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Accepted Manuscript Extremely high aerosol loading over Arabian Sea during June 2008: the specific role of the atmospheric dynamics and Sistan dust storms D.G. Kaskaoutis, A. Rashki, E.E. Houssos, D. Goto, P.T. Nastos PII: S1352-2310(14)00359-8 DOI: 10.1016/j.atmosenv.2014.05.012 Reference: AEA 12956 To appear in: Atmospheric Environment Received Date: 19 March 2014 Revised Date: 3 May 2014 Accepted Date: 6 May 2014 Please cite this article as: Kaskaoutis, D.G., Rashki, A., Houssos, E.E., Goto, D., Nastos, P.T., Extremely high aerosol loading over Arabian Sea during June 2008: the specific role of the atmospheric dynamics and Sistan dust storms, Atmospheric Environment (2014), doi: 10.1016/ j.atmosenv.2014.05.012. This is a PDF file of an unedited manuscript that has been accepted for publication. As a service to our customers we are providing this early version of the manuscript. The manuscript will undergo copyediting, typesetting, and review of the resulting proof before it is published in its final form. Please note that during the production process errors may be discovered which could affect the content, and all legal disclaimers that apply to the journal pertain.

Extremely high aerosol loading over Arabian Sea during June 2008: The specific role of the atmospheric dynamics and Sistan dust storms

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Accepted Manuscript

Extremely high aerosol loading over Arabian Sea during June 2008: the specific roleof the atmospheric dynamics and Sistan dust storms

D.G. Kaskaoutis, A. Rashki, E.E. Houssos, D. Goto, P.T. Nastos

PII: S1352-2310(14)00359-8

DOI: 10.1016/j.atmosenv.2014.05.012

Reference: AEA 12956

To appear in: Atmospheric Environment

Received Date: 19 March 2014

Revised Date: 3 May 2014

Accepted Date: 6 May 2014

Please cite this article as: Kaskaoutis, D.G., Rashki, A., Houssos, E.E., Goto, D., Nastos, P.T.,Extremely high aerosol loading over Arabian Sea during June 2008: the specific role of theatmospheric dynamics and Sistan dust storms, Atmospheric Environment (2014), doi: 10.1016/j.atmosenv.2014.05.012.

This is a PDF file of an unedited manuscript that has been accepted for publication. As a service toour customers we are providing this early version of the manuscript. The manuscript will undergocopyediting, typesetting, and review of the resulting proof before it is published in its final form. Pleasenote that during the production process errors may be discovered which could affect the content, and alllegal disclaimers that apply to the journal pertain.

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Extremely high aerosol loading over Arabian Sea during June 2008: the 1

specific role of the atmospheric dynamics and Sistan dust storms 2

3

D.G. Kaskaoutis1*, A. Rashki2, E.E. Houssos3, D. Goto4, P.T. Nastos5 4

5

1School of Natural Sciences, Department of Physics, Shiv Nadar University, Tehsil Dadri, – 6

203207, India 7

2Natural Resources and Environment College, Ferdowsi University of Mashhad, Mashhad, Iran 8

3Laboratory of Meteorology, Department of Physics, University of Ioannina, 45110 Ioannina, 9

Greece 10

4National Institute for Environmental Studies (NIES), Tsukuba, Ibaraki 305-8506, Japan 11

5Laboratory of Climatology and Atmospheric Environment, Faculty of Geology and 12

Geoenvironment, University of Athens, 15784 Zografou, Greece 13

14

*Corresponding author: Dimitris G. Kaskaoutis: [email protected], 15

[email protected] Tel-Fax: +911202663801 16

17

Abstract 18

This study focuses on analyzing the extreme aerosol loading and the mechanisms, source areas 19

and meteorological conditions that favored the abnormal dust exposure towards Arabian Sea 20

during June 2008. The analysis reveals that the spatial-averaged aerosol optical depth (AOD) 21

over Arabian Sea in June 2008 is 0.5 (78.2%) higher than the 2000-2013 mean June value and is 22

mostly attributed to the enhanced dust activity and several (18) dust storms originated from the 23

Sistan region (Iran-Afghanistan borders). Landsat images show that the marshy lakes in Sistan 24

basin got dried during the second half of June 2008 and the alluvial silt and saline material got 25

easily eroded by the intense Levar winds, which were stronger (>15-20 ms-1) than the 26

climatological mean for the month of June. These conditions led to enhanced dust exposure from 27

