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Environmental Research Letters ACCEPTED MANUSCRIPT • OPEN ACCESS Quantifying process-level uncertainty contributions to TCRE and Carbon Budgets for meeting Paris Agreement climate targets To cite this article before publication: Chris D Jones et al 2020 Environ. Res. Lett. in press https://doi.org/10.1088/1748-9326/ab858a Manuscript version: Accepted Manuscript Accepted Manuscript is “the version of the article accepted for publication including all changes made as a result of the peer review process, and which may also include the addition to the article by IOP Publishing of a header, an article ID, a cover sheet and/or an ‘Accepted Manuscript’ watermark, but excluding any other editing, typesetting or other changes made by IOP Publishing and/or its licensors” This Accepted Manuscript is © 2020 The Author(s). Published by IOP Publishing Ltd.. As the Version of Record of this article is going to be / has been published on a gold open access basis under a CC BY 3.0 licence, this Accepted Manuscript is available for reuse under a CC BY 3.0 licence immediately. Everyone is permitted to use all or part of the original content in this article, provided that they adhere to all the terms of the licence https://creativecommons.org/licences/by/3.0 Although reasonable endeavours have been taken to obtain all necessary permissions from third parties to include their copyrighted content within this article, their full citation and copyright line may not be present in this Accepted Manuscript version. Before using any content from this article, please refer to the Version of Record on IOPscience once published for full citation and copyright details, as permissions may be required. All third party content is fully copyright protected and is not published on a gold open access basis under a CC BY licence, unless that is specifically stated in the figure caption in the Version of Record. View the article online for updates and enhancements. This content was downloaded from IP address 171.5.225.56 on 09/04/2020 at 16:06

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Environmental Research Letters

ACCEPTED MANUSCRIPT • OPEN ACCESS

Quantifying process-level uncertainty contributions to TCRE and CarbonBudgets for meeting Paris Agreement climate targetsTo cite this article before publication: Chris D Jones et al 2020 Environ. Res. Lett. in press https://doi.org/10.1088/1748-9326/ab858a

Manuscript version: Accepted Manuscript

Accepted Manuscript is “the version of the article accepted for publication including all changes made as a result of the peer review process,and which may also include the addition to the article by IOP Publishing of a header, an article ID, a cover sheet and/or an ‘AcceptedManuscript’ watermark, but excluding any other editing, typesetting or other changes made by IOP Publishing and/or its licensors”

This Accepted Manuscript is © 2020 The Author(s). Published by IOP Publishing Ltd..

 

As the Version of Record of this article is going to be / has been published on a gold open access basis under a CC BY 3.0 licence, this AcceptedManuscript is available for reuse under a CC BY 3.0 licence immediately.

Everyone is permitted to use all or part of the original content in this article, provided that they adhere to all the terms of the licencehttps://creativecommons.org/licences/by/3.0

Although reasonable endeavours have been taken to obtain all necessary permissions from third parties to include their copyrighted contentwithin this article, their full citation and copyright line may not be present in this Accepted Manuscript version. Before using any content from thisarticle, please refer to the Version of Record on IOPscience once published for full citation and copyright details, as permissions may be required.All third party content is fully copyright protected and is not published on a gold open access basis under a CC BY licence, unless that isspecifically stated in the figure caption in the Version of Record.

View the article online for updates and enhancements.

This content was downloaded from IP address 171.5.225.56 on 09/04/2020 at 16:06

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Quantifying process-level uncertainty

contributions to TCRE and Carbon Budgets for

meeting Paris Agreement climate targets

Chris D. Jones1, Pierre Friedlingstein2,3

1 Met Office Hadley Centre, Exeter, EX1 3PB, UK 2 College of Engineering, Mathematics and Physical Sciences, University of Exeter, Exeter, EX4 4QF,

UK 3 Laboratoire de Meteorologie Dynamique, Institut Pierre-Simon Laplace, CNRS-ENS-UPMC-X, Paris,

France

E-mail: [email protected]

Received xxxxxx

Accepted for publication xxxxxx

Published xxxxxx

Abstract

To achieve the goals of the Paris Agreement requires deep and rapid reductions in

anthropogenic CO2 emissions, but uncertainty surrounds the magnitude and depth of

reductions. Earth system models provide a means to quantify the link from emissions to

global climate change. Using the concept of TCRE – the transient climate response to

cumulative carbon emissions – we can estimate the remaining carbon budget to achieve 1.5 or

2oC. But the uncertainty is large, and this hinders the usefulness of the concept. Uncertainty

in carbon budgets associated with a given global temperature rise is determined by the

physical Earth system, and therefore Earth system modelling has a clear and high priority

remit to address and reduce this uncertainty. Here we explore multi-model carbon cycle

simulations across three generations of Earth system models to quantitatively assess the

sources of uncertainty which propagate through to TCRE.

Our analysis brings new insights which will allow us to determine how we can better direct

our research priorities in order to reduce this uncertainty. We emphasise that uses of carbon

budget estimates must bear in mind the uncertainty stemming from the biogeophysical Earth

system, and we recommend specific areas where the carbon cycle research community needs

to re-focus activity in order to try to reduce this uncertainty. We conclude that we should

revise focus from the climate feedback on the carbon cycle to place more emphasis on CO2 as

the main driver of carbon sinks and their long-term behaviour. Our proposed framework will

enable multiple constraints on components of the carbon cycle to propagate to constraints on

remaining carbon budgets.

Keywords: Carbon budgets, carbon cycle feedbacks, constraints, research priorities

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1. Introduction

Perhaps the most common question required for mitigation policy is “by how much do we need to reduce our

carbon emissions?”. It is well accepted that deep and rapid emissions cuts are required in order to achieve the

UN’s Framework Convention on Climate Change goal of avoiding dangerous climate change, but in order to

develop quantitative and measurable policy targets we must quantify the emissions compatible with any climate

goal. Since the global community has adopted the Paris Agreement, which entered into force in November 2016,

the requirement to quantify carbon budgets for low climate targets has grown.

