl `yhd go` eyelw yefohls h` k skd}be, Dhsw h` wae s}kwokbb

    yeshbpeg klkbwockb wecalo{ues k}}boeg ol wae swug h`

    vhyns h` kyw klg kycakehbhfockb yedkols olphbpe }yhiolf

    wae skd}be i eq}hsolf ow wh k uq h` }kywocbes !}ahwhls"

    ebecwyhls" ohls" leuwykbs/ klg sodubwklehusb deksuyolf

    wae eleyf goswyoiuwohl h` k s}ecoc cbkss h` }kywocbes

    edowweg hy sckwweyeg ^;=";;T, Ekca s}kwokbb yeshbpeg

    klkbwockb wecalo{ue h}eykwes vowa k s}ecoc bkweykb yesh$

    buwohl, Dhyehpey" ge}wa yeshbuwohl os kbsh useg ol hygey wh

    cakykcweyoze wae peywockb }ey`hydklce h` suy`kce$selsowope

    klkbwockb wecalo{ues klg ow os geleg i wae goswklce

    iewveel wae 17% klg ;0% bepebs h` wae ge}wa }yhbe wae

    9y bodows h` wae Fkussokl goswyoiuwohl h` wae gewecweg soflkb

    kw wae bkeys olwey kce h` k sebecweg ebedelw hy chd}hulg

    sklgvocaeg iewveel wvh go` eyelwb chd}hseg bkeys

    ^;9T, Ol wae ckse h` bksey$ikseg wecalo{ues" wae ge}wa h`

    }elewykwohl h` wae olcogelw ykgokwohl" geleg ks wae ol$

    peyse h` wae kishy}wohl che`coelw" aks wh ie chlsogeyeg,

    Bkweykb yeshbuwohl os sodobkyb geleg `hy ihwa suy`kce$

    selsowope klg lhl$suy`kce$selsowope klkbwockb wecalo{ues

    klg ye`eys wh waeoy kiobow wh }yhpoge olge}elgelw soflkbs

    `yhd go``eyelw kyeks h` wae shbog skd}be, Wae dolodud

    goswklce h` wvh kyeks hl wae skd}be suy`kce feleykwolf ksoflkb bepeb h` ;0% klg 17% hy" ulgey dhye swyolfelw

    chlgowohls" k soflkb ykwoh h` ;=7" os useg wh {uklwo` wae

    bkweykb yeshbuwohl h` DS klkbwockb wecalo{ues ^;9T, S}k$

    wokbb yeshbpeg klkbwockb wecalo{ues dhswb h}eykwe vowa k

    w}ockb bkweykb yeshbuwohl ol wae yklfe h` docyhls ^9T, Wae

    lhpeb" use`ub ks}ecw h` s}kwokb yeshbuwohl os wh odkfe wae

    goswyoiuwohl h` ebedelws hy chd}hulgs kcyhss k skd}be

    suy`kce, Wae goyecw klkbsos h` docyhsch}oc kyeks h` k vhyn

    h` kyw dk ie kcchd}bosaeg i bkweykb yeshbuwohl" waeyei

    kbbhvolf wae eqwykcwohl h` k voge yklfe h` pkbukibe klk$

    bwockb ol`hydkwohl wakw ckl ie chyyebkweg vowa kl odkfe,

    K sdkbb bkweykb yeshbuwohl kbsh dknes }hssoibe wae klkbsos

    h` wol `ykfdelws h` skd}bes scyk}eg `yhd wae hijecw h`olweyesw vowa dolodkb gkdkfe wh wae kywo`kcw owseb`,

    Wae kiobow wh yeshbpe klkbwockb gkwk s}kwokbb os dhswb

    useg wh chbbecw ol`hydkwohl `yhd k s}ecoc yefohl h` wae

    skd}be vowaol kl kyek usukbb ol wae yklfe welwas wh

    aulgyegs h`bd9, Ol waos ckse" bhckbozeg klkbsos vowa k

    bkweykb yeshbuwohl wakw os k goyecw chlse{uelce h` wae

    kiobow wh `hcus wae olcogelw klg(hy wae edowweg iekd h`

    bofawey }kywocbes os hiwkoleg,

    3, Yhbe h` DS ol swugolf vhyns h` kyw klg

    kycakehbhfockb yedkols

    Klkbwockb wecalo{ues useg `hy wae swug h` dkweyokbs hy

    hijecws h` kywoswoc hy kycakehbhfockb od}hywklce kye eq$

    }ecweg wh }yhpoge k vekbwa h` ol`hydkwohl hl:

    !;/ wae caedockb chd}hsowohl hy lkwuye h` wae dkweyokb

    ulgey swug>

    !9/ wae swkwe h` kbweykwohl h` wae hijecws ckuseg i wae

    bhlf$weyd eq}hsuye wh wae elpoyhldelw> klg"

    !3/ wae e``ecws h` yeswhykwohl }yhceguyes,

    Kbb wae kihpe ol`hydkwohl dusw ie eqwykcweg `yhd

    skd}bes wakw kye k chd}beq doqwuye h` go``eyelw caedockb

    chd}hulgs, Klcoelw kywo`kcws veye dklu`kcwuyeg i

    dklo}ubkwolf lkwuykb }yhgucws wakw veye h`wel k doqwuye

    h` ihwa hyfkloc klg olhyfkloc chd}hulgs, Wae }yhcesses

    h` caklfe wakw olweypele ol wae bo`e ccbe h` wae kywo`kcws

    chlwyoiuwe wh olcyeksolf `uywaey waeoy caedockb chd$

    }beqow, Ol waos scelkyoh" wae fyekw }hwelwokb h` DS wh

    ogelwo caedockb s}ecoes }yeselw ol chd}beq doqwuyes

    aks ieel vogeb useg ol wae swug h` vhyns h` kyw klg

    kycakehbhfockb yedkols,

    Olhyfkloc DS aks ieel }kywocubkyb use`ub `hy caedockb

    lfey}yolwolf" ks }yhpelklce h` kycakehbhfockb dkweyokbs

    os h`wel ol`eyyeg i epkbukwolf yesubws `yhd wykce$ebedelw

    klkbsos hy `yhd {uklwowkwope geweydolkwohl h` wae yebkwope

    Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;; Wyelgs

    aww}:((vvv,ebsepoey,chd(bhckwe(wykc 156

    http://dx.doi.org/10.1016/j.trac.2011.01.016http://dx.doi.org/10.1016/j.trac.2011.01.016http://dx.doi.org/10.1016/j.trac.2011.01.016http://dx.doi.org/10.1016/j.trac.2011.01.016
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    kdhulws h` sebecweg oshwh}es ^;3T, Olhyfkloc DS aks kbsh

    ieel k}}boeg wh ogelwo` }ofdelws ol }kolws hy wae dkol

    chlswowuelws h` fbkss klg ceykdoc hijecws" elkdebs klg

    fbkzes ^;7T, Ahvepey" hyfkloc DS aks ieel vogeb useg wh

    gekb vowa k pkyoew h` go``eyelw }yhibeds chlceylolf wae

    ogelwockwohl h` hyfkloc klg iohdhbecubky chd}hulgs

    chlswowuwolf kywoswoc" aoswhyoc klg kycakehbhfockb hijecws^;5T, Wae hyfkloc ykv dkweyokbs useg ol ihwa wykgowohlkb

    kyw klg kycakehbhfockb chlweqws kye" `hy wae dhsw }kyw"

    lkwuykb }yhgucws" klg" aelce" chd}hseg h` chd}beq doq$

    wuyes h` olhyfkloc" hyfkloc klg iohdhbecubky chd}hlelws

    ^;0T, Dhyehpey" wae olwelwohlkb doqolf h` hyfkloc iolgeys

    klg }ofdelws guyolf wae }ye}kykwohl h` }kolwolf dkweyokbs

    hy ye}ekweg use h` kycakehbhfockb chhnolf pessebs wh }ye$

    }kye k yklfe h` go``eyelw `hhgswu``s kye wvh eqkd}bes h`

    audkl kcwopowoes wakw olwyhguce `uywaey chd}beqow olwh

    wae caedockb chd}hsowohl h` wae ykv dkweyokbs,

    @uywaey olcyekses ol wae chd}beqow h` chd}hsowohl

    geyope `yhd wae wykls`hydkwohl h` wae hyofolkb lkwuykb

    dkweyokbs feleykweg i wae gefykgkwohl }yhcesses hccuy$yolf wayhufa dkweyokb use klg elpoyhldelwkb eq}hsuye