Sistan that strongly affected the northern and central parts of the Arabian Sea, as forward air-28

mass trajectories show. The NCEP/NCAR reanalysis reveals an abnormal intensification and 29

spatial expansion of the Indian low pressure system towards northern Arabian Sea in June 2008. 30

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This suggests strengthening of the convection over the arid southwest Asia and exposure of 31

significant amount of dust, which can reach further south over Arabian Sea favored by the 32

enhanced cyclonic circulation. MODIS imagery highlighted several dust storms originated from 33

Sistan and affecting Arabian Sea during June 2008, while the SPRINTARS model simulations of 34

increased AOD and dust concentration over Sistan and downwind areas are in agreement with 35

ground-based and satellite observations. 36

37

Keywords: Arabian Sea; severe AOD; dust storms; remote sensing; synoptic meteorology; 38

SPRINTARS 39

40

1. Introduction 41

The aerosol field over Arabian Sea is strongly influenced by the Asian pollution outflow during 42

the post-monsoon and winter seasons and by dust storms originated from Middle East, Arabia 43

and southwest Asia during pre-monsoon and monsoon seasons (Tindale and Pease, 1999; Dey 44

and di Girolamo, 2010), resulting in the highest annual aerosol optical depth (AOD) of about 0.6-45

0.8 during June - August (Kaskaoutis et al., 2011). Satellite observations have shown a strong 46

south-to-north gradient in AOD, with values above 1.0-1.2 in the northernmost part associated 47

with larger contribution of aerosols of desert origin (Satheesh et al., 2010; Prijith et al., 2013). 48

The vertical profile of aerosols also revealed the significant continental dust outflow, which 49

progressively increases in altitude (>2-3 km) along its transport over central and southern 50

Arabian Sea (Prijith et al., 2013). The dominance of the dust aerosols over central and northern 51

parts of the Arabian Sea was also revealed from ship-cruise campaigns (ARMEX, ICARB) 52

during the pre-monsoon (Kalapureddy et al., 2009) and monsoon (Moorthy et al., 2005) seasons. 53

The aerosol field over Arabian Sea, its variations and the dusty clouds that are usually formed 54

are interlinked with the southwest Indian summer monsoon (Rahul et al., 2008; Manoj et al., 55

2011, 2013; Vinoj et al., 2014), while previous studies have shown some teleconnections with 56

El-Nino Southern Oscillation (ENSO) (Gadgil et al., 2003; Abish and Mohanakumar, 2013). 57

Furthermore, the seasonal change of the Inter-Tropical Convergence Zone (ITCZ) controls the 58

meteorological and atmospheric dynamics over Arabian Sea (Krishnamurthi et al., 1998), while 59

Satheesh et al. (2006) found large negative aerosol radiative forcing at surface associated with an 60

overall top of the atmosphere cooling. 61

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The Sistan region, which is located in the southeastern Iran along the Afghanistan and Pakistan 62

borders, has been considered as a major dust source in southwest Asia (Middleton, 1986; 63

Prospero et al., 2002; Léon and Legrand, 2003; Ginoux et al., 2012; Goudie et al., 2013) due to 64

the extreme intensity of the northerly Levar or “120-day” wind during the June-September 65

period (McMahon, 1906). Several papers have investigated the dust activity, outflows and 66

relation with the Levar wind over the region (Rashki et al., 2012, 2013a, b, 2014; Alizadeh 67

Choobari et al., 2013; Ekhtesasi and Gohari, 2013; Rezazadeh et al., 2013). The dust outbreaks 68

originated from Sistan take place in the northernmost lowland of the region, which is covered by 69

shallow (<4 m in depth), marshy and ephemeral lakes (Hamouns, approximately 160 km long 70

and 8–25 km wide with nearly 4,500 km2 surface area) that are fed from the discharge of the 71

Helmand river in Afghanistan. Rashki et al. (2013c) and Sharifikia (2013) revealed the strong 72

linkage between the dust activity and water coverage in the Hamoun dry-bed lakes. Due to 73

extreme hot-dry conditions during the summer months and, depending on the snowfall and 74

snowmelt in southern Hindu Kush mountains and on the precipitation variability over the region, 75

the lakes usually get dried, as occurred in several years during the last decade (Rashki et al., 76

2013c). When the lakes get dried, a saline alluvial clay material is left at the dried beds, which is 77

easily eroded by the strong Levar wind (>15 ms-1), thus forming intense dust storms that cover 78

Sistan and downwind areas, also affecting Karachi (Alam et al., 2011) and northern part of the 79