The Transient Climate Response to cumulative carbon Emissions

A body of literature from 2009 found consistently that warming was much more closely related to the

cumulative CO2 emissions than the time profile or particular pathway (Allen et al., 2009; Matthews et al., 2009;

Meinshausen et al., 2009). This relationship between warming and cumulative emissions was one of the new and

innovative outcomes of the IPCC’s Fifth Assessment Report (AR5) report (IPCC, 2013). AR5’s Figure SPM.10

showed this relationship – known as TCRE: the Transient Climate Response to cumulative carbon Emissions.

The physical basis of TCRE was first hinted at by Caldeira & Kasting (1993) who noted that saturation of the

radiative effect of CO2 in the atmosphere could be balanced by saturation of uptake by ocean carbon leading to

insensitivity of the warming to the pathway of CO2 emissions. Literature since then has put this on a firm footing

with numerous authors showing that trajectories of ocean heat and carbon uptake have similar effects on global

temperature due to the diminishing radiative forcing from CO2 in the atmosphere and the diminishing efficiency

of ocean heat uptake (Ehlert, et al., 2017; Goodwin et al, 2015; MacDougall, 2016). Although as noted by

MacDougall (2017) that terrestrial carbon uptake is equally important for the magnitude of TCRE – in fact we

will show here that land and ocean contribute equally to the magnitude of TCRE and that land dominates over the

ocean in terms of model spread.

Application of TCRE to quantify carbon budgets

IPCC AR5 assessed a total carbon budget of 790 PgC to likely (66% chance) remain below 2oC above pre-

industrial, of which about 630 PgC has been emitted over the 1870-2018 period (Friedlingstein et al., 2019).

However, the spread of models means that the uncertainty in the remaining carbon budget to achieve 1.5 or 2oC

is very large – in fact possibly larger than the remaining budget itself. This large uncertainty hinders the potential

usefulness of this simplifying concept to policy makers. All studies and reports which present estimates of the

remaining carbon budget (e.g. The IPCC’s Fifth Assessment Report, its Special Report on Global Warming of

1.5oC, or the UNEP Gap Report) have to make an assumption on how to deal with and present this uncertainty.

Some explicitly describe the chosen assumptions (such as 50% or 66% probability of meeting targets) or tabulate

multiple options, but all are hindered in some way by the precision with which carbon budgets are known.

The AR5 Synthesis Report quoted a value of 400 GtCO2 (110 GtC) remaining budget from 2011 for a 66%

chance to keep warming below 1.5oC. It is now clear that this was an underestimate as this would mean a

remaining budget of about 20 GtC from 2020. Since AR5 there has been extensive literature on the application of

the TCRE concept and its limitations including the choice of temperature metric and baseline period and issues

of biases in Earth system models (ESMs). Some studies accounted for climate model biases by relating warming

from present day onwards to the remaining carbon budget (e.g. Millar et al., 2017; Tokarska & Gillett, 2018).

Other studies have used the historical record to constrain TCRE and the remaining budget using simple models

(Goodwin et al., 2018) or attribution techniques (Millar & Friedlingstein, 2018). Both these approaches find a

substantial increase in the remaining carbon budget for 1.5oC compared to the IPCC AR5 SPM approach. Further

studies have tried to additionally account for non-CO2 warming. Matthews et al. (2017) show CO2-only TCRE

budgets are a robust upper limit but taking account of non-CO2 forcing results in lower allowable emissions. Smith

et al. (2012) and Allen et al. (2018) have proposed techniques for combining emissions rates of short-lived climate

pollutants with long-term CO2 cumulative emission budgets. In light of these advances, the IPCC Special Report

on Global Warming of 1.5oC (SR15, Rogelj et al., 2018) quotes a value of 420 GtCO2 remaining carbon budget

for a 66% chance to keep warming below 1.5oC – a value very similar to the AR5 value from 5 years earlier.

There is also a lot of focus on how to achieve such carbon budgets and the increasing realisation of the need

for carbon dioxide removal and research into the feasibility and implications of negative emissions technology.

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The discussion around carbon dioxide removal (CDR) requires more detailed assessment of the magnitude and

timing of any requirement for negative emissions technology and hence more precise estimates of remaining

carbon budgets (Fuss et al., 2016). While Peters (2018) argues that large uncertainty in budget estimates may be

used to “justify further political inaction”, Sutton (2018) argues for careful consideration of the full range of

climate projections, including “physical plausible high impact” outcomes in the tails of the likelihood distribution.

The same argument applies to TCRE and carbon budgets: we need information on best estimates but also possible

extremes however unlikely. For example, Kriegler et al. (2018) show that the feasibility of achieving 1.5 oC

without net negative emissions depends on the remaining budget being at the high end of current estimates.

Knowing the likelihood of the range as well as central estimate is required to inform the debate on requirements

for negative emissions.

SR15 and Rogelj et al. (2019) present a framework to breakdown individual contributions to uncertainty in

carbon budgets. They separately assess: (i) the historical human induced warming to date; (ii) the likely range of

TCRE, (iii) the potential additional warming after emissions reached zero (zero-emissions commitment, ZEC);

(iv) the warming from non-CO2 forcing agents (such as other greenhouse gases and aerosols); (v) carbon emissions

from Earth system feedbacks not yet represented in ESMs (such as carbon release from thawing of permafrost).

While there are multiple ways of decomposing this issue, an unavoidable conclusion is that our imperfect ability

to model the climate-carbon cycle system plays a dominant role in uncertainty surrounding assessment of the

remaining carbon budget.

Of the five components described above, 3 are directly linked to coupled climate-carbon cycle modelling:

TCRE, ZEC and missing feedbacks. These are being addressed. For example, a new initiative – ZECMIP (Jones

et al., 2019) - was launched to address uncertainty in the zero-emission commitment and initial results

(MacDougall et al., 2019) suggest that SR15 assumptions of no significant further warming after CO2 emissions

cease is consistent with the multi-model mean. Similarly, CMIP6 and ever increasingly sophisticated ESMs (e.g.

