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Intersubband Intersubband Response: Response: Lineshape Lineshape , Coulomb Renormalization, , Coulomb Renormalization, and and Microcavity Microcavity Effects Effects F. T. Vasko F. T. Vasko Inst. of Semiconductor Physics Inst. of Semiconductor Physics Kiev, Kiev, Ukraine Ukraine

Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

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Page 1: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Inte

rsub

band

Inte

rsub

band

Res

pons

e:R

espo

nse:

Line

shap

eLi

nesh

ape ,

Cou

lom

b R

enor

mal

izat

ion,

, C

oulo

mb

Ren

orm

aliz

atio

n,

and

and

Mic

roca

vity

Mic

roca

vity

Effe

cts

Effe

cts

F. T

. Vas

koF.

T. V

asko

Inst

. of S

emic

ondu

ctor

Phy

sics

In

st. o

f Sem

icon

duct

or P

hysi

cs

Kie

v,K

iev,

Ukr

aine

Ukr

aine

Page 2: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

In c

olla

bora

tion

with

:A.

V. K

orov

inan

dO

.E. R

aich

ev(In

st. S

emic

ond.

Phy

s.,U

krai

ne)

A.H

erna

ndez

-Cab

rera

and

P. A

ceitu

no(U

niv.

La

Lagu

na, S

pain

)

Mot

ivat

ion:

Mid

-IR

–TH

z spe

ctra

l reg

ion

(sol

id st

ate

devi

ces f

or g

ener

atio

n,de

tect

ion,

and

mod

ulat

ion)

.Tw

o (m

ulti)

-leve

l phy

sics

(coh

eren

ce, e

.g. m

acro

-qbi

t for

med

~ 10

6el

ectr

ons)

.

Page 3: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

•QW

: lev

els,

diso

rder

, e-e

inte

ract

ion,

sp

in-fl

ip, a

nd m

icro

cavi

ty•E

-E re

norm

aliz

atio

n: d

epol

ariz

atio

n an

d ex

chan

ge•

Line

shap

e: h

omog

eneo

us a

nd

•in

hom

ogen

eous

broa

deni

ng

•Spi

n-fli

p tr

ansi

tions

•Sh

ort-r

ange

scat

teri

ng: b

eyon

d th

eBo

rn

appr

oxim

atio

n•M

icro

cavi

tyef

fect

Page 4: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Dis

orde

rQ

W le

vels

IR P

umpin

g

E

dd

GaA

sor

InA

s

AlG

aAs

orIn

GaA

s

ε 1

δd

ε

d

ε 2

l c

δd

Inho

mog

eneo

usB

road

enin

g:

n+p2 /2

mD

ispe

rsio

n la

w:

δεn=

ε n(2

δd/d

)in

-pla

ne m

otio

n

Page 5: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

EE-in

tera

ctio

nM

icro

cavi

tyef

fect

MQ

Ws

Met

als

ε 2

dM

QW

sε 1

Mom

entu

m tr

ansf

er:

( ∆q,

~d

-1)

ε 2D

iele

ctri

c w

aveg

uide

( ε1>

ε 2 )

Page 6: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Spin

spl

ittin

g

E

pσ=-1

σ=+1

Vs a

ppea

rs d

ue to

:Tr

ansv

erse

fiel

d H

eter

ojun

ctio

n po

tent

ial

Bul

k as

ymm

etry

Page 7: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Uns

cree

ned

inho

mog

enei

ties

Diff

eren

t ran

dom

pot

entia

ls +

the

sing

le P

oiss

on e

quat

ion

Non

-scr

eene

d po

tent

ial

Scre

ened

pot

enti

als:

Page 8: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Cur

rent

den

sity

:

Wig

nere

q. fo

r

pola

rizat

ion:

Ener

gy s

plitt

ing

Pertu

rbat

rion

Indu

ced

dens

ity

Excange

Basic Equations

Page 9: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

The

2D-li

mit:

qd<<

1

a Bis

the

Borh

radi

us

Cou

lom

b m

atrix

elem

ent:

Page 10: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Kin.

eq.