Arabian Sea. 80

The dust-storm occurrence over Sistan has a significant inter-seasonal and intra-annual 81

variability due to the reasons mentioned above, thus contributing to significant fluctuation in the 82

aerosol loading over the downwind areas, one of which is the northern Arabian Sea. In the 83

present study, we highlight the significant role that the Sistan dust storms play in the aerosol 84

loading over Arabian Sea, focusing on June 2008, when an extremely high aerosol loading 85

covered its northern and central parts. This work supplements the results obtained by Prijith et al. 86

(2013), who analyzed the atmospheric and meteorological conditions over Arabian Sea during 87

June 2008 providing some reasons for the exceptionally high AOD, but without reporting the 88

main dust source region, the topographic and meteorological dynamics that favored the 89

enhancement in dust activity. Thus, the role of the Sistan basin and the associated dust storms in 90

the aerosol loading over Arabian Sea remain unexplored. These issues are analyzed and 91

discussed in the current work by the synergy of ground-based (Zabol station) meteorological 92

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data, synoptic meteorological reanalysis (NCEP/NCAR), satellite (Landsat, MODIS) remote 93

sensing, HYSPLIT air-mass trajectories and model (SPRINTARS) simulations. 94

95

2. Dataset 96

The dataset used in the current work consists of meteorological observations of surface wind at 97

10 m above ground level (agl) and horizontal visibility (vis) taken at Zabol meteorological 98

station located ~10-20 km away from the Hamoun lakes (Rashki et al., 2012). This dataset is 99

used in order to reveal the intensity of the northerly Levar wind and the frequency of occurrence 100

of dust-storms (vis<1 km, WMO 2005) over Sistan during June 2008. These observations are 101

compared with the climatological means reported elsewhere (Rashki et al., 2012) in order to 102

highlight the specific meteorological/atmospheric conditions over Sistan during June 2008 103

having as a consequence the significant dust aerosol outflow and the high loading over Arabian 104

Sea. 105

Level 3 collection 5 (C005.1) Terra MODIS AOD550 values using the dark target approach (Levy 106

et al., 2010) were obtained over Arabian Sea (8-26oN, 54-75oE) in order to reveal the high 107

abnormal AOD during June 2008 and the anomalies (spatially and temporally averaged) from the 108

long-term (2000-2013) AOD550 mean. Cloud-screening has been performed in the used MODIS 109

dataset via the procedure described in Levy et al. (2007). The dataset underlines the extreme 110

aerosol loading over Arabian Sea during June 2008, the source of which is worth to be examined. 111

Furthermore, MODIS imagery of certain dust storms originated from Sistan is provided as well 112

as Landsat ETM+ L1T (Enhanced Thematic Mapper plus) false color composite images over 113

Sistan focusing on land use – land cover changes and dryness of the Hamoun lakes during June 114

2008. 115

5-days forward air-mass trajectories were obtained via the HYSPLIT model (Draxler and Rolph, 116

2003) in order to reveal the transport pathways of the dusty air masses originated from the Sistan 117

basin (31.5oN, 61.5oE) at 500 m agl during 18 dust-storm events (vis< 1km) that were identified 118

during June 2008. This analysis helps in understanding the pathways and the altitudinal variation 119

of the dust plume along its transport, and to identify the downwind areas that are mostly affected 120

by the Sistan dust storms during June 2008. 121

Composite means of the geopotential heights at 1000 hPa, 850 hPa and 700 hPa were obtained 122

from the National Center for Environmental Prediction/National Center for Atmospheric 123

Research (NCEP/NCAR) re-analysis project (Kalnay et al., 1996) aiming to identify the synoptic 124

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meteorological conditions that prevailed over southwest Asia during June 2008 as well as the 125

composite anomalies from the mean climatology (1981-2010) in June. This analysis reveals the 126

important role of the atmospheric circulation on the excessive dust outflow from southwest Asia 127

towards Arabian Sea during June 2008. The NCEP/NCAR maps cover a broad region of south-128

central Asia (40o to 120o E and 0o to 50o N) with 2.5o x 2.5o spatial resolution. 129

Finally, the SPRINTARS (Spectral Radiation-Transport Model for Aerosol Species) model was 130

used to simulate the AOD550 and dust concentration over south Asia during June 2008 and to 131

reveal differences from the long-term (2001-2010) means. SPRINTARS simulates AOD for 132

various aerosol components (black carbon, organic carbon, sulfate, soil dust and sea salt) with 133

prescribed optical properties and meteorological fields from NCEP/NCAR reanalysis (wind 134

field, water vapor and temperature) with the T106 horizontal resolution (1.1°x1.1°) (Nakajima et 135

al., 2000; Takemura et al., 2009). The dust emission processes are online-calculated at 6 bins 136