Sellar et al., 2019; Seferian et al., 2019) begin to include additional Earth system feedbacks into models – e.g.

coupled terrestrial nitrogen cycle is now expected in approximately half of CMIP6 ESMs and some also begin to

include permafrost carbon (Arora et al., 2019). However, the elephant in the room is that past generations of

models has not seen a decreased spread in TCRE (Friedlingstein et al., 2006; Arora et al., 2013; Arora et al., 2019)

and rarely does adding complexity reduce this. Much longer experience on assessment of the climate sensitivity

to increasing CO2 (ECS, equilibrium climate sensitivity; Flato et al., 2013) suggests little GCM convergence with

a persistent large range of about 3°C (from about 1.5 to about 4.5 °C) since the Charney report (1979).

It is therefore required to understand at a process level where the uncertainty in TCRE comes from in order to

target observational constraints and prioritise model development and associated evaluation.

Here we perform a new analysis of three generations of Earth System Model results, spanning over a decade,

to examine whether or not existing simulations and analyses are well placed to answer the increasing requirements

of policy makers on the carbon cycle research community. In section 2 we present a new analytical framework

which allows us to quantify sources of uncertainty in carbon budgets to land or ocean response to CO2 or climate.

Analysis of results in section 3 shows that it is the carbon cycle response to CO2, rather than its response to

climate, which dominates the uncertainty in TCRE and hence carbon budgets. We conclude with

recommendations for the carbon cycle research community.

2. Framework for uncertainty propagation

At a very broad level the global carbon cycle can be characterised by two strong and opposing responses: how

it responds to rising CO2 concentration and how it responds to a changing climate. Firstly, as atmospheric CO2

increases, natural carbon reservoirs act to take up carbon from the atmosphere, inducing carbon sinks. Secondly,

as the world warms, this climate change also affects these carbon sinks, for example through changes in vegetation

growth or ocean stratification. This paradigm has become a widely-used framework for carbon cycle analyses

with the former (carbon cycle response to CO2) often referred to as “concentration-carbon feedback” and denoted

β, while the latter is often termed “climate-carbon feedback” and denoted by γ (Arora et al., 2013; Friedlingstein

et al., 2006; Gregory et al., 2009).

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There are some clear and obvious similarities between feedbacks in the physical climate system and the carbon

cycle system, which have aided derivation of this carbon cycle feedback framework but may also have mis-

directed carbon cycle research attention. A radiative imbalance which warms the planet in turn increases the

amount of outgoing energy radiated by the Earth and so represents a very strong negative (stabilising) feedback.

On top of this stabilising response there are many feedbacks within the climate system caused by physical

components responding to the change in global temperature. The response of clouds is commonly acknowledged

to be the largest source of model spread but others include ice and snow-albedo feedbacks, water vapour or

atmospheric lapse rate (Bony et al., 2006; Soden et al., 2008).

However, in the case of climate feedbacks, the stabilising negative response (Planck response) is extremely

well known and almost all of the uncertainty in the overall climate sensitivity comes from the multitude of

additional physical feedbacks within the climate system (see Gregory et al., (2009), figure 2), whereas in the

carbon cycle case the stabilising negative response – carbon sinks induced by elevated CO2 – is not quantitatively

well known. Gregory et al. (2009) showed that in fact it is both stronger and more uncertain than the carbon cycle

response to climate.

These similarities between carbon cycle and climate feedback formalisms led early analyses to focus on the

positive feedbacks in the system. These were analogies to the climate feedbacks and were often seen as the largest

source of uncertainty (Matthews et al., 2005; Raddatz et al., 2007). Even before the first generation of C4MIP

modelling results, Friedlingstein et al. (2003) derived an uncertainty analysis to show that the carbon cycle

response to climate (“γ”) contributes the majority of the differences between the first Hadley Centre and IPSL

carbon cycle feedback experiments (Cox et al., 2000; Friedlingstein et al., 2001). While this remains true: γ

contributes most of the uncertainty in the climate carbon cycle gain, it neglects the underlying uncertainty in the

unmodified sinks themselves.

Here we derive analytical expressions to substantially extend the analysis of Friedlingstein et al (2003) and

allow us to quantify the contribution of uncertainty in carbon cycle components to different quantities of interest.

We show that TCRE and the airborne fraction (AF, the ratio of atmospheric CO2 increase to anthropogenic CO2

emissions) can be derived from process-level feedback metrics and that although the derivation assumes linearity

(as per Friedlingstein 2003; 2006) our framework can accurately reproduce TCRE and AF of two generations of

ESMs and therefore can be used to identify sources of uncertainty in these quantities.

The linearized feedback framework adopted by C4MIP in Friedlingstein et al (2006) was first derived by

Friedlingstein et al (2003). They defined α, β, γ such that:

∆𝑇 = 𝛼∆𝐶𝑎 (1)

∆𝐶 = 𝛽∆𝐶𝑎 + 𝛾∆𝑇 (2)

where T, C and Ca are global mean temperature, land plus ocean carbon stock and atmospheric CO2

concentration respectively. The carbon store, and β and γ terms can be split into land and ocean components often

denoted by “L” and “O” suffices respectively (e.g. CL or βO) but here we combine into a single term for clarity.

They also showed that the carbon cycle feedback gain, g, could be expressed in terms of these quantities:

𝑔 = −𝛼𝛾

1+𝛽 (3)

This applies to quantities expressed in common units, such as PgC, PgC/K, PgC/PgC. More commonly, land

and ocean carbon stores are expressed in PgC while atmospheric CO2 is in ppm, and sensitivities to it in ppm-1.

Hence the expression for g requires an additional constant, k, to account for unit conversion: k=2.12 PgC/ppm,

giving:

𝑔 = −𝛼𝛾

𝑘+𝛽 (4)

Further manipulation of these metrics (see Methods) allows us to express other quantities in terms of individual

feedbacks. Cumulative airborne fraction, AF, defined as the increase in atmospheric CO2 per unit emission (both

in units of mass of carbon) is given by:

𝐴𝐹 = 𝑘

𝑘+𝛽+𝛼𝛾 (5)

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Finally, TCRE, defined as the warming per unit emission of mass of carbon, is simply related to the airborne

fraction by the climate sensitivity parameter:

𝑇𝐶𝑅𝐸 = 𝛼

𝑘+𝛽+𝛼𝛾 (6)

Crucially, our framework can be extended to also quantify propagation of uncertainty in component feedback

parameters to gain, AF and TCRE. Identification of sources of uncertainty is important if we are to target model

development and evaluation on aspects of performance which most affect the outcomes we care about. For

derivation see Methods, but we show that the variance in gain, AF and TCRE can be given by:

𝑑𝑔2 = 𝑔2 (1

𝛼2 𝑑𝛼2 + 1

𝛾2 𝑑𝛾2 + 1

(𝑘+𝛽)2 𝑑𝛽2) (7)

𝑑𝐴𝐹2 = 𝐴𝐹4

𝑘2(𝛾2𝑑𝛼2 + 𝑑𝛽2 + 𝛼2𝑑𝛾2) (8)

𝑑(𝑇𝐶𝑅𝐸)2 = 𝐴𝐹4

𝑘4((𝑘 + 𝛽)2𝑑𝛼2 + 𝛼2𝑑𝛽2 + 𝛼4𝑑𝛾2) (9)

If required, these equations can be broken down further into land and ocean components of β and γ.

