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A Near-Term-Deployable Salt-Cooled Advanced Nuclear Reactor Huali Wu, Francesco Carotti, Michael Young, Mohamed Abou Dbai, Raluca O. Scarlat Department of Engineering Physics, Nuclear Engineering http:// heatandmass.ep.wisc.edu / ABSTRACT KEY SYSTEM COMPONENTS THE INTEGRATED RESEARCH PROJECTS RESEARCH FOCUS I: TRITIUM TRANSPORT RESEARCH FOCUS II: FREEZING TRANSIENTS EXTERNAL LINKS PREVIOUS EXPERIENCES The Fluoride-Salt-Cooled High-Temperature Reactor (FHR) is an advanced nuclear reactor concept that combines high temperature fluoride salt coolants with solid fuel elements containing ceramic fuel micro particles and a Nuclear Air-Brayton Combined Cycle (NACC). NACC allows for base-load, power peaking with natural gas, and heat processing applications. Tritium control is important in FHR design because Tritium is created from neutron irradiation of molten salt and it will permeate through metal at FHR operation temperature. Another focus of our research regards the freezing and overcooling transients of fluoride salt, in which the coolant solidifies or becomes highly viscous as it approaches freezing around 459ºC. Adapted from (UCBTH-12-003, 2013) LARGE TRITIUM PRODUCTION Tritium is produced by neutron irradiation with Li and Be in FHR coolant, and it produces 1,000 to 10,000 times more tritium than a PWR. TO WHAT EXTENT CAN GRAPHITE FUEL BE AN EFFECTIVE AND REMOVABLE TRITIUM SINK IN THE FHR? SYSTEM TRANSPORT Tritium is produced in the core, absorbed on graphite, and may leak to air through metallic heat exchangers (Atsumi, 2011) DIFFUSION MECHANISM IN GRAPHITE Tritium diffuses through open pores and could be trapped on crystalline surfaces. INCREASED RETENTION WITH IRRADIATION Neutron irradiation will increase tritium retention in graphite. (Atsumi, 2009) Heat and Mass Transport Group UW-Madison HEATandMASS.ep.wisc.edu UC-Berkeley FHR Website FHR.nuc.berkeley.edu Energy from Thorium energyfromthorium.com Oak Ridge National Laboratory FHR Website http://www.ornl.gov/science-discovery/nuclear-science/research- areas/reactor-technology/advanced-reactor-concepts/fluoride-salt- cooled-high-temperature-reactors International Thorium Energy Organization www.itheo.org In 2011, Department of Energy (DOE) initiated a 3 year Integrated Research Project (IRP I) involving universities (University of Wisconsin-Madison, University of California-Berkeley and MIT) and National lab (ORNL) to develop the technical basis to design, develop, and license a commercially attractive FHR. The new project (IRP II), supported by DOE starting in 2015, involving more universities and resources, shows the intention to pursue the development of FHR as a safe future source of energy . NON-EQUILIBRIUM FREEZING SUPER- COOLING PHENOMENON Cooling rate, nucleation sites and purity of the salt also affects freezing phenomena HOW DOES THE FREEZING AFFECT THE FLOW IN A PIPE AND IN THE NATURAL CIRCULATION SYSTEM? FREEZING POINT Freezes at 459ºC and FHRs operate in the temperature range of 600ºC to 700ºC, and the ultimate heat sink is ambient air or water (Kelleher, 2014) EQUILIBRIUM FREEZING PHASE DIAGRAM Freezing temperature and phenomenology depends on composition (Romberger, 1972) 2 - A COMPACT HIGH- TEMPERATURE, LOW-PRESSURE CORE 3 - UNIQUE PROPERTIES OF FLUORIDE MOLTEN SALT AS A HEAT TRANSFER FLUID 4 PASSIVE SAFETY SYSTEMS RELY ON NATURAL CIRCUALTION COOLING 5- COMMERICIALLY AVAILABLE TECHNOLOGIES AND EASY TO COUPLE WITH OTHER ENERGY SOURCES Micro-particles encapsulate fuel with low failure rates up to 1600 o C. Graphite pebble fuel elements host the micro-particles, and provide accident scenario temperatures < 1000 o C. This fuel technology has been developed for gas-cooled reactors since 1960s. Heterogeneous mixed pebble-bed in an annular core design High thermal density (23 MW/m 3 ) of the core and low pressures allows the core to be smaller and cheaper. Flibe (2LiF-BeF 2 ) as a coolant of the reactor. Unique heat transfer properties. Limited corrosion and low vapor pressure. Good neutron physics behavior inside the reactor. Successfully used during Molten Salt Rector Experiment (1960s-1970s) Challenges connected to its toxicity, tritium generation, and its high freezing point (459ºC). Coolant properties enable inherent safety features of the FHR design. High operating temperatures, 600- 700ºC, allowing high thermal efficiency (42% at baseload and 65% peaking; compared to 34% conventional nuclear). Natural gas co-firing enables power peaking, opening a new part of the electricity market for nuclear plants. Natural circulation cooling systems (“DRACS”) rely on buoyancy as the driving force. A fluidic diode is used to restrict parasitic flow during normal operation of the reactor and to passively activate natural circulation upon pump failure. DRACS were demonstrated for liquid-metal cooled reactors (since 1960s), and they are more compact for salts due to more effective coolant properties. 1 - A ROBUST FUEL DESIGN 3.5 m vessel diameter (rail transportable) The Pebble Bed Fluoride-Salt Cooled, High-Temperature Reactor (PB-FHR) 236 MW th 100 MW e base-load 242 MW e peaking Molten Salt Reactor Experiment (MSRE) ORNL (1960s) - Power reactor using molten salt technology successfully operated for 5 years. Aircraft Reactor Experiment (1946-1961) High power density reactor designed to be placed inside an aircraft to power the turbines. Very High Temperature Reactors (VHTR) introduced the concept of pebble-bed core design. (ORNL/TM-2009/181,2010) (Stacy, Susan M, INL) (Stefan Kühn, Deutschland) (Kelleher, 2013) (UCBTH-14-002, 2014) (UCBTH-14-002, 2014) (UCBTH-14-002, 2014) (UCBTH-14-002, 2014) (UCBTH-14-002, 2014) April 9 th 2015