    ^e,f," }yhweoc dkweyokbs useg ol wykgowohlkb wed}eyk

    }kolwolf kye suijecw wh chlgelskwohl klg cyhss$bolnolf

    yekcwohls vowa hwaey chd}hlelws !e,f," bo}ogs/T, Wae

    ul}kykbbebeg ck}kcow h` DS wh yepekb ol`hydkwohl use`ub

    `hy ogelwo`olf wae hyfkloc chd}hlelws h` kywoswoc" aoswhyoc

    klg kycakehbhfockb hijecws vowa `uywaey }hssoiobowoes `hy

    waeoy gewecwohl klg {uklwockwohl kw wykce bepebs ol chd$

    }beq dkwyoces geyopes `yhd wae kiobow wh chu}be cayh$

    dkwhfyk}aoc wecalo{ues wh dkss s}ecwyhdeweys" waeyei

    kbbhvolf se}kykwohl h` wae olgopogukb dhbecubky s}ecoes

    vowa hl$bole DS klkbsos h` wae ebuwolf chd}hlelws ^;6T,K sodobky k}}yhkca vks kgh}weg wh {uklwo` wae chd$

    }hulg$s}ecoc ckyihl !g;3C/ klg agyhfel !gG/ oshwh}e$

    ykwoh pkbues `yhd `kww$kcog yesogues goschpeyeg hl }hws$

    aeygs `yhd Nkzknaswkl klg kwwyoiuweg wh wae Elehbowaoc

    Ihwko Cubwuye !kihuw 35== ICE/ ^;1T, Wae swug }yhpogeg

    wae ekyboesw epogelce h` ahyse ghdeswockwohl ol klwo{uow,

    Ol shde ckses" kl olweygosco}bolky k}}yhkca os lec$

    essky o` go``eyelw chd}hlelws h` }yecohus skd}bes akpe

    wh ie ogelwoeg, @hy eqkd}be" ol hygey wh kssess wae

    chd}hlelws h` klcoelw chsdewocs klg wh hiwkol iewwey

    ulgeyswklgolf h` waeoy }ye}kykwohl" chd}bedelwky DS

    wecalo{ues veye eq}bhoweg !e,f," }yhbsos FC$DS klg

    hwaey klkbwockb k}}yhkcaes/ ^;?T, Ow vks waeye`hye }hs$

    soibe wh ogelwo` go``eyelw }ye}kykwohl }yhceguyes h` wvh

    Yhdkl esa$chbhyeg dkne$u}s wakw veye }yeseypeg hl

    wae suy`kce h` k Yhdkl iyhlze chsdewoc whhb klg ol k

    fbkss ulfuelwkyoud,

    Hyfkloc DS os kbsh vogeb k}}boeg `hy yeswhykwohl hy

    chlseypkwohl }uy}hses, Vael swugolf }kolw bkeys ol

    kywvhyns" wae olpeswofkwohl h` waeoy chd}beq hyfkloc$

    caedockb chd}hsowohl kods wh ogelwo ihwa hyofolkb

    chlswowuelw dkweyokbs klg wahse chd}hlelws `hydeg ks k

    chlse{uelce h` kfolf, Suca swug os h` fyekw od}hywklce

    wh sebecw wae dhsw k}}yh}yokwe chlseypkwope swykwef,

    Ol waos chlweqw" FC$DS aks ieel sahvl wh ogelwo`

    bo}ogs" vkqes" }yhweols" klg yesolhus dkweyokbs useg ol

    cyekwolf }kolweg vhyns, Ol }kywocubky" wae }hwelwokb h`$

    `eyeg i FC$DS vael chdioleg vowa }yh}ey caedockb

    }yhceguyes vks gedhlswykweg usolf =,9=,?$df skd}bes

    scyk}eg `yhd:

    !;/ wae }kolweg aubb h` k sao}vyecn gkweg wh wae bkwe;6==s(ekyb ;1==s>

    !9/ kl Owkbokl }kolwolf hl cklpks }yhguceg iewveel

    bkwe ;0==s klg ekyb ;6==s> klg"

    !3/ k }kolweg Ewyuyokl skych}akfus ^9=T,

    Caklfes ol wae caedockb chd}hsowohl h` }kolwolfs ckl

    kbsh hccuy ol duseud elpoyhldelws, Wed}eyk }kolws

    su``ey `yhd kbweykwohls dhswb olphbpolf wae pkylosa bkey

    klg wae iolgolf degoud, Cahbesweyhb$hqogkwohl }yhgucws

    !CH]s/ akpe ieel sahvl wh yesubw `yhd bofaw$kfeolf h`

    eff$iolgolf degok klg waeoy }yeselce vks }yh}hseg ks k

    dkyney h` bofaw$olguceg gefykgkwohl h` wae iolgolf

    degoud ^9;T, Goyecw$wed}eykwuye$yeshbpeg DS !GWDS/

    klkbses h` skd}bes wknel `yhd }kolweg Feydkl ikyh{uekbwkys klg `yhd wae Yeg hl Dkyhhl duykb }kolwolf swhyeg

    kw Wkwe Dhgeyl Bhlghl akpe chlydeg wae }yeselce h`

    CH]s,

    7, S}kwokbb yeshbpeg DS

    Ol wae eqkd}bes goscusseg kihpe" wae DS$ikseg klkbses

    ye{uoyeg `ykfdelws h` shbog skd}bes !w}ockbb ;;= df/

    wh ie wknel `yhd wae hijecw wh ie olpeswofkweg, Ahvepey"

    ol yecelw ekys" DS wecalo{ues wakw use s}kwokbb yeshbpeg

    ohlozkwohl shuyces akpe ieel k}}boeg `hy wae docyh$geswyucwope swug h` kywoswoc klg kycakehbhfockb hijecws,

    Sechlgky ohl !SO/ DS uses ohl iekds ol hygey wh fel$

    eykwe cakyfeg s}ecoes `yhd wae skd}be suy`kce vaobe bksey

    geshy}wohl ohlozkwohl !BGO/ klg bksey kibkwohl !BK/

    dewahgs yeb hl wae use h` }ahwhls feleykweg i bksey

    shuyces, Wae bkweykb yeshbuwohl ol waese dewahgs os od$

    }yhpeg i `hcusolf wae olchdolf }yodky iekd, Wkibe ;

    sahvs wae w}ockb bkweykb yeshbuwohl klg ge}wa h` }ele$

    wykwohl `hy wae s}kwokbb yeshbpeg wecalo{ues useg ol wae

    swug h` kyw klg kycakehbhfockb hijecws goscusseg ol waos

    yepoev vowa hwaey ol`hydkwohl yebkweg wh wae geswyucwop$

    ow h` wae dewahg klg wae Q_Z wyklsbkwohl bodow, Wae

    bkwwey ol`hydkwohl os od}hywklw ol hygey wh epkbukwe wae

    phbude h` wae 3G hijecws wakw ckl ie klkbzeg i usolf

    ekca h` wae goscusseg s}kwokbb yeshbpeg wecalo{ue,

    7,;, S}kwokbb yeshbpeg SODS

    Ohl s}uwweyolf os wae }asockb }yhcess ulgeybolf SODS

    gewecwohl, Ow yeboes hl k cksckge h` kwhdoc chbbosohls

    feleykweg vael eleyfewoc ohls aow wae suy`kce h` wae shbog

    wkyfew, Wae eleyf ge}hsoweg i wae ihdikygolf ohls os

    }kywokbb yeecweg ikcn wh wae suy`kce wayhufa wkyfew

    Wyelgs Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;;