for p

olar

izat

ion

(inte

gral

eqs

.):

The

loca

l app

roxi

mat

ion

(

, a

lgeb

r. eq

s.):

∞→

cl

,),

()

/2()

('

2'

∑=

px

px

ssss

fL

δ,)

,(

)/2(

)(

'2

'∑

=p

xp

vx

iss

ssf

δTh

e hy

drod

ynam

ics

chai

n fo

r:

Page 11: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

1-2

Tran

sitio

ns:

2112

nn

δδ

±=

±

The

rela

tive

abso

rptio

n:

The

lines

hape

trans

form

atio

n:

Lore

ntzi

an--

Gau

ssia

n

dd

s/

~21

δε

γ∝

JETP

93,1

270

(200

1)

Phys

.Rev

. B 6

6,12

5303

(200

2)

Page 12: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Spin

-flip

tran

sitio

ns

ξ ω

ε F

ωm

in

ε

ωm

ax

ωm

axω

ωm

inp Sing

le p

arti

cle

abso

rpti

on a

t T=

0

Page 13: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Ham

ilton

ian:

Pert

urba

tion

:

In-p

lane

cur

rent

den

sity

:

Line

ariz

ed k

inet

ic E

q.:

(inte

gral

equ

ntio

n)

Dis

trib

utio

n fu

ncti

on:

VQ

is th

e C

oulo

mb

mat

rix e

lem

ent

Page 14: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

2D a

ppro

xim

atio

n:

2 x

2 m

atri

x eq

.:

Page 15: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

)sin

,(cos

φφ

φ=

nMomentum relaxation rate

Page 16: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

JETP

96,1

02 (2

003)

J. P

hys.

D 3

6,11

66(2

003)

Line

shap

e of

abs

orpt

ion

at T

=0,

InG

aAs

stru

ctur

e:

Leve

l spl

ittin

g

Ener

gy o

f tr

ansi

tions

The

rela

tive

abso

rptio

n:

Eff

ect o

f exc

hang

e:

“spr

ead”

of l

ine,

wea

k sh

ift

Page 17: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Intr

subb

and

Tran

siti

ons

in B

iase

d SL

Cur

rent

Intr

subb

and

tran

sitio

ns

In th

e B

orn

appr

oxim

atio

n

abso

rptio

n =0

Iden

tical

QW

s,Eq

uipo

pula

ted

leve

ls

?B

ut th

ere

is a

bsor

ptio

n/ga

in fo

r unb

iase

d SL

, w

ith cos

-dis

pers

ion

law

??

Page 18: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Abs

orpt

ion

Stim

ulat

ed

emis

sion

Spec

tral

func

tions

Ain

, Af

Dis

trib

utio

n fu

nctio

ns

f in, f

f

Bey

ond

the

Bor

n ap

prox

imat

ion:

α ∆ε∝

Ain

xA

f x∆f

αG

ain

∆ε

Abs

orpt

ion

Page 19: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Hig

h-fr

eque

ncy

curr

ent

& C

ompl

ex c

ondu

ctiv

ity

An

exac

t spe

ctra

l den

sity

func

tion:

Pert

urba

tion:

Line

ariz

ed K

inet

ic E

q.:

Abs

orpt

ion:

Page 20: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

α ω∝

Reσ ω,

Results:

Phys

.Rev

. B 6

9,20

5309

(200

4)

The

aver

aged

spe

ctra

l de

nsity

func

tion:

Ave

ragi

ng o

ver r

ando

m

pote

ntia

ls in

r-th

QW

s:

Page 21: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Exci

toni

cm

icro

cavi

ty (a)S

chem

atic

s of

ban

d di

agra

m o

f stru

ctur

e an

d fie

ld d

istri

butio

n; (b

)Sch

emat

ics

of

stru

ctur

e; (c

)A c

oupl

ed o

scilla

tors

; (d)

Ener

gy o

f pe

aks

as a

func

tion

of d

etun

ing

betw

een

exci

tons

and

cavi

tyH

ayge

ns, 1

665

Page 22: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Mid

-IR

mic

roca

vity

(in

ters

ubba

ndpo

lari

ton)

Ref

lect

ance

of t

he s

ampl

e as

obt

aine

d at

diff

eren

t in

cide

nce

angl

es. I

n th

e in

set:

a co

mpa

rison

be

twee

n th

e ex

perim

enta

l and

cal

cula

ted

spec

trum

at

the

reso

nanc

e an

gle

of 6

0.05

°.

