Regional studies of the optical, chemical and microphysical properties

of atmospheric aerosols

Radiative impacts and cloud formation

Admir Créso Targino Doctoral thesis

Department of Meteorology Stockholm University, 2005

Cover illustrations: Scanning Electron Microscope images of aerosol particles by A.C. Targino Regional studies of the optical, chemical and microphysical properties of atmospheric aerosols: Radiative impacts and cloud formation © Admir Créso Targino, 2005 ISBN 91-7155-141-7, pp. 1-55 Doctoral thesis Stockholm University Department of Meteorology SE-106 91 Stockholm Sweden Typesetting: Intellecta Docusys Printed in Sweden by Intellecta Docusys, Stockholm 2005 Distributor: Stockholm University Library

To my mom Cristina, my sister Andreza and

my wife Patricia. To whom I owe a lot... ==========================================

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Paper I Airborne in situ characterization of dry aerosol optical properties in a multisource influenced marine region

A.C. Targino, K.J. Noone, and E. Öström Tellus 57B, 247Ó260, 2005.

Paper II Airborne in situ characterization of dry urban aerosol

optical properties around complex topography

A.C. Targino, and K.J. Noone Atmospheric Research, 2005. In press.

Paper III Single particle analysis of ice crystal residuals observed

in orographic wave clouds over Scandinavia during INTACC experiment

A.C. Targino, R. Krejci, K.J. Noone, and P. Glantz Atmos. Chem. Phys. Discuss., 5, 1Ó36, 2005. Paper IV Microphysical and chemical characteristics of cloud

droplet residuals and interstitial particles in continental stratocumulus clouds

A.C. Targino, K.J. Noone, R. Krejci, F. Drewnick, J. Schneider, G. Olivares, S. Hings, and S. Borrmann Manuscript intended for Atmos. Chem. Phys. Discuss.

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24

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25

Surface

Unperturbed cloud Increased CDNC (constant LWC) (Twomey, 1974)

Drizzle suppression.Increased LWC

Increased cloud height(Pincus and Baker, 1994)

Increased cloud lifetime(Albrecht, 1989)

** ** ***

Indirect effecton ice cloudsand contrails

. . . . ..

..

......

..

.

.... . . .

. .

. . . .

Heating causes cloudburn-off

(Ackerman et al., 2000)

Albedo effect/1st indirect effect/ Twomey effect

Cloud lifetime effect/ 2nd indirect effect/ Albrecht effect

Semi-direct effect

Top of theatmosphere

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Profile 2 (TF22) − July 19, 1997

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