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Page 1: Huali Wu, Francesco Carotti, Michael Young, Mohamed Abou Dbai, Raluca … · A Near-Term-Deployable Salt-Cooled Advanced Nuclear Reactor Huali Wu, Francesco Carotti, Michael Young,

A Near-Term-Deployable Salt-Cooled Advanced Nuclear Reactor

Huali Wu, Francesco Carotti, Michael Young, Mohamed Abou Dbai, Raluca O. Scarlat

Department of Engineering Physics, Nuclear Engineering

http://heatandmass.ep.wisc.edu/

ABSTRACT KEY SYSTEM COMPONENTS

THE INTEGRATED RESEARCH PROJECTSRESEARCH FOCUS I:

TRITIUM TRANSPORTRESEARCH FOCUS II:

FREEZING TRANSIENTS

EXTERNAL LINKS

PREVIOUS EXPERIENCES

The Fluoride-Salt-Cooled High-Temperature

Reactor (FHR) is an advanced nuclear reactor

concept that combines high temperature

fluoride salt coolants with solid fuel elements

containing ceramic fuel micro particles and a

Nuclear Air-Brayton Combined Cycle (NACC).

NACC allows for base-load, power peaking

with natural gas, and heat processing

applications.

Tritium control is important in FHR design

because Tritium is created from neutron

irradiation of molten salt and it will permeate

through metal at FHR operation temperature.

Another focus of our research regards the

freezing and overcooling transients of fluoride

salt, in which the coolant solidifies or becomes

highly viscous as it approaches freezing

around 459ºC.

Adapted from (UCBTH-12-003, 2013)

LARGE TRITIUM PRODUCTION

Tritium is produced by neutron

irradiation with Li and Be in FHR

coolant, and it produces 1,000 to

10,000 times more tritium than a PWR.

TO WHAT EXTENT CAN GRAPHITE FUEL BE AN EFFECTIVE AND

REMOVABLE TRITIUM SINK IN THE FHR?

SYSTEM TRANSPORT

Tritium is produced in the core,

absorbed on graphite, and may leak

to air through metallic heat

exchangers

(Atsumi, 2011)

DIFFUSION MECHANISM IN GRAPHITE

Tritium diffuses through open pores

and could be trapped on crystalline

surfaces.