3. Results

3.1 Synthesis across multiple C4MIP generations

In order to develop and test the framework we assemble feedback metrics and related quantities from the three

generations to date of coupled climate-carbon cycle models: “C4MIP” (first generation C4MIP simulations, from

circa 2006; documented in Friedlingstein et al 2006), “CMIP5” (carbon cycle ESMs from CMIP5, documented

in Arora et al., 2013) and “CMIP6” (simulations and results documented in Jones, et al., 2016; Arora et al., 2019

respectively). Individual values from the models contributing to those studies and the values we use in this analysis

are shown in Supplementary Information, table SI.1. There are multiple choices of CMIP5 feedback metrics that

we could use. In the Supplementary Information we discuss the implications of these and explain our choice of

using feedback metrics derived from CMIP5 models at a level of 2xCO2, rather than 4xCO2.

Figure 1 summarizes these numbers graphically to help visualize changes in feedback metrics over the three

model generations. Although the original C4MIP analysis made use of a different scenario of CO2 (SRES A2)

and simulations were emissions-driven instead of concentration-driven, the comparison is useful to see, but we

note especially for ocean β and γ the reduced spread is more likely due to experimental design differences than

due to model changes. Since the adoption of the 1% p.a. simulation results are much more directly comparable

between CMIP5 and CMIP6 generations.

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Figure 1. Comparison of ESM carbon cycle feedback metrics by generation (C4MIP, CMIP5, CMIP6). Metrics shown are:

response of climate to elevated CO2 (α: red axis); response of carbon sinks to CO2 (β: green axis) split into land (left hand side of axis) and ocean (right hand side); response of carbon sinks to climate (γ: blue axis) split into land (left hand side of axis) and ocean (right hand side).

Comparing specifically between CMIP5 and CMIP6 we find that α has the same mean value but a larger spread

(Table 1), β has similar mean value but smaller spread. γ values have decreased slightly between CMIP5 and

CMIP6. Arora et al. (2019) discuss reasons for the changes, especially on land, where the introduction of a

terrestrial nitrogen cycle in approximately half the models has reduced values of both β and γ in those models.

α

(K ppm-1)

β land

(PgC ppm-1)

β ocean

(PgC ppm-1)

γ land

(PgC K-1)

γ ocean

(PgC K-1)

C4MIP 0.0061 ± 0.0012 1.34 ± 0.58 1.04 ± 0.24 -78.6 ± 43.7 -30.9 ± 15.5

CMIP5 0.0069 ± 0.0010 1.14 ± 0.56 0.93 ± 0.07 -42.0 ± 26.7 -9.2 ± 2.5

CMIP6 0.0069 ± 0.0015 1.22 ± 0.38 0.91 ± 0.09 -34.1 ± 36.6 -8.6 ± 2.8

All

models

0.0066 ± 0.0013 1.24 ± 0.52 0.96 ± 0.17 -52.2 ± 41.9 -16.7 ± 14.2

Table 1. Compiled mean and standard deviation of feedback metrics for the 3 generations of model ensembles and across all models.

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3.2 Reconstructing gain, AF and TCRE

Figure 2(a) shows the successful reconstruction of gain across C4MIP and CMIP5 generations of models with R2 of 0.89 for

the correlation of actual and reconstructed values of g (no gain values are available for CMIP6). Figure 2b and 2c show similar

success of our framework to reconstruct AF and TCRE from all three multi-model ensembles (R2 = 0.85, 0.89 respectively).

For the same reasons (see Supplementary Information) that using feedback metrics diagnosed at 2xCO2 gave a better fit to AF

and TCRE, it also means we get a worse fit to gain, g, which was diagnosed for CMIP5 at 4xCO2.

Figure 2. Actual and reconstructed values of (a) gain; (b) Airborne fraction, AF; (c) TCRE using ensemble output from C4MIP (2006) CMIP5 (2013) and CMIP6 (2019) listed in Supplementary Information, table SI1. The black dashed line is the one-to-one line for illustration.

The agreement of our reconstruction is strong – each component is accurately reproduced not only in its mean but also its

spread (shown here as standard deviation) (Table 2). This gives us confidence not only that we can reconstruct the global

behavior of these models from their component sensitivities, but also that we can reconstruct and understand their variance and

hence reliably test the dependence of these aggregate quantities on their components.

gain, g Airborne Fraction TCRE (K EgC-1)

C4MIP actual 0.149 ± 0.073 0.554 ± 0.084 1.58 ± 0.37

reconstructed 0.150 ± 0.075 0.566 ± 0.085 1.62 ± 0.39

CMIP5 actual 0.106 ± 0.048 0.563 ± 0.071 1.81 ± 0.33

reconstructed 0.084 ± 0.047 0.556 ± 0.074 1.82 ± 0.32

CMIP6 actual -- 0.532 ± 0.031 1.78 ± 0.39

reconstructed -- 0.534 ± 0.031 1.75 ± 0.39

All models actual 0.130 ± 0.067 0.548 ± 0.067 1.72 ± 0.38

reconstructed 0.099 ± 0.068 0.552 ± 0.068 1.72 ± 0.38 Table 2. Actual and reconstructed values of gain, AF and TCRE and also their uncertainty. Shown here as mean and standard deviation across the available models. Gain and AF are expressed without units, TCRE is in units of K per Exagram of carbon (1 EgC = 1015 gC).

