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NH 3. C 2 H 4. CH 3 OH. IASI measurements of biomass burning and volcanic plumes. Pierre Coheur , Daniel Hurtmans, Lieven Clarisse. Cathy Clerbaux, Solène Turquety, Juliette Hadji-Lazaro,. Spectroscopie de l’Atmosphère, Chimie Quantique et Photophysique, - PowerPoint PPT Presentation
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P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
IASI measurements of biomass burning and volcanic
plumes
Spectroscopie de l’Atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles, Belgique
Service d'Aéronomie / CNRS,IPSL, Université Paris 6Paris, France
Cathy Clerbaux, Solène Turquety, Juliette Hadji-Lazaro,
Pierre Coheur, Daniel Hurtmans, Lieven Clarisse
NH3 C2H4 CH3OH
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Measurements and Products
CFCs
Short-lived species (days/weeks)and aerosols
Long-lived species (years) Climate
+ CO, O3 (months) Chemistry (C. Clerbaux tuesday)
Inter hemispheric mixing: ~1 year
hemispheric mixing: ~1-2 months
PBL mixing: ~few hours
CO2
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
MetOp
• Spectral coverage = 645-2760 cm-
1
• Spectral resolution = 0.5 cm-1
• Radiometric noise ~ <0.1-0.2 K
MetOP
IASI instrument
• 12 km pixel x 4 @ nadir • 120 spectra along the swath (±48.3° Scan 2400 km), each 50 km along the trace
IASINadir looking FTS IASI
MetOp: First European meteorological platform on polar orbit (EPS system)
Broad spectral coverage without gaps
Medium spectral resolution
Excellent radiometric performances
Small ground pixel size
Global coverage twice daily (morning and evening orbits)
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Trace species in biomass burning plumes
SO2/aerosols in volcanic plumes
IASI measuremen
ts of short-
lived species
Objectives
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Fire plumes
Countries most affected: Greece: 270 563 ha;
Italy: 153 884 ha; Albania: 127 880 ha;
Bulgaria: 67 747 ha; Spain: 55956 ha
868 252 ha burned in 14 countries (EFFIS/JRC)
Burnt areas
Fires in Southern Europe in Summer 2007
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Greece: 270 563 ha have burned during the summer,releasing large amounts of trace gases and aerosols
Aerosol measurements from space by OMI/AuraAerosol index OMI gridded 1x1 :
Credit S. Turquety (SA)
Fire plumesFires in Southern Europe in Summer 2007
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Fire plumes
Rapid transport across the Mediterranean and across North AfricaTransport pathways consistent with OMI aerosol measurements
IASI NRT CO-profile measurements from ULB/SA processing
Fires in Southern Europe in Summer 2007
2 × day
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Fire plumes
4 ppm
IASI NRT CO-profile measurements from ULB/SA processing
15 ppm 3 ppm 2 ppm
Remarkably high CO concentrations with peak at low altitude (< 2 km)Note: Peak altitude questionable due to weak sensitivity to the surface. However, consistent with Calipso aerosol profiles
Fires in Southern Europe in Summer 2007
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Fire plumes
Plume composition
Ammonia (NH3) Ethene (C2H4) and methanol (CH3OH)
Fires in Southern Europe in Summer 2007
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Fire plumesFires in Southern Europe in Summer 2007
Total column retrievals for August 25
NH3
C2H4
CH3OH
molecules cm-2
molecules cm-2
molecules cm-2
Total emitted mass:NH3 = 40 kTonsC2H4 = 6.5 kTonsCH3OH = 7 kTons
Chemistry in the fire
plume
Atmospheric budgets
Plume composition
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Fire plumesFires in Boreal regions in Spring/Summer 2008
April/May 2008: Russia worst forest fires in 30 years
MODIS fire counts (red dots) for April 18, 2008
IASI short-lived species in the fire plumeNH3
AM PM
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Trace species in biomass burning plumes
SO2/aerosols in volcanic plumes
IASI measuremen
ts of short-
lived species
Objectives
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Volcano plumes
35 36 37 38 39 40 41 42 43 44 45
13
14
15
16
17
18
19
20
-45 -40 -35 -30 -25 -20 -15 -10 -5
Inside of plume
Outside of plume
SO2-ν1 SO2-ν3
Sensitive –highly– to high altitude plumes only Use for aerial security
Sensitive to high and low altitude plumes
Jebel-at-Tair
30/09/2007 18:48
Plume composition SO2L. Clarisse, ACPD, 2008
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Volcano plumes
35 36 37 38 39 40 41 42 43 44 45
13
14
15
16
17
18
19
20
-45 -40 -35 -30 -25 -20 -15 -10 -5
Jebel-at-Tair
30/09/2007 18:48
Plume composition Aerosols
ICE
ASH SO2
Ash
AVHRR
Jebel-at-TairSept./Oct. 2007
Chaiten, ChileMay 2008
L. Clarisse, ACPD, 2008
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Volcano plumes
Etna (Sicily), July 2008Tracking SO2 plumes
GOME-2
July 10 July 12, 2008
IASI
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Volcano plumes
Etna (Sicily), July 2008Tracking SO2 plumes
± 3 hours
One day
IASI AIRS
Benefit of different platforms
July 10, 8 PM July 11, 0 AM
July 11, 9 AM July 11, 12 AM
July 11, 6 PM July 11, 9 PM
July 12, 6 AM July 12, 9 AM
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Volcano plumes
Kilauea (Hawaii), May 2008Tracking SO2 plumes from
degassing volcanoes
Use of SO2 1 to increase sensitivity to the surface (<5 km)Sensitivity down to less than 1 DU
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Conclusions
IASI Small pixel sizeGlobal Earth’s coverage twice dailyWide spectral coverageLow radiometric noise
Fires• Can best be followed on the global scale from CO profile distributions. • Reveals –for some events– signatures of a series of short-lived species including NH3 and organic species
Potential for improving some atmospheric budgetsPotential for performing in-depth chemistry studies in the fire plumes
NRT-identification and tracking of pollution
plumes
Volcanoes• Can best be tracked using SO2 signatures.
3 band provides high sensitivity to high-altitude clouds. Dedicated filter in 3 has been developed for operational monitoring (no false alerts since January 2008 while identifying all major eruptions: Etna, Chaiten, Sulawesi, Okmok, Kasatochi).
1 band provides information for degassing volcanoes (Kilauea)• Continuous spectral channels provides information on volcanic aerosols (ice and ash).
P.F. Coheur. 7th AT2, Helsinki, September 30 - October1 2008
Okmok
July 12 July 23, 2008
Kasatochi SO2 plume seen for more than a month after the eruption
July 2008 eruptions in Alaska