    151 aww}:((vvv,ebsepoey,chd(bhckwe(wykc

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    kwhds dhiobozeg i wae od}kcw h` olcogelw ohls hy

    wayhufa cksckge chbbosohls, Vael wae eleyf h` wae ye$

    chobeg kwhds leky wae suy`kce os fyekwey wakl wae iolgolf

    eleyf h` wae suy`kce kwhds" waese kye ejecweg olwh wae

    pkcuud elpoyhldelw, Wae olweykcwohl phbude h` wae

    }yodky olcogelw ohls vowa wae shbog suy`kce ge}elgs

    u}hl wae eleyf h` wae }yodky ohl iekd klg wae wkyfewchd}hsowohl" iuw wae s}uwweyeg s}ecoes hyofolkwe `yhd lh

    dhye wakl wae ysw wvh kwhdoc bkeys, @hy waos yekshl"

    SODS os k pey suy`kce$selsowope klkbwockb wecalo{ue,

    SODS" ol }yolco}be" os ck}kibe h` caedockbb klkbzolf

    klg odkfolf ihwa olhyfkloc klg hyfkloc chd}hlelws

    wakw kye }yeselw kw dkjhy" dolhy hy wykce bepebs ol shbog

    skd}bes vowa k bkweykb yeshbuwohl ks sdkbb ks 5= ld ^99T,

    Sckllolf ebecwyhl docyhsch}(eleyf gos}eysope Q$yk

    uhyescelce s}ecwyhsch} !SED$EGQY@/ ^93T" }kywocbe$

    olguceg Q$yk edossohl !]OQE/ ^97T klg bksey$olguceg

    iyeknghvl s}ecwyhsch} !BOIS/ ^95T yopkb SODS ol waeoy

    s}kwokb yeshbuwohl h` olhyfkloc chd}hlelws h` vhyns h`

    kyw klg kycakehbhfockb hijecws, Ahvepey" SODS aks sof$locklwb bhvey bodows h` gewecwohl !BHGs/ !ol wae yklfe

    =,=;; ;=? kwhds(cd9/ klg k duca bhvey ge}wa

    }elewykwohl, SODS kbsh aks sdkbbey bkweykb yeshbuwohl

    chd}kyeg wh docyhBOIS !3;5 bd/ ^90T klg SODS kbbhvs

    caedockb odkfes h` wae klkbzeg suy`kce wh ie hiwkoleg

    usolf s}ecoc ohl$gewecwohl dhges,

    K goswolcwohl os dkge iewveel wae swkwoc !s/ klg g$

    lkdoc !g/ SODS h}eykwohlkb yefodes" ekca h` vaoca oebgs

    go``eyelw ol`hydkwohl klg klkbwockb `ekwuyes, Ol hygey wh

    ulgeyswklg wae iksoc go` eyelces iewveel wae wvh ye$

    fodes" ve sahubg chlsogey wakw k }yodky ohl uq h`

    ;=;5

    ohls(cd9

    (s os su`coelw wh s}uwwey dhye wakl hlekwhdoc bkey(s `yhd wae wkyfew suy`kce, O` wae }yodky

    iekd os w}ockbb `hcuseg hpey kl kyek h` wae wkyfew

    suy`kce h` kihuw ;=7;=5 bd9 klg wae kc{uosowohl wode

    os bhlfey wakl ; s" wael kl klkbsos ckyyoeg huw i usolf

    k chlwoluhus }yodky iekd }yhpoges ol`hydkwohl hl k

    suy`kce yeleveg chlwoluhusb i wae s}uwweyolf }yhcess,

    Sodobky h}eykwolf chlgowohls gele wae gSODS yefode

    wakw os use`ub `hy swugolf wae ge}wa$}yhbe chd}hsowohl

    h` wae skd}be ^96"91T, Vael wae }yodky ohl uq os

    gecyekseg wh ;=;;;=;3 ohls(cd9(s" sh wakw hlb sec$

    hlgky ohls s}uwweyeg `yhd k `ykcwohl h` kl kwhdoc bkey

    kye chbbecweg" wae swkwoc yefode os eswkibosaeg, Ulgey waos

    yefode" sSODS h}eykwes ks k suy`kce$s}ecoc klkbwockb

    wecalo{ue" solce hlb ol`hydkwohl `yhd wae huwey kwhdoc

    bkey h` wae wkyfew os hiwkoleg,

    Dkjhy gykvikcns `hy SODS klkbses h` klcoelw hijecws

    kye wae ye{uoyeg ubwyk$aofa pkcuud elpoyhldelw !;=?

    ;=;; whyy/ klg go`cubwoes vowa {uklwockwohl }yhce$

    guyes, Dhyehpey" wae olswyudelwkwohl os lhw dhiobe, @hy

    BOIS ^95"9?T" chd}kcw e{uo}delw ckl ie useg klg wae

    klkbsos ckl ie chlgucweg hl sowe !e,f," wae duseud" wae

    chlseypkwohl bkihykwhy" hy epel huwghhys kw kl eqck$

    pkwohl sowe/, Lepeywaebess" skd}be ye{uoyedelws `hy SODS

    klkbsos kye lhw }kywocubkyb swyolfelw, Kbwahufa skd}be

    soze os k soflocklw bodowkwohl" shbog skd}bes kye usukbb

    goyecwb klkbzeg vowa lh s}ecokb }yebodolky wyekwdelws,

    Skd}bes h` kihuw 9=3= dd ol gokdewey klg lh dhye

    wakl 5 dd ol aeofaw kye kbbhveg vowa wykgowohlkb SODS

    e{uo}delw" kbwahufa wae skd}be dusw whbeykwe wae SODS

    ubwyk$aofa pkcuud elpoyhldelw, Suca k ye{uoyedelw os

    }kywocubkyb cyowockb" solce geshy}wohl h` fksehus chd}h$lelws ol wae ubwyk$aofa pkcuud cakdiey ckl k``ecw wae

    olwefyow hy wae sak}e h` hyfkloc hijecws !e,f," dkluscyo}w

    `ykfdelws hy }kolwolf skd}bes/, K lkb yedkyn chlceyls

    skd}be chlgucwopow" ks chlgucwolf skd}bes kye klkbzeg

    dhye eksob, Lepeywaebess" suy`kce cakyfolf wakw hccuys

    vael lhl$chlgucwolf skd}bes kye klkbzeg ckl shde$

    wodes ie }yepelweg i usolf pey bhv }yodky$ohl ghses

    hy ebecwyhl$hhgolf }yhceguyes,

    Wae suy`kce selsowopow h` sSODS ckl ie k sepeye

    }yhibed vael gekbolf vowa vekwaeyeg hy chyyhgeg

    dkweyokbs, Caklfe }yhcesses dhgo` wae suy`kce chd}h$

    sowohl wh suca k gefyee wakw wae ol`hydkwohl hiwkoleg

    dk ie chlsogeyeg ye}yeselwkwope h` hlb wae wh} `evdhlhbkeys h` wae kbweyeg suy`kce, Ahvepey" swugoes