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As with the individual feedback metrics, it is illustrative to look at changes in gain, AF and TCRE over the generations of

coupled climate carbon cycle modelling (Figure 3). As before, the different experimental design and scenario make precise

comparison impossible back to the original C4MIP but possible between CMIP5 and CMIP6. We see that AF has decreased

slightly in magnitude and markedly in spread between the two most recent generations. This change in mean and variance is

captured by our reconstruction allowing us to probe the underlying reasons, as discussed below. Conversely, TCRE has not

changed systematically between the two generations either in magnitude or spread. We note here that AF is defined and

calculated when CO2 reaches 2x pre-industrial levels in the 1% p.a. simulation and as such has different values from, and should

not be compared to, observational airborne fraction of approximately 45% derived over the recent historical record

(Friedlingstein et al., 2019).

Figure 3. Comparison of ESM sensitivities by generation (C4MIP, CMIP5, CMIP6). Metrics shown are carbon cycle feedback gain, g (left hand axis), airborne fraction, AF (middle axis) and TCRE (right hand axis).

3.3 Quantified sources of uncertainty

In order to quantify sources of uncertainty in g, AF and TCRE, we apply our framework to this 3-generation multi-model

ensemble. When we use calculated variances of α, β and γ from the ensembles we can quantify the uncertainty in each of gain,

AF and TCRE due to each feedback term. Figure 4 shows the contribution to variance in these terms which arises from model

spread in α, β and γ. We find, as expected, that the carbon cycle response to climate (γ: blue bars) is indeed the primary driver

of uncertainty in the climate carbon cycle gain, g. However, this is not the case for the more policy relevant quantities of

cumulative airborne fraction (AF) and TCRE. We find that the response to CO2 (β: green bars) is a much greater source of

uncertainty in the other quantities, being the dominant uncertainty controlling AF and jointly dominating TCRE with the climate

response to CO2 (α: red bars). Model spread of γ plays very little role in the ultimate spread of TCRE.

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Figure 4. Contributions to variance in g, AF and TCRE respectively from α (red), β (green) and γ (blue). Β and γ are further split into land (dark) and ocean (light) components.

For both β and γ we show that spread in terrestrial ecosystem response is much greater than the ocean response and therefore

contributes much more to resultant uncertainty in AF and TCRE. However, we stress that this refers only to the contribution of

components to uncertainty (or more strictly, model spread) in g, AF and TCRE from the given sets of models available here.

But of course oceans, as well as land, are still vitally important in determining the overall magnitude of the feedback responses:

the ocean contributes almost exactly the same as land to β and a significant fraction to γ (Figure 5). Only in the uncertainty

terms does land dominates.

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Figure 5. Contributions to the absolute values of β and γ, and their variances, dβ2, dγ2, from land (green) and ocean (blue) carbon cycle respectively.

4. Discussion

We discussed earlier that initial analysis of C4MIP results focussed on the climate feedback, γ, as the largest source of

uncertainty. While both carbon cycle terms (β and γ) exhibit substantial spread across models, on land and in the oceans, our

results show that the most important component to constrain depends on which measure we look at. If we want to know the

climate carbon cycle feedback gain, g, then the biggest source of uncertainty is indeed γ. But, to constrain the cumulative

airborne fraction, we need to constrain β, and to constrain TCRE we need to constrain both α and β. Our results demonstrate

that a change in emphasis is required in order to target carbon cycle research more directly at issues associated with meeting

the goals of the Paris Agreement. Specifically, we argue that there is a need to re-focus analysis and model evaluation on CO2

response and drivers of sinks. It is this response to CO2 that drives a greater amount of the future behaviour of carbon sinks

under low CO2 pathways where climate change is limited.

What does this analysis mean for projections for the 21st century? To date almost all climate-carbon cycle modelling and

feedback analysis has focussed on high, monotonic CO2 scenarios: from IS92a (Cox et al., 2000) to SRES-A2 (Friedlingstein

et al., 2006) to the RCP8.5 and 1% idealised experiments of CMIP5. These scenarios see rapid and continuous increase in CO2

reaching between 700 and 1100ppm by 2100 (Figure 6). In contrast, however, strong mitigation scenarios aimed at achieving

the climate targets of the Paris Agreement stabilise or peak and decline at much lower levels: e.g. RCP2.6 peaks CO2 at 443

ppm by 2050, just 30ppm above 2020 levels. How do we know, therefore, that our feedback analysis remains valid under the

very difference scenario characteristics?

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Figure 6. CO2 concentration scenarios commonly used – previous analysis has focussed on rapid/monotonic increase. For example Cox et al (2000) used IS92a (blue line), the first C4MIP (Friedlingstein et al., 2006) used SRES A2 (green line) and CMIP5 and CMIP6 simulations drew on both 1% per annum increase (red line: Arora et al., 2013; 2019; Ciais et al., 2013) and RCP8.5 (yellow line: Collins et al., 2013; Friedlingstein et al., 2014). Note 1% per annum increase nominally begins in 1850 but plotted here relative to 1960 for ease of comparison on this schematic figure. Policy relevant mitigation scenarios that aim to achieve global climate targets typically show overshoot of CO2 concentration – e.g. RCP2.6 and SSP5-3.4-OS (dashed lines).

Analysis of CMIP5 simulations (Jones et al., 2013) showed that in future, land, ocean and airborne fractions of emissions

were quite different under RCP2.6 than the other scenarios. This is not unexpected – Raupach (2013) showed that the near-

constancy of historical airborne fraction was a direct result of the near-exponential increase in emissions. Deviation from

exponential increase would therefore lead to deviation from a constant airborne fraction. Other recent work has shown path-

dependence of carbon cycle response and TCRE. For example, MacDougall et al. (2015) demonstrate carbon budgets after

overshoot may be smaller than without overshoot due to non-linearities in the ocean thermal and carbon response and

permafrost carbon feedbacks. Tokarskaet al. (2019) showed path dependence of the land versus ocean division of net carbon

uptake leading also to path dependence of impacts on terrestrial and marine ecosystems, although for limited overshoot cases,

carbon budgets were similar with and without overshoot. Zickfeld et al. (2016) explicitly showed non-linearity of global

temperature decrease during rampdown of CO2 and therefore a smaller TCRE to negative emissions, due to the time lag in

response to 1% increase in CO2.