?

(a)T

rans

mitt

ance

of a

3.9

µm

thic

k la

yer o

f AlA

s em

bedd

ed in

GaA

sat

an

angl

e of

inci

denc

e of

60°

; th

e ar

row

indi

cate

s th

e en

ergy

of t

he c

hose

n in

ters

ubba

ndtra

nsiti

on (1

43 m

eV).

(b)S

chem

atic

vie

w o

f the

pris

m-s

hape

d m

icro

-re

sona

to;;

thic

knes

s va

lues

are

giv

en in

nm

. (D

. Din

i, et

al.

Phys

. Rev

. Let

t. 90

, 116

401,

200

3) .

Page 23: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Res

pons

e (L

oren

tzos

cilla

tors

):

?? V

irtua

l tra

nsiti

ons

to a

noth

er le

vels

??

to c

ontin

uum

??

cont

inuu

m

Ref

lect

ance

of t

he m

icro

cavi

tysa

mpl

e fo

r diff

eren

t ang

les

of in

cide

nce

in T

M

pola

rizat

ion.

das

hed

lines

are

just

a g

uide

to th

e ey

e. In

the

left

inse

t: th

e ex

p.

poin

ts c

orre

spon

ding

to th

e en

ergy

pos

ition

of t

he d

ips

are

repo

rted

and

the

solid

line

s ar

e fit

ted

with

a s

tand

ard

dipo

le o

scilla

tor d

ispe

rsio

n. T

he ri

ght i

nset

: a

spec

trum

reco

rded

und

er T

E po

lariz

atio

n.

12ε i

Page 24: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

ε i

Kub

o fo

rmul

a +

sing

le p

artic

le a

ppro

xim

atio

n:f-m

ass

fule

(

,

)co

nst

=∆

→0

ωε0

=∆

∞→

ωε

nm nm

nm

Page 25: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Con

clus

ions

:C

oncl

usio

ns:

I. U

nscr

eene

d in

hom

ogen

eiti

esin

mul

ti-l

evel

sys

tem

due

to

the

si

ngle

Poi

sson

equ

atio

n.

II. E

E-re

norm

aliz

atio

n: d

epol

ariz

atio

n (s

elf-

cons

iste

nt f

ield

) +

non-

loca

l exc

hang

e

III.

Int

erpl

ay b

etw

een

EE-r

enor

mal

izat

ion

and

inho

mog

eneo

us

br

oade

ning

(fo

r no

n-lo

cal

resp

onse

)

IV. E

xcha

nge

effe

ct o

n sp

in-f

lip t

rans

itio

ns

V. G

ain

wit

hout

glo

bal i

nver

sion

in a

bia

sed

SL

VI.

Mic

roca

vity

pola

rito

nsp

litti

ng o

f in

ters

ubba

ndtr

ansi

tion

s

Q.:

Is

inte

rsub

band

exci

ton

poss

ible

?

Page 26: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Dou

blin

g of

inte

rsub

band

abs

orpt

ion

due

to n

on-lo

cal e

xcan

geD

QW

s

Abs

orpt

ion:

ω

BSL

DQ

Ws:

Phys

. Rev

. B 6

0,77

76 (1

999)

BSL

:Ph

ys. R

ev. B

66,

0753

06 (2

002)

New

inte

rsub

band

ex

cita

tion

(??)

Page 27: Modern Problems of Semiconductor Physicscophen04/Talks/Vasko.pdf · Intersubband Response: Lineshape, Coulomb Renormalization, and Microcavity Effects. F. T. Vasko. Inst. of Semiconductor

Intr

eban

dex

cito

n

ε F

Inte

rsu

bban

dex

cito

n??