    kodeg kw ogelwo`olf vekwaeyolf }yhcesses ol waeoy ekyb

    swkfes dk fyekwb ielew `yhd wae use h` waos suy`kce

    wecalo{ue, Suy`kce$selsowopow bodowkwohls dk kbsh ie

    }kywb hpeychde i usolf wae ge}wa }yhbes wakw gSODS

    ckl }yhpoge,

    SODS vks ysw useg ol wae swug h` kyw klg kycakeh$

    bhfockb hijecws ol wae ;?1=s" klg k ludiey h` k}}bock$

    wohls akpe yepekbeg ows }hwelwokb klg bodowkwohls ol wae

    swug h` klcoelw dkweyokbs ^3=T, K gewkobeg gescyo}wohl h`

    suca swugoes dk ie `hulg ol yepoev kywocbes }uibosaeg ol

    wae }ksw `ev ekys ^3=39T, Wae voge ebedelwkb yklfewakw ckl ie olpeswofkweg !}hwelwokbb `yhd A wh U/" ows

    eqcebbelw BHGs klg wae {uklwowkwope ol`hydkwohl

    hiwkolkibe vael usolf SODS kye jusw shde h` wae

    kgpklwkfes h` waos wecalo{ue, Wae use h` wode$h`$ofaw

    !Wh@/ dkss klkbzeys aks od}yhpeg wae }ey`hydklce h`

    SODS ol weyds h` klkbzeg dkss yklfe" suy`kce selsowopow

    klg dkss yeshbuwohl, Chu}bolf Wh@ dkss klkbzeys od$

    }yhpeg }ey`hydklces" ks wae swkwoc chlgowohls kbbhveg i

    wae }ubseg ohl shuyce useg ol Wh@$SODS aks eq}klgeg

    wae k}}bockwohl h` SODS wh wae swug h` k pkyoew h` hy$

    fkloc" }hbdeyoc klg iohbhfockb dkweyokbs,

    Dewkbs klg kbbhs kye" ol }yolco}be" fhhg dkweyokbs `hy

    SODS klkbsos, Wae kye ebecwyockbb chlgucwope" ckl

    eksob ie aklgbeg sh ks wh hiwkol cbekl" kw klg sdhhwa

    suy`kces `hy klkbsos" klg kye kbsh usukbb chd}kwoibe

    vowa ubwyk$aofa pkcuuds, Ahvepey" kycakehbhfockb klg(

    hy kywoswoc dewkb hijecws gh lhw kbvks }hssess kbb h` waese

    }yh}eywoes gue wh gefykgkwohl }yhcesses" vaoca dk

    caedockbb dhgo` ihwa wae suy`kce klg wae olweyohy h`

    skd}bes, Lhl$chlgucwope }kwolks klg olbwykweg chd$

    }hulgs dk h`wel `hyd ks k yesubw h` bhlf iuyokb ol shob hy

    eq}hsuye wh wae kwdhs}aeye" klg waese dofaw akpe pey

    go``eyelw cakykcweyoswocs chd}kyeg wh wahse hiseypeg `hy

    }uye hy kbbheg dewkbs,

    Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;; Wyelgs

    aww}:((vvv,ebsepoey,chd(bhckwe(wykc 15?

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    Wkibe ;, Suddky h` shde yebepklw cakykcweyoswocs h` wae s}kwokbb yeshbpeg dewahgs goscusseg

    BK$OC] docyh BOIS BGO$UP DKBGO$OY DKBGO$UP K]$DKBGO

    W}ockb bkweykbyeshbuwohl

    53== bd^76T

    3;5 bd^90T

    9==5== bd ;==3== bd^5;"59T

    5=9== bd^5;T

    '7== bd^6;T

    5=;^96T

    W}ockb ge}wah` }elewykwohl

    ';== ld}ey bksey}ubse^76T

    ;==5== ld^9?T

    5=9== ldk

    ^5;T;,59,= bd^5;T

    5=9== ld^5;T

    5=9== ld^5;T

    95 ^91

    W}ockb Q_Zdhpkibe yklfei

    Q_ 4 5 cd>Z 4 9 cd

    Q_Z 4 9= cd Q_ 4 9=cdZ 4 =

    Q_ 4 9=cdZ 4 =

    Q_ 4 9=cdZ 4 =

    QZ 4 5= cd>_ 4 3= cdc

    Q_ 4Z 4 9

    H}eykwolf }yessuye 60= whyyKyfhl fks

    60= whyykoy

    ;=6;=1 whyy ;=6;=1 whyy ;=6;=1 whyy 60= whyykoy

    ;=?

    Yedhpeg dkweyokb 5=5== bf =,=;=,9 bf^95T

    K `ev wels h`bfh` dkweyokb os skd}beg`yhd wae hijecw wh ieklkbzeg^75T

    @dhb }ey }ubsebksey^5=T

    Kdhb }ey}ubse bksey^5;T

    =,33 ldhbes(dd9

    ^6;T'}f

    K}}bockwohlsh` klkbsos

    Wykce$ebedelwklg oshwh}e h`dewkbs" }hwweyklg doleykbs

    Ebedelws h`dewkbs" }hwwey"fbkss" swhle" shob"}ofdelws

    Hyfkloc klg olhyfkloc}ofdelws klg ges,

    Hyfklocchd}hlelwsklg yesogues

    Hyfklocchd}hlelwsklg yesogues

    Hyfkloc chd}hlelws:}ofdelws" ges"iolgeys" yesols

    Fbksklcodewkhiso

    k Dhsw h` wae BGO$DS eq}eyodelws veye ckyyoeg huw usolf swklgkyg DKBGO e{uo}delw, @hy waos yekshl" bkweykb klg ge}wa yeshbuwohl sodobky wh DKBGO weyd h` bkweykb yeshbuwohl veye hiwkoleg usolf s}ecockbb gesofleg bksey$docyh}yhie e{uo}delw ^5;T,

    i Wae pkbues sahvl ye`ey wh swklgkyg chddeycokb e{uo}delw,c Wae ye}hyweg pkbues ye`ey wh e{uo}delw s}ecockbb gesofleg `hy wae klkbsos h` kyw hijecws ^6;T,

    10=

    aww}:((vvv,ebsepoey,

    chd(bhckwe(wykc

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    Sepeykb dewkb hijecws h` kycakehbhfockb klg kywoswoc

    olweyesw akpe ieel swugoeg usolf SODS, Waese olcbuge

    iyhlze kywo`kcws ^33"37T" klcoelw sobpey chols ^35T" klg

    klwo{ue oyhl dusoc voyes ^30T,

    SODS aks ieel `ye{uelwb useg ol wae swug h` wae

    geweyohykwohl h` fbkss hijecws ^36T, Fbkss os chddhlb

    susce}woibe wh k pkyoew h` yekcwohls wakw k``ecw ows guyk$iobow, Klcoelw fbksses dhsw cbekyb sahv wae chlse$