As the policy focus moves towards low targets, it seems therefore likely that future emissions will deviate strongly from

continued exponential increase and therefore that the future airborne fraction will depart from its historical value of

approximately 50%. Although we know that TCRE and individual elements of the carbon cycle may behave differently under

low scenarios such as RCP2.6, very little specific feedback analysis has been conducted on low stabilisation or peak-and-

decline scenarios. Under such scenarios which limit global climate change, focus on the drivers of natural carbon sinks and

their persistence becomes even more important – for example, Schwinger & Tjiputra (2018) showed non-reversibility of

components of the ocean carbon store in response to CO2 reversal. Specifically, for CMIP6 the ScenarioMIP and C4MIP pair

of simulations based around SSP5-3.4OS will bring valuable insights into how feedback metrics change in time.

The framework we have developed here serves multiple purposes. Firstly, it allows us to construct the behaviour of key parts

of the Earth system such as airborne fraction and TCRE from process-level carbon feedback components. Secondly it allows

us to attribute uncertainty in these properties to uncertainty in components and therefore focus research priorities onto the

carbon cycle response to CO2 (“β”). Thirdly, in addition to these, it opens up possibilities of applying and combining constraints

on feedbacks. For example, if we know α we can calculate how the value and range of AF, TCRE is constrained. The β and γ

quantities are formed linearly from the contribution at each gridbox (e.g. Ciais et al., 2013; Roy et al., 2011) and so we could

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further allocate uncertainty more regionally such as to ocean basins or on land in latitude bands. Currently we have no way of

perfectly constraining these components, but our feedback framework would allow partial constraints to be combined into a

stronger one. Literature is emerging that demonstrates emergent constraints on regional aspects of carbon feedbacks such as

interannual variability in the tropics (Cox et al., 2013) or seasonal cycle in mid-latitudes (Wenzel et al., 2016) as well as on

TCR (Nijsse et al., 2020). Further work will apply these constraints to reduce spread in AF and TCRE.

5. Conclusions

The concept of TCRE has been successful in combining the full Earth system response into a single, simplifying number

which can be used to calculate remaining carbon budgets to help achieve global climate targets. But in order to understand it

and constrain its sources of uncertainty we need to break it apart again. It can be easily split into “climate” and “carbon cycle”

terms (although these are not independent as they interact) e.g. Gillett et al. (2013). Williams et al. (2017; 2020) focus on the

climate aspect and split TCR into terms of individual feedbacks and ocean heat uptake. Here we focus on the carbon cycle

aspect and explore within AF the contribution from carbon-cycle feedback components. The two approaches are complimentary

and find similar results - that both climate and carbon responses are similarly responsible for TCRE, with the balance of

uncertainty varying in time within a simulation (Williams et al., 2017) and between generations of models (this study). The

comparison between generations of models, however, should be interpreted with caution due to the small sample of models.

Ringer (2020) shows how even across 30-40 models in CMIP generations, changes in the distribution of feedbacks may happen

by chance. Our samples here of the order <10 models per generation are not enough to draw robust conclusions that changes

in uncertainty follow a systematic change. Therefore, we conclude that both climate and carbon cycle must remain vital avenues

of research to reduce uncertainty TCRE.

Based on our analysis we make some recommendations for the climate-carbon cycle research community. These

recommendations feed into the WCRP number-1 question “where does the carbon go?” (Marotzke et al., 2017) and also address

the 3 priority questions of the WCRP Grand Challenge on carbon cycle feedbacks – what processes drive land and ocean carbon

sinks? how will climate-carbon feedbacks amplify climate change? and how will it affect vulnerable carbon stores?

Our primary recommendation is to re-focus research effort onto understanding and better simulating carbon cycle response,

both land and marine, to CO2. This represents the primary driver of natural carbon sinks, the largest source of uncertainty in

future airborne fraction and contributes much more than γ to uncertainty in TCRE. If we are to reduce uncertainty in future

carbon budgets this must be our primary focus. While land contributes most to model spread, ocean sinks contribute equally to

the carbon sink and have substantial uncertainty at regional level (Hewitt et al., 2016) and become increasingly important on

timescales beyond 2100 (Jones, et al., 2016; Randerson et al., 2015).

Secondly, we have shown that reconstruction of the airborne fraction of CO2 emissions and TCRE, are achieved more

precisely using feedback metrics derived at a level of 2xCO2 in the 1% simulation than at the end (at 4xCO2). Therefore we

recommend that future feedback analyses quote values at both of these levels as has been done in Arora et al. (2019).

Thirdly, research is lacking into the behaviour of carbon cycle feedbacks in low stabilisation and overshoot scenarios. The

airborne fraction and sink efficiency are not uniform under different scenarios or rates of change. We know that TCRE and

other components of the Earth system can exhibit path dependence, so research must also focus on low stabilisation or overshoot

scenarios. For such low scenarios, both fully coupled and biogeochemically coupled simulations are required.

Fourthly, we recommend that more effort is put into understanding the full range of uncertainty within and across models.

We have demonstrated marked differences in the ensemble spread between CMIP5 and CMIP6 but we do not know how robust

this finding is, nor its full implication, due to the small set of models available. Perturbed parameter approaches (e.g. Booth et

al., 2012; MacDougall et al., 2016) offer a way to more systematically explore the uncertainty range of feedback metrics and

their implications for AF and TCRE, and we recommend that more ESM models should consider such approaches.

Finally, we stress the vital role of evaluation. As ESMs have developed in complexity, they bring unprecedented opportunity

to simulate these quantities such as AF and TCRE which inform global negotiations on carbon budgets, but they also require

increasing levels of evaluation to ensure process realism (Jones, 2020). CMIP6 sees a marked difference over CMIP5 regarding

inclusion of terrestrial nitrogen cycle in many models: a key systematic omission in previous generations. But whether CMIP6

models will systematically evaluate better than CMIP5 is not yet known. Comparison of models against the growing wealth of

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ecosystem observations and manipulation experiments (e.g., Medlyn et al., 2015; Walker et al., 2015) is crucial. Posterior

constraints on projections can also be very powerful. Our framework offers an exciting opportunity to combine existing and

new constraints and make real progress towards reduced uncertainty in assessing remaining carbon budgets.