INCREASED RETENTION WITH IRRADIATION

Neutron irradiation will increase tritium

retention in graphite.(Atsumi, 2009)

Heat and Mass Transport Group – UW-Madison

HEATandMASS.ep.wisc.edu

UC-Berkeley FHR Website

FHR.nuc.berkeley.edu

Energy from Thorium

energyfromthorium.com

Oak Ridge National

Laboratory FHR Websitehttp://www.ornl.gov/science-discovery/nuclear-science/research-

areas/reactor-technology/advanced-reactor-concepts/fluoride-salt-

cooled-high-temperature-reactors

International Thorium Energy

Organization

www.itheo.org

In 2011, Department of Energy (DOE) initiated a 3 year Integrated

Research Project (IRP I) involving universities (University of

Wisconsin-Madison, University of California-Berkeley and MIT) and

National lab (ORNL) to develop the technical basis to design,

develop, and license a commercially attractive FHR.

The new project (IRP II), supported by DOE starting in 2015,

involving more universities and resources, shows the intention to

pursue the development of FHR as a safe future source of energy.

NON-EQUILIBRIUM FREEZING SUPER-

COOLING PHENOMENON

Cooling rate, nucleation sites and

purity of the salt also affects freezing

phenomena

HOW DOES THE FREEZING AFFECT THE FLOW IN A PIPE AND IN THE

NATURAL CIRCULATION SYSTEM?

FREEZING POINT

Freezes at 459ºC and FHRs operate in the temperature range of

600ºC to 700ºC, and the ultimate heat sink is ambient air or water

(Kelleher, 2014)

EQUILIBRIUM FREEZING PHASE

DIAGRAM

Freezing temperature and

phenomenology depends on

composition

(Romberger, 1972)

2 - A COMPACT HIGH-

TEMPERATURE, LOW-PRESSURE

CORE

3 - UNIQUE PROPERTIES OF FLUORIDE

MOLTEN SALT AS A HEAT TRANSFER FLUID 4 – PASSIVE SAFETY SYSTEMS RELY

ON NATURAL CIRCUALTION COOLING

5- COMMERICIALLY

AVAILABLE TECHNOLOGIES

AND EASY TO COUPLE WITH

OTHER ENERGY SOURCES

• Micro-particles encapsulate fuel with low

failure rates up to 1600oC.

• Graphite pebble fuel elements host the

micro-particles, and provide accident

scenario temperatures < 1000oC.

• This fuel technology has been

developed for gas-cooled reactors since

1960s.

• Heterogeneous mixed pebble-bed in

an annular core design

• High thermal density (23 MW/m3) of

the core and low pressures allows the

core to be smaller and cheaper.

• Flibe (2LiF-BeF2) as a coolant of the

reactor.

• Unique heat transfer properties.

• Limited corrosion and low vapor

pressure.

• Good neutron physics behavior inside

the reactor.

• Successfully used during Molten Salt

Rector Experiment (1960s-1970s)

• Challenges connected to its toxicity,

tritium generation, and its high freezing

point (459ºC).

• Coolant properties enable inherent

safety features of the FHR design.

• High operating temperatures, 600-

700ºC, allowing high thermal

efficiency (42% at baseload and

65% peaking; compared to 34%

conventional nuclear).

• Natural gas co-firing enables

power peaking, opening a new

part of the electricity market for

nuclear plants.

• Natural circulation cooling systems (“DRACS”) rely

on buoyancy as the driving force.

• A fluidic diode is used to restrict parasitic flow during

normal operation of the reactor and to passively

activate natural circulation upon pump failure.

• DRACS were demonstrated for liquid-metal cooled

reactors (since 1960s), and they are more compact

for salts due to more effective coolant properties.

1 - A ROBUST FUEL DESIGN

3.5 m vessel diameter (rail transportable)

The Pebble Bed Fluoride-Salt Cooled, High-Temperature Reactor (PB-FHR)

236 MWth

100 MWe base-load

242 MWe peaking

Molten Salt Reactor

Experiment (MSRE)

ORNL (1960s) - Power

reactor using molten salt

technology successfully

operated for 5 years.

Aircraft Reactor Experiment

(1946-1961) – High power

density reactor designed to

be placed inside an aircraft

to power the turbines.

Very High Temperature

Reactors (VHTR)

introduced the concept

of pebble-bed core

design.

(ORNL/TM-2009/181,2010)

(Stacy, Susan M, INL)

(Stefan Kühn, Deutschland)

(Kelleher, 2013)

(UCBTH-14-002, 2014)

(UCBTH-14-002, 2014)

(UCBTH-14-002, 2014)

(UCBTH-14-002, 2014)

(UCBTH-14-002, 2014)

April 9th 2015