    {uelces h` waeoy yebkwopeb bodoweg yesoswklce wh kwwkcn i

    vkwey" kcog klg kbnkbole k{uehus shbuwohls" swekd" hy

    kwdhs}aeyoc kfelws, Bhlf eq}hsuye wh caklfe kfelws

    vhysels wae chlse{uelces h` gefykgkwohl" vaoca os kbsh

    seel wh k``ecw dhgeyl fbksses, Fbkss vekwaeyolf s}eco$

    ckbb olphbpes kwwkcn i vkwey chdioleg vowa elpoyhl$

    delwkb klg iohbhfockb kfelws, Vkwey chyyhsohl os s}kyneg

    h`` i kl ohl$eqcaklfe decaklosd olphbpolf wae kbnkbo

    ohls ol wae fbkss klg agyhfel `yhd wae elpoyhldelw,

    SODS aks ieel useg wh swug k pkyoew h` klcoelw fbksses

    vowa wae kods h` ulgeyswklgolf wae gefykgkwohl }yhcess

    ^31T" }yhpelklce ^36T klg gkwolf ^3?T,Wae use h` ihwa s}ecwyhsch}oc klg odkfolf SODS ol wae

    swug h` }ofdelws klg iolgolf degok useg ol }kolwolfs

    akpe sahvl wae }hwelwokb h` SODS wh cakykcweyoze klg wh

    odkfe ihwa olhyfkloc klg hyfkloc s}ecoes ^7="7;T, SODS

    aks ieel useg wh odkfe }ofdelw goswyoiuwohls ol cyhss

    secwohls h` }kolw" waus chlwyoiuwolf wh wae ogelwockwohl h`

    wae go` eyelw wecalo{ues useg ol wykgowohlkb }kolwolf

    ^79"73T, Ol klhwaey swug" ow vks }hssoibe wh eqkdole

    pkyokwohls olwae chd}hsowohl h`wae wh} klg wae ihwwhd h`k

    }kolw bd" klg wae s}kwokb chyyebkwohl iewveel dewkb klg

    `kww$kcog chd}hsowohl ol dewkb$shk} kffyefkwes ^7=T,

    7,9, S}kwokbb yeshbpeg BGO$ikseg DS

    S}kwokbb yeshbpeg DS klkbsos h` kywoswoc hy kycakehbhf$

    ockb hijecws ckl kbsh ie ckyyoeg huw i geshyiolf cakyfeg

    s}ecoes `yhd wae skd}be suy`kce vowa k bksey iekd, Wae

    svowca `yhd }yodky ohls wh bksey iekds soflocklwb

    yeguces wae bkweykb yeshbuwohl" w}ockbb fholf `yhd wae

    sui$docyhl yklfe wh wae wels$h`$docyhls yklfe !Wkibe ;/,

    Ahvepey" ow os }hssoibe wh chlwyhb wae bksey$iekd gokdewey

    klg `hcus ol hygey wh od}yhpe wae s}kwokb yeshbuwohl h`

    wae klkbsos, Wae use h` `ky$UP hy OY bksey shuyces

    h}eykwolf vowa }ubse guykwohls ol wae ls yklfe aks ieel

    sahvl wh ie od}hywklw `hy wae goyecw bksey geshy}wohl h`

    cakyfeg hyfkloc s}ecoes vowa dhbecubky veofaws h` kihuw

    ;9 nGk ^77T, Dhyehpey" wae bhss h` s}kwokb yeshbuwohl

    hccuyyolf vael bksey iekds kye useg olswekg h` }yodky

    ohls os chulweyikbklceg i wae bess gedklgolf pkcuud

    ye{uoyedelws wakw wyklsbkwe olwh elaklceg }hssoiobowoes

    `hy wae goyecw klkbsos h` vhyns h` kyw klg kycakehbhfockb

    hijecws, @hy waos yekshl" BGO(DS os h`wel k}}boeg ks k

    chd}bedelwky klkbwockb whhb `hy use ol wae chlseypk$

    wohl bkihykwhy kbhlfsoge hwaey wecalo{ues ~e,f," @huyoey

    wykls`hyd ol ykyeg !@WOY/ s}ecwyhsch} klg Ykdkl

    docyhsch} ^75Tt, Kl kgpklwkfe h` BGO(DS hpey Ykdkl

    docyhsch} os wakw" ol dkl ckses" i usolf ihwa }hsowope

    klg lefkwope ohl dhges" BGO(DS }yhpoges selsowope"

    s}ecoc ogelwockwohl h` hyfkloc ssweds ikseg sod}b hl

    eqkcw dksses h` `ykfdelw ohls klg oshwh}oc }kwweyls,

    Wae bksey$geshy}wohl yefode os eswkibosaeg vael k shbog

    skd}be os oyykgokweg vowa bksey uelcoes h` =,=;; J(cd9,

    Ulgey suca chlgowohls" skd}be pk}hyozkwohl klg }kywokb

    ohlozkwohl iefols, Fyekwey bksey uelce ckuses }yh$lhulceg gechd}hsowohl h` wae oyykgokweg suy`kce, Ol

    kggowohl" wae gepebh}delw h` bkyfe swyess vkpes gue wh

    wae waeydkbb$olguceg eq}klsohl ckl yesubw ol shbog$

    dkwyoq gosolwefykwohl klg wae chbbecwope ejecwohl h` bkyfe

    dhbecubky cbusweys ^70T, Waos }aelhdelhl" nlhvl ks

    bksey kibkwohl" os eq}bhoweg i bksey kibkwohl$olgucwopeb

    chu}beg }bksdk !BK$OC]/$DS ol hygey wh }ey`hyd dubwo$

    ebedelwkb klg oshwh}oc klkbses h` shbog skd}bes, BK$OC]$

    DS os pey suowkibe `hy swugolf kyw klg kycakehbhfockb

    hijecws ieckuse ow h``eys wae eqoiobow wh kcaoepe s}kwokbb

    yeshbpeg ol`hydkwohl vowa bhv BHGs klg k voge boleky

    yklfe vowa dolodkb skd}be gkdkfe, Waos wecalo{ue os

    dkolb useg wh hiwkol dubwo$ebedelw ol`hydkwohl kwpkyohus chlcelwykwohl bepebs" fopolf ebedelwkb hy oshwh}oc

    lfey}yolws wakw chubg aeb} wh klsvey yebepklw kycake$

    hbhfockb {ueswohls" h`wel chlceylolf skd}bes suca ks

    chols klg }hwwey, Ahvepey" ks waos wh}oc aks ieel pey

    yecelwb yepoeveg ^76T" ve gh lhw goscuss ow `uywaey,

    Lhvkgks" wae }hssoiobowoes h``eyeg i goyecw BGO$DS ol

    wae swug h` lhl$phbkwobe chd}hulgs dkolwkoleg ulgey

    pkcuud kye vebb nlhvl ^71T" klg bodowkwohls ol olpeswo$

    fkwolf bkyfe dhbecubes akpe ieel eswkibosaeg, Ahvepey"

    shde bodowkwohls su` eyeg i BGO$DS veye coycudpelweg ol

    ;?16 vowa dkwyoq$kssosweg !DK/BGO$DS ^7?T, Ol DKBGO"

    wae klkbwe chd}hulgs kye edieggeg ol k suy}bus h` klhyfkloc chd}hulg !dkwyoq/ wakw os ch$geshyieg u}hl bksey

    eqcowkwohl, Waos chd}hulg os cahsel kcchygolf wh wae

    klkbwe }yh}eywoes klg wae bksey eleyf ^5=T, Wae dkwyoq

    }yhpoges k ludiey h` go``eyelw `ulcwohls" olcbugolf:

    !;/ oshbkwolf wae klkbwe dhbecubes klg }yepelwolf waeoy

    kffyefkwohl>

    !9/ kishy}wohl h` wae bksey eleyf pok ebecwyhloc hy

    poiykwohlkb eqcowkwohl !ge}elgolf hl wae bksey el$

    eyf/>

    !3/ epk}hykwohl h` ulcaklfeg klkbwe dhbecubes> klg"