Acknowledgements

CDJ was supported by the Joint UK BEIS/Defra Met Office Hadley Centre Climate Programme (GA01101). CDJ and PF

were supported by the European Union's Horizon 2020 research and innovation programme under CRESCENDO (grant

agreement No 641816), and PF was also supported by the European Union's Horizon 2020 research and innovation programme

under 4C (grant agreement No 821003). We acknowledge two anonymous reviewers for their helpful comments.

Data availability

No new data were created or analysed in this study. Data analysed has been assembled from previously published work.

Data sources are listed in the caption for Table SI-1 in the Supplementary Information.

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cumulative CO2emissions during periods of net negative CO2emissions. Environmental Research Letters, 11(5), 55006.

https://doi.org/10.1088/1748-9326/11/5/055006

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17

Methods

The linearized feedback framework adopted by C4MIP in Friedlingstein et al. (2006) was first derived by Friedlingstein et

al. (2003). They defined α, β, γ such that:

∆𝑇 = 𝛼∆𝐶𝑎

∆𝐶 = 𝛽∆𝐶𝑎 + 𝛾∆𝑇

where T, C and Ca are global mean temperature, land plus ocean carbon stock and atmospheric CO2 concentration

respectively. The carbon store, and β and γ terms can be split into land and ocean components often denoted by “L” and “O”

suffices respectively (e.g. CL or βO) but here we combine into a single term for clarity.

In the following sections we show the derivation of gain, g, in terms of , , sensitivity components and also similar

derivations for the cumulative airborne fraction, AF, and TCRE. We then derive analytical expressions for the uncertainty terms

of each and calculate, based on CMIP5 ESM outputs, the fractional cause of uncertainty (percent of variance explained) in each

of g, AF, TCRE due to each feedback term.

Derivation of terms

Gain, g, is defined so that the ratio of CO2 increase with vs without climate change is given by:

∆𝐶𝑎𝐶𝑂𝑈

∆𝐶𝑎𝑈𝑁𝐶

= 1 + 𝑔 + 𝑔2 + 𝑔3 + ⋯ = 1

1 − 𝑔

Therefore, under the same emissions:

𝐸 = ∆𝐶𝑎𝐶𝑂𝑈 + ∆𝐶𝐶𝑂𝑈 = ∆𝐶𝑎

𝑈𝑁𝐶 + ∆𝐶𝑈𝑁𝐶

So (assuming ΔTUNC≈0)

∆𝐶𝑎𝐶𝑂𝑈 + (𝛽∆𝐶𝑎

𝐶𝑂𝑈 + 𝛾∆𝑇𝐶𝑂𝑈) = ∆𝐶𝑎𝑈𝑁𝐶 + (𝛽∆𝐶𝑎

𝑈𝑁𝐶)

∆𝐶𝑎𝐶𝑂𝑈(1 + 𝛽 + 𝛼𝛾) = ∆𝐶𝑎

𝑈𝑁𝐶(1 + 𝛽)

Hence

1

1 − 𝑔=

∆𝐶𝑎𝐶𝑂𝑈

∆𝐶𝑎𝑈𝑁𝐶

= (1 + 𝛽)

(1 + 𝛽 + 𝛼𝛾)

Which gives

𝑔 = −𝛼𝛾

1 + 𝛽

This only holds if all carbon quantities are in the same units (i.e. C and Ca are both in PgC) and β is in PgC PgC-1. If, as we

commonly do, we want Ca in ppm, C in PgC and β in PgC ppm-1 then we need a unit conversion factor, k=2.12 PgC ppm-1.

𝑔 = −𝛼𝛾

𝑘 + 𝛽

Cumulative airborne fraction, AF, defined as the increase in atmospheric CO2 per unit emission, both in units of mass of

carbon. Again, taking care with units so that we can use α, β and γ in their common units (K ppm-1, PgC ppm-1, PgC K-1

respectively):

𝐴𝐹 =𝑘 ∆𝐶𝑎

𝐸

Where

𝐸 = 𝑘∆𝐶𝑎 + ∆𝐶 = 𝑘∆𝐶𝑎 + 𝛽∆𝐶𝑎 + 𝛼𝛾∆𝐶𝑎

Hence:

𝐴𝐹 = 𝑘

𝑘 + 𝛽 + 𝛼𝛾

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18

Transient Climate Response to cumulative carbon Emissions, TCRE, defined as the warming per unit emission of mass

of carbon (here taken as being expressed in units of K PgC-1, although often per exa-gram is used). Here the conversion factor

is required to convert a fraction of emissions into ppm in order to combine it with α which is warming per ppm

𝛥𝑇 = 𝑇𝐶𝑅𝐸 ∗ 𝐸 = 𝐴𝐹. 𝐸

𝑘 𝛼

So:

𝑇𝐶𝑅𝐸 = 𝛼

𝑘 + 𝛽 + 𝛼𝛾

Derivation of uncertainty terms

Our framework can be extended to also quantify propagation of uncertainty in component feedback parameters to gain, AF

and TCRE.

Gain uncertainty terms.

g is linear in α and γ, so

𝜕𝑔

𝜕𝛼= −

𝛾

𝑘 + 𝛽=

𝑔

𝛼

Similarly for γ. Also:

𝜕𝑔

𝜕𝛽= 𝛼𝛾 (𝑘 + 𝛽)−2 = −

𝑔

𝑘 + 𝛽

If we assume the terms of variance are independent, we can combine by sum of squares:

𝑑𝑔2 = (𝜕𝑔

𝜕𝛼𝑑𝛼)

2

+ (𝜕𝑔

𝜕𝛽𝑑𝛽)

2

+ (𝜕𝑔

𝜕𝛾𝑑𝛾)

2

𝑑𝑔2 = 𝑔2 (1

𝛼2 𝑑𝛼2 +

1

𝛾2𝑑𝛾2 +

1

(𝑘 + 𝛽)2𝑑𝛽2)

To split into land/ocean components, we repeat above with γ = γL+ γO etc. and get:

𝑑𝑔2 = 𝑔2 (1

𝛼2 𝑑𝛼2 +

1

𝛾2𝑑𝛾𝐿

2 + 1

𝛾2𝑑𝛾𝑂

2 + 1

(𝑘 + 𝛽)2𝑑𝛽𝐿

2 + 1

(𝑘 + 𝛽)2𝑑𝛽𝑂

2)

AF uncertainty terms

Writing: 𝐴𝐹 = 𝑘(𝑘 + 𝛽 + 𝛼𝛾)−1, and 𝐴𝐹2 = 𝑘2(𝑘 + 𝛽 + 𝛼𝛾)−2 then:

𝑑𝐴𝐹

𝑑𝛼= −𝑘𝛾(𝑘 + 𝛽 + 𝛼𝛾)−2 = −

𝛾𝐴𝐹2

𝑘

And by symmetry the same for γ.

Then simply for β:

𝑑𝐴𝐹

𝑑𝛽= −𝑘(𝑘 + 𝛽 + 𝛼𝛾)−2 = −

𝐴𝐹2

𝑘

Leaving:

𝑑𝐴𝐹2 = 𝐴𝐹4

𝑘2(𝛾2𝑑𝛼2 + 𝑑𝛽2 + 𝛼2𝑑𝛾2)

TCRE uncertainty terms

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Journal XX (XXXX) XXXXXX Author et al

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If 𝑇𝐶𝑅𝐸 = 𝛼

𝑘𝐴𝐹, then:

𝜕(𝑇𝐶𝑅𝐸)

𝜕𝛼=

𝐴𝐹

𝑘+

𝛼

𝑘 𝜕𝐴𝐹

𝜕𝛼

= (𝐴𝐹

𝑘− 𝛼𝛾

𝐴𝐹2

𝑘2)

= 𝐴𝐹2

𝑘2(

𝑘

𝐴𝐹− 𝛼𝛾)

= 𝐴𝐹2

𝑘2(𝑘 + 𝛽)

And:

𝜕(𝑇𝐶𝑅𝐸)

𝜕𝛽=

𝛼

𝑘

𝜕𝐴𝐹

𝜕𝛽

= −𝛼𝐴𝐹2

𝑘2

And:

𝜕(𝑇𝐶𝑅𝐸)

𝜕𝛾=

𝛼

𝑘

𝜕𝐴𝐹

𝜕𝛾

= −𝛼2𝐴𝐹2

𝑘2

Therefore:

𝑑(𝑇𝐶𝑅𝐸)2 = 𝐴𝐹4

𝑘4((𝑘 + 𝛽)2𝑑𝛼2 + 𝛼2𝑑𝛽2 + 𝛼4𝑑𝛾2)

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Journal XX (XXXX) XXXXXX Author et al

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Glossary

We define briefly here some terms used throughout the text. Terms are clustered by category rather than strictly alphabetical.

Explanations are intended to help understand the usage of these terms in the context of this paper and are not intended to be

exhaustive definitions of each term.

Measures of climate response:

AF: Airborne Fraction. Denotes the fraction of anthropogenic CO2 emissions which remain in the atmosphere.

TCR, ECS: Transient Climate Response and Equilibrium Climate Sensitivity. Deonte the response of global mean

temperature to a doubling of CO2. Transient climate response is measured at the time of CO2 doubling in an idealized model

simulation where CO2 increases at a compound rate of 1% per year. Equilibrium climate sensitivity is diagnosed as half of the

long-term warming in response to a constant 4x CO2 simulation.

TCRE: Transient Climate Response to cumulative carbon Emissions. Denotes the climate response to emissions rather than

concentration of CO2. Defined as the warming per unit CO2 emission at the time of doubling of CO2 in order to be consistent

with TCR.

Model terms and modelling activities:

GCM, ESM: General Circulation Model and Earth System Model. GCMs represent the fluid dynamics of the atmosphere

and ocean at discrete gridboxes of approximately 1-2 degrees resolution. They have formed the basis of climate modelling for

several decades. Earth system models are GCMs which additionally include biogeochemical processes and feedbacks – taken

here to primarily mean the carbon cycle and hence the ability to simulate carbon cycle feedbacks which affect atmospheric

CO2.

CMIP5, CMIP6: Coupled Model Intercomparison Project, Phases 5 and 6. Coordinated modelling activity which sets out

an agreed experimental design for model centres around the world to perform numerical simulations (see, e.g., Eyring et al.,

2016). Typically, successive IPCC Assessment Reports draw on results from CMIP generations.

C4MIP, ZECMIP: Coupled Climate-Carbon Cycle MIP (Jones, et al., 2016) and Zero Emissions Commitment MIP (Jones

et al., 2019). These modelling activities set out experimental designs to explore carbon cycle feedbacks and committed climate

changes after emissions cease.

Carbon cycle feedback experiments and terminology:

Coupled, BGC, RAD simulations: refer to simulations in which all of the model components interact (“coupled”) or can

be isolated from changes in atmospheric CO2. “BGC” coupled runs involve the carbon cycle components responding to elevated

CO2 but not the atmospheric radiation scheme. Conversely “RAD” coupled runs involve the CO2 being radiatively active but

the ecosystems do not experience elevated CO2. These simulations allow specific responses within the model to be isolated and

quantified individually.

Feedback metrics, alpha, beta, gamma, gain (α, β, γ): From the above coupled and partially-coupled simulations feedback

metrics can be calculated: α represents the global warming per ppm of CO2 rise; β (split into land and ocean) the change in

carbon store due to CO2 rise; γ (split into land and ocean) the change in carbon store per degree Celsius of global temperature

change. The carbon cycle feedback is characterized by a feedback gain, g, which determines the amplification of atmospheric

CO2 in fully coupled compared with BGC coupled simulations. α is related to TCR: conventionally it is the warming at a given

point in the simulations divided by the change in CO2. If it is diagnosed at 2xCO2 in the 1% simulation then it is equivalent to

TCR (albeit in units of K ppm-1 rather than K), but it can also be diagnosed at other levels of CO2 or in other scenarios of CO2

increase.

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