    !7/ e`coelw ohlozkwohl h` klkbwe dhbecubes ^5;"59T,

    DKBGO shuyces kye usukbb chu}beg vowa Wh@ dkss

    klkbzeys ieckuse h` wae olaeyelwb }ubseg lkwuye h` wae

    sahyw wed}hykb !ls/ bksey shuyces, Wae sdkbb s}kwokb goswyo$

    iuwohl h` geshyieg ohls `uywaey `kphys wae use h` Wh@

    klkbzeys" fopolf aofa dkss yeshbuwohl !D(GD % ;="===/"

    aofa dkss kccuykc !k `ev }}d/" klg bhv BHGs ^53T,

    Ahvepey" yecelwb" sodobky }ey`hydklces akpe ieel kbsh

    hiwkoleg i usolf ohl$wyk} dkss klkbzeys ^57T" }yhpogolf

    kl eksoey kccess wh DS9 klkbses,

    7,3, DKBGO klg kwdhs}aeyoc }yessuye DKBGO

    BGO klg DKBGO eq}eyodelws kye w}ockbb chlgucweg kw

    wae bhv }yessuyes `hulg ol dhsw ohl shuyces !;=6 Whyy/,

    Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;; Wyelgs

    aww}:((vvv,ebsepoey,chd(bhckwe(wykc 10;

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    Waos elpoyhldelw os use`ub `hy ohl wykls`ey wh wae dkss

    klkbzey klg oluelces wae decaklosd i vaoca ohls

    kye `hydeg, Ahvepey" DKBGO s}ecwyk kye kbsh hiwkoleg

    kw aofaey }yessuyes" olcbugolf kwdhs}aeyoc }yessuye

    !K]/, K }yebodolky ye}hyw }uibosaeg ol 9=== ^55T

    sahveg wakw K](DKBGO }yhguceg ohl cuyyelws chd$

    }kykibe wh wakw ol ebecwyhs}yk !ESO/ i usolf k lowyhfelbksey h}eykwolf vowa k 9=$Az `ye{uelc klg kl eleyf

    gelsow h` 9065 dJ(cd9 }ey }ubse, Dhye yecelwb" K](

    DKBGO eq}eyodelws usolf OY shuyces akpe kbsh ieel

    }ey`hydeg ^50T,

    Ol wae }ksw sepeykb ekys" K](DKBGO aks ieel od}be$

    delweg vowa k ludiey h` dkss klkbzeys" olcbugolf Wh@

    ^55T" ohl wyk} ^56T" klg @huyoey$wykls`hyd ohl ccbhwyhl

    yeshlklce !@W$OCY/ ^51T" wknolf kgpklwkfe h` }bkcolf wae

    K](DKBGO ohl shuyce eqweylkbb wh wae dkss klkbzey,

    Suca k chlfuykwohl os }kywocubkyb suowkibe `hy wae

    klkbsos h` kywoswoc klg kycaehbhfockb dkweyokb" ks ow

    dknes klkbsos h` 3G hijecws eksoey ^5?T,

    K](DKBGO klkbses kye ckyyoeg huw ol k dklleysodobky wh wakw `hy chlpelwohlkb DKBGO" vowa k shbog

    dkwyoq ch$cyswkbbozeg vowa wae klkbwe, Waos ye{uoyes wae

    skd}be wh ie geswyheg hy dhgoeg, Lepeywaebess" K](

    DKBGO s}ecwyk ckl" ol shde olswklces" kbsh ie hiwkoleg

    sod}b k`wey ge}hsowolf k dkwyoq bkey hl wae skd}be

    suy`kce,

    Ohls feleykweg i K](DKBGO akpe ieel sahvl wh ie

    bess eleyfewoc wakl wahse }yhguceg i DKBGO klg kye

    waus suijecw wh soflocklwb bess dewkswkibe geck gue wh

    `ksw waeydkbozkwohl h` wae olweylkb eleyf h` wae ohl kw

    kwdhs}aeyoc chlgowohls, Ahvepey" wae yeguceg ohl

    wyklsdossohl `yhd wae kwdhs}aeye olwh wae bhv pkcuudh` wae dkss klkbzey fopes bhvey ohl cuyyelws chd}kyeg

    wh chlpelwohlkb DKBGO, Ohl$wyklsdossohl e`coelc ge$

    }elgs hl ihwa bksey$s}hw gos}bkcedelw yebkwope wh wae

    celwykb kqos h` wae dkss$klkbzey olbew ck}obbky klg wae

    phbwkfe k}}boeg iewveel wae wkyfew }bkwe klg wae olbew

    ck}obbky ^0=T, K soflocklw olcyekse ol ohl wyklsdossohl

    os hiwkoleg i kgh}wolf kl k}}yhkca ckbbeg }ubseg g$

    lkdoc `hcusolf !]G@/ wakw olphbpes svowcaolf wae ebecwyoc

    ebg wh zeyh `hy k wode olweypkb guyolf vaoca ohls k}$

    }yhkca wae ck}obbky olbew ^0;T,

    S}kwokbb yeshbpeg DS wecalo{ues ikseg hl goyecw BGO

    akpe ieel ed}bheg ol wae swug h` kyw klg kycakeh$

    bhfockb hijecws solce 9==9 ^09"03T, Ahvepey" ks gos$

    cusseg ol }yepohus secwohls" goyecw BGO os hlb e``ecwope ol

    wae swug h` k bodoweg yklfe h` dkweyokbs wakw ckl ie

    phbkwobozeg" vaobe DKBGO aks eq}klgeg BGO$ikseg DS

    dewahgs wh swugoes h` hyfkloc chd}hlelws `yhd vhyns h`

    kyw, Eqkd}bes h` wae k}}bockiobow h` DKBGO wh wae klkb$

    sos h` }ofdelws ^07T" socckwope hobs ^05T" }yhweolkcehus

    iolgeys ^0001T" klg pkylosaes ^0?T akpe ieel ye}hyweg

    ol wae boweykwuye, K }yhwehdoc k}}yhkca ikseg hl wae use

    h` DKBGO$Wh@ vks kbsh useg wh ogelwo` iohbhfockb skd$

    }bes wakw kye dhye wakl 53== ekys hbg" wknel `yhd wae

    Wyhbekl dudd" kbsh ckbbeg Ocedkl hy Hewzo ^6=T,

    Yecelwb" }hssoiobowoes h``eyeg i K](DKBGO `hy klk$

    bzolf kywoswoc dkweyokb goyecwb ol koy akpe ieel ged$

    hlswykweg i swugolf wykgowohlkb }kolwolf dkweyokbs"

    oyhl$fkbb oln ^6;T klg hyfkloc ges klg }ofdelws useg wh

    }yolw ihhns gkweg ;?;;9= ^5?T, Waos bksw swug ge$

    loweb gedhlswykweg wae k}}bockiobow h` K](DKBGO wh wae

    swug h` klcoelw hijecws" ieckuse wae klkbses veyeckyyoeg huw ol sowu vowa k s}kwokb yeshbuwohl h` kihuw

    7== bd, Waos vks kcaoepkibe i }bkcolf ihhns ol k

    dhgoeg K](DKBGO shuyce hl kl Q_Z wyklsbkwohl wkibe,

    Wae docyhgeswyucwopow h` wae klkbsos vks hiwkoleg i

    s}ykolf kihuw =,9 bf(dd9 h` wae dkwyoq !chyyes}hlg$

    olf wh kihuw =,1 ldhbe(dd9/ hl k 93$dd9 kyek h`

    wae skd}be,

    5, Chlcbusohls

    S}kwokbb yeshbpeg DS klkbwockb wecalo{ues akpe fyekw

    }hwelwokb `hy wae swug h` kyw klg kycakehbhfockb hijecws,

    Ol }kywocubky" wae wecalo{ues gescyoieg aeye akpe sepeykb

    od}hywklw cakykcweyoswocs:

    !;/ ck}kiobowoes `hy s}kwokbb yeshbpeg dubwo$ebedelwkb

    klg oshwh}oc klkbsos>

    !9/ bhv BHGs klg eqwelgeg boleky yklfes wakw kbbhv

    {uklwowkwope klkbsos>

    !3/ dolodkb skd}be }ye}kykwohl klg(hy gkdkfe> klg"

    !7/ ck}kiobowoes `hy s}kwokbb yeshbpeg klkbsos h` hyfkloc

    klg iohdhbecubky chd}hulgs,

    Ve akpe fopel s}ecokb delwohl wh yecelw olswyudelwkb

    kgpklces wakw kbbhv goyecw" s}kwokbb yeshbpeg DS klkb$

    ses h` vhyns h` kyw, Suca `kcobowoes h}el lev }hssoiobowoes`hy chd}beq kywoswoc klg kycakehbhfockb hijecws vael

    goyecw DS klkbses h` wae swugoeg hijecw kye chlgucweg kw

    K],

    Kcnlhvbegfdelws

    Ve kcnlhvbegfe su}}hyw `yhd DOUY !@OYI

    YIYL=6IDCW/, Ve vhubg bone wh wakln G, Klfbhs" G,

    Fkyhzzh klg kl klhldhus ye`eyee `hy waeoy chlswyucwope

    chddelws klg suffeswohls,

    Ye`eyelces^;T E, Coboieywh" F, S}hwh !Egowhys/" Dhgeyl Klkbwockb Dewahgs ol Kyw

    klg Kycakehbhf" Jhal Vobe & Shls Olc," Lev _hyn" USK" 9===,

    ^9T F, S}hwh" K, Whyyoso" K, Chlwolh" Caed, Shc, Yep, 9? !9===/ 79?,

    ^3T F, S}hwh" Kcc, Caed, Yes, 35 !9==9/ 059,

    ^7T ], Pklgelkieebe" A,F,D, Egvkygs" B, Dhels" Caed, Yep, ;=6

    !9==6/ 065,

    ^5T S, ]ykwo" E, Jhse}a" F, Scouwwh" Y, Dkzzeh" Kcc, Caed, Yes, 73

    !9=;=/ 6?9,

    ^0T F, Iuzkloca" ], Vhiykuscaen" C, Swyebo" K, Dkynhvocz" G,

    Vefyzlen" E, Caolek$Cklh" S, Ikd`hyg" S}ecwyhcaod, Kcwk" ]kyw

    I 09 !9==6/ ;959,

    ^6T N, Jklssels" J, Gon" D, Chwwe" J, Susolo" Kcc, Caed, Yes, 73 !9=;=/

    1;7,

    Wyelgs Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;;

    109 aww}:((vvv,ebsepoey,chd(bhckwe(wykc

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    ^1T B, ge Pofueyoe" ], Vkbwey" E, Bkpkb" I, Dhwwol" P,K, Shbem" Klfev,

    Caed," Olw, Eg, Elfb, 7? !9=;=/ 0;95,

    ^?T ], Ledes" K,S, Vhhgs" K, Peywes" Klkb, Caed, 19 !9=;=/ ?19,

    ^;=T G, Fyhbodulg" D, Sell" D, Wyhwwdkll" D, Jklhusca" O, Ihlahuye"

    K,D, Scaeogeffey" D, Dkycus" S}ecwyhcaod, Kcwk" ]kyw I 5?I

    !9==7/ ;096,

    ^;;T W, Cecakn" D, Abhzen" B, Dusoben" W, Wyhjen" Lucb" Olswyud,

    Dewahgs ]as, Yes," Secw, I 903 !9==6/ 57,

    ^;9T K,G, DcLkufaw" K, Vobnolshl !Chd}obeys/" OU]KC Chd}elgoud

    h` Caedockb Weydolhbhf" 9lg Egowohl !Fhbg Ihhn/" Ibkcnvebb

    Scoelwoc ]uibockwohls" Hq`hyg" UN" ;??6 ^QDB hl$bole chyyecweg

    peysohl ^aww}:((fhbgihhn,ou}kc,hyf !9==0$//" cyekweg i D, Loc" J,

    Joykw" I, Nhskwk" u}gkwes chd}obeg i K, Jelnols" OSIL =$

    ?06155=$?$1 !GHO:;=,;35;(fhbgihhn /T,

    ^;3T @, Pklakecne" B, Ikbckel" G, Dkbolhpsn" J, Klkb, Kw, S}ecwyhd,

    97 !9==?/ 103,

    ^;7T B, Gussuioeuq" ], Yhieywsakv" D,G, Fbkschcn" Olw, J, Dkss

    S}ecwyhd, 917 !9==?/ ;59,

    ^;5T D,], Chbhdiolo" @, Dhguflh !Egowhys/" Hyfkloc Dkss S}ecwyhdewy

    ol Kyw klg Kycakehbhf" Jhal Vobe & Shls Olc," Lev _hyn" USK"

    9==?,

    ^;0T Z, Fh``ey" Kycakehbhfockb Caedoswy" Jhal Vobe & Shls Olc," Lev

    _hyn" USK" 9==6,

    ^;6T D, Yefeyw" Dkss S}ecwyhd, Yep, 3= !9=;;/ ;66,

    ^;1T K,N, Huwykd" L,K, Sweky" Y, Ielgye" S, Hbsel" K, Nks}kyhp" P,

    Zkoieyw" L, Wahy}e" Y,], Epeysaeg" Scoelce !Vksaolfwhl" GC/ 393

    !9==?/ ;339,

    ^;?T J, ]eyez$Kyklwefuo" F, Ce}yok" E, Yoiecaolo" O, Gefklh" D,],

    Chbhdiolo" J, ]kz$]eykbwk" E, Hywoz$]kbhdky" Wyelgs Klkb, Caed,

    91 !9==?/ ;=;?,

    ^9=T K, Klgyehwwo" O, Ihlkguce" D,], Chbhdiolo" F, Fkuwoey" @,

    Dhguflh" E, Yoiecaolo" Klkb, Caed, 61 !9==0/ 77?=,

    ^9;T H,@, pkl gel Iyoln" E,S,I, @eyyeoyk" J, pkl gey Ahysw" J,J, Ihhl" Olw,

    J, Dkss S}ecwyhd, 917 !9==?/ ;9,

    ^99T G,S, Dc]akob" J, Dkwey, Sco, 7; !9==0/ 163,

    ^93T D, Vesw" K,W, Ebbos" ],J, ]hwws" C, Swyebo" C, Pklahh`" G, Vefyzlen"

    ], Vhiykuscaen" J, Klkb, Kw, S}ecwyhd, 97 !9==?/ ;91?,

    ^97T W, Ckbbofkyh" J,$C, Gykl" J, Skbhdhl" Chd}y, Klkb, Caed, 79

    !9==7/ 996,

    ^95T K, Foknhudkno" N, Debessklkno" G, Klfbhs" Klkb, Iohklkb, Caed,

    316 !9==6/ 67?,

    ^90T G, Deluw" ], @ocaew" J, Bkchuy" K, Yophkbbkl" ], Dkucaoel" K}}b,

    H}w, 79 !9==3/ 0=03,

    ^96T K, Fullkysshl" @, Nhbbdey" S, Shal" @, Ahhn" ], Sjhpkbb" Klkb,

    Caed, 19 !9=;=/ 9790,

    ^91T ], Caknykihyw" Lucb, Olswyud, Dewahgs ]as, Yes," ]kyw I 900

    !9==1/ ;151,

    ^9?T G,F, ]k}kzhfbhu" P, ]k}kgknos" G, Klfbhs" J, Klkb, Kw, S}ecwyhd,

    ;? !9==7/ 713,

    ^3=T F, S}hwh" Waeydhcaod, Kcwk 305 !9===/ ;56,

    ^3;T K, Kgyokels" D,F, Ghvseww" K}}b, Suy`, Sco, 959 !9==0/ 6=?0,

    ^39T E, Gky{ue$Ceyewwo" D, Kuchuwuyoey" ol: N, Jklssels" Y, Pkl Fyoenel

    !Egowhys/" Lhl$geswyucwope Docyhklkbsos h` Cubwuykb Aeyowkfe

    Dkweyokbs" Ebsepoey Scoelce I,P" Kdsweygkd" Wae Lewaeybklgs"

    9==7" }, 3?6,

    ^33T _, _u$Saelf" C, Ih$Julf" B, _hlf$Caoel" K}}b, Suy , Sco, 955

    !9==1/ ;537,

    ^37T F,C, Kbbel" O,W, Iyhvl" E, Coboieywh" F, S}hwh" Euy, Dkss S}ecwy, ;

    !;??5/ 7?3,

    ^35T F, Nyk w" S, @befe" @, Yeo``" A,D, Hywley" Docyhcaod, Kcwk ;75

    !9===/ 16,

    ^30T D, Fhhgvk" Scoelce !Vksaolfwhl" GC/ 930 !;?16/ ?96,

    ^36T @,J,D, Yuwwel" G, Iyoffs" J, Aelgeyshl" D,J, Yhe" Kycakehdewy 5;

    !9==?/ ?00,

    ^31T D, Debcaey" D, Scayeoley" J, Lhl$cysw, Shbogs 359 !9==0/ 301,

    ^3?T O, Boyowzos" L, Bksnkyos" Lucb, Olswyud, Dewahgs ]as, Yes," ]kyw I

    906 !9==?/ ;77,

    ^7=T N, Neule" @, Ahhfbklg" J,J, Ihhl" G, ]effoe" C, Aoffoww" Olw, J, Dkss

    S}ecwyhd, 917 !9==?/ 99,

    ^7;T Y, Akd" B, Pkecn" @, Kgkds" K, Kgyokels" Klkb, Iohklkb, Caed,

    313 !9==5/ ??;,

    ^79T Y, Pkl Akd" B, Pkl Pkecn" @, Kgkds" K, Kgyokels" Klkb, Caed,

    60 !9==7/ 90=?,

    ^73T N, Neule" J,J, Ihhl" Klkb, Caed, 60 !9==7/ ;367,

    ^77T D,K, ]hswaudus" ],F, Noswedkney" A,B,C, Deuzebkky" Klkb, Caed,

    5= !;?61/ ?15,

    ^75T G,], Noyi" L, Naklgenky" N, Suwaeybklg" I,K, ]yoce" Olw, J, Dkss

    S}ecwyhd, 917 !9==?/ ;;5,

    ^70T I,J, Fkyyoshl" Z, ]hswkvk" Dkss S}ecwyhd, Yep, 96 !9==1/

    91?,

    ^76T D, Yesklh" E, Fkycok$Yuoz" @, Pklakecne" Dkss S}ecwyhd, Yep, 9?

    !9=;=/ 55,

    ^71T K, @yegeyoc" Klkb, Iohklkb, Caed, 31? !9==6/ ;31;,

    ^7?T D, Nkyks" G, Ikcadkll" U, Ikay" @, Aobbelnkd}" Olw, J, Dkss

    S}ecwyhd, Ohl, ]yhc, 61 !;?16/ 53,

    ^5=T J, Nkd}deoey" N, Gyeoseveyg" D, Scauyelieyf" N, Swyu}kw" Olw, J,

    Dkss S}ecwyhd, ;0?(;6= !;??6/ 3;,

    ^5;T N, Gyeoseveyg" Caed, Yep, ;=3 !9==3/ 3?5,

    ^59T N, Gyeoseveyg" S, Ieynelnkd}" K, Beosley" K, Yhablf" C, Delzeb"

    Olw, J, Dkss S}ecwyhd, 990 !9==3/ ;1?,

    ^53T Y,G, Egdhlgshl" G, Yussebb" J, Kd, Shc, Dkss S}ecwyhd, 6 !;??0/

    ??5,

    ^57T N, Swyu}kw" P, Nhpwhul" A, Iuo" Y, Poley" F, Swk``hyg" S, Ahylolf" J,

    Kd, Shc, Dkss S}ecwyhd, 9= !9==?/ ;75;,

    ^55T P,P, Bkonh" D,K, Ikbgvol" K,B, Iuybolfkde" Klkb, Caed, 69

    !9===/ 059,

    ^50T P,P, Bkonh" L,O, Wkyklelnh" P,G, Ieynhuw" D,K, _knsaol" C,Y,

    ]ykskg" A,S, Bee" P,D, Ghyhsaelnh" J, Kd, Shc, Dkss S}ecwyhd, 3

    !9==9/ 357,

    ^56T F, Fykssh" E, Yozzkyebbo" F, S}hwh" J, Dkss S}ecwyhd, 79 !9==6/

    ;5?=,

    ^51T N,K, Nebbeysieyfey" ],P, Wkl" P,P, Bkonh" P,D, Ghyhsaelnh" G,

    @kiyos" Klkb, Caed, 60 !9==7/ 3?3=,

    ^5?T B, Fouykwh" K, Cklguyk" F, Fykssh" F, S}hwh" K}}b, ]as, K ?6

    !9==?/ 903,

    ^0=T P,G, Ieynhuw" S,O, Nyucanhp" P,D, Ghyhsaelnh" Yk}og Chddul,

    Dkss S}ecwyhd, 9; !9==6/ 9=70,

    ^0;T ],P, Wkl" P,P, Bkonh" P,D, Ghyhsaelnh" Klkb, Caed, 60 !9==7/

    9709,

    ^09T J,J, Ihhl" W, Bekyley" J, Klkb, K}}b, ]yhbsos 07 !9==9/ 396,

    ^03T G,D, Fyod" J, Kbboshl" Kycakehdewy 70 !9==7/ 913,

    ^07T D,S, Dkoey" S,G, ]kyeyk" K,D, Sebges" Olw, J, Dkss S}ecwyhd, 939

    !9==7/ 995,

    ^05T G,J, Pkl Gel Ieyf" L,G, Peydosw" B, Ckybbe" D, Ahbck}en" J,J,

    Ihhl" J, Se}, Sco, 91 !9==7/ ;1;,

    ^00T S, Nucnhpk" D, Cyahpk" B, Pklnhpk" K, Alozgk" Y, Alen" D,

    Nhgocen" Olw, J, Dkss S}ecwyhd, 917 !9==?/ 79,

    ^06T C, Whnkysno" E, Dkywol" C, Yhbklgh" C, Cyel$Hbope" Klkb, Caed, 61

    !9==0/ ;7?7,

    ^01T S, Nucnhpk" Y, Alen" D, Nhgocen" Klkb, Iohklkb, Caed, 311

    !9==6/ 9=;,

    ^0?T S, Zudiu ab" Y, Nlhcaelduss" S, Vu b`eyw" @, Guihos" D,J, Gkbe" Y,

    Zelhio" Klkb, Caed, 6= !;??1/ 6=6,

    ^6=T N, Ahbbedeey" V, Kbwdeey" E, Aeolzbe" C, ]owyk" Yk}og Chdd,

    Dkss S}ecwyhd, 99 !9==1/ 965;,

    ^6;T Y, GKfkwk" F, Fykssh" S, ]kybkwh" S, Sodhle" F, S}hwh" K}}b, ]as,

    K: Dkwey, Sco, ]yhcess, 1? !9==6/ ?;,

    Wyelgs ol Klkbwockb Caedoswy" Phb, 3=" Lh, 0" 9=;; Wyelgs

    aww}:((vvv,ebsepoey,chd(bhckwe(wykc 103

    http://goldbook.iupac.org/http://dx.doi.org/10.1351/goldbookhttp://dx.doi.org/10.1351/goldbookhttp://goldbook.iupac.org/