(from 0.1 to 10 µm) according to an empirical relation by Gilletee (1978), depending on near-137

surface wind speed above 6.5 ms-1, vegetation cover, leaf area index, soil moisture and snow 138

amount (Goto et al., 2011). The sea-salt emissions over the oceanic environment are also online-139

calculated at 4 bins (from 0.1 to 10 µm) as a function of wind speed using Monahan’s (Monahan 140

et al., 1986) parameterization. The SPRINTARS AODs have been compared with various 141

satellites, including MODIS, under AeroCom (http://aerocom.met.no/) project (Kinne et al., 142

2006), while the dust loading, which dominates in the current simulations, was also compared to 143

various measurements under the same project (Huneeus et al., 2011), revealing that SPRINTARS 144

simulations are well within the uncertainty of the other global aerosol models and have 145

satisfactory agreement with observations. 146

147

3. Results and Discussion 148

3.1 The anomalous high AOD over Arabian Sea in June 2008 149

Figure 1 shows the spatial-averaged monthly mean AOD550 values over Arabian Sea (8o – 26oN, 150

54o – 74oE) in June during the period 2000-2013 in box & whisker view. The Terra MODIS 151

AOD550 over the region ranges from 0.4 to 0.75 on monthly-mean basis exhibiting a mean of 152

0.59±0.13. However, during June 2008 an abnormal high AOD550 of 1.09±0.49 is observed over 153

the marine environment, which is 0.50 (72.8%) above than the 14-years (2000-2013) mean or 154

97% higher than the 2000-2010 mean according to Prijith et al. (2013). Detailed discussions 155

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about the wind field, continental outflow, vertical aerosol structure and possible reasons favoring 156

the extreme aerosol loading in June 2008 are included in Prijith et al. (2013). 157

The mean MODIS-AOD550 distributions over Arabian Sea during June 2000-2013 and June 2008 158

are shown in Fig. 2a, b, respectively for comparison purposes. The spatial distribution of the 159

AOD550 anomalies in June 2008 with respect to the long-term mean is shown in Fig. 3. The June 160

2000-2013 AOD spatial distribution (Fig. 2a) shows enhanced values over northernmost eastern 161

Arabian Sea along the Pakistan coast and over the Oman Sea at the western part. The AODs over 162

these areas are in the range of 0.8-1.0 and are strongly influenced by the nearby desert regions. 163

More specifically, the high AOD along the Pakistan coast is mostly attributed to dust outbreaks 164

primarily from Sistan and secondarily from dust-source regions located in valleys (Dasht-e Lut) 165

and from salt/dry lakes along the coastal Makran Mountains (e.g. Hamun-e-Jaz Murian, 1087 166

km2, http://commons.wikimedia.org/wiki/File:Dasht-e_Lut_Dust_Storm_Iran_TMO_2010023_lrg.jpg). 167

The high aerosol loading along the Oman coast is associated with dust exposure from the Oman 168

and Rub Al Khali deserts, which are the most active dust sources in Arabian Peninsula (Najafi et 169

al., 2013; Rezazadeh et al., 2013). The aerosol loading is significantly lower over the central part 170

of the Arabian Sea, while the southern part can be characterized as moderate-polluted marine 171

environment, with AOD around 0.4. This long-term aerosol field is strongly altered in June 2008 172

(Fig. 2b), when very high (>2) AOD550 values are observed over the northeastern coast and along 173

the Oman coast. However, the extreme aerosol loading is not limited only over these areas, but 174

covers nearly the whole Arabian Sea northern than 12oN, with anomalies from the 14-year mean 175

as high as 1-1.5 in absolute AOD550 values corresponding to ~150-200% (Fig. 3). The spatial-176

averaged AOD550 was found to range from 0.36 (5 June) to 2.95 (19 June), while its mean value 177

was above 0.9 from 8 to 30 June 2008, except of 25 June, revealing the intensity and permanency 178

of the phenomenon. 179

The latitudinal-mean gradient of AOD550 over Arabian Sea in June shows a progressively 180

increasing trend from south-to-north (Fig. 4a), which is analytically investigated along with 181

radiative forcing values in Satheesh et al. (2010). On long-term basis, the AOD550 increases from 182

0.4 at 8oN to about 0.7 at the northernmost Arabian Sea (23o - 24oN). This pattern is drastically 183

changed during June 2008, when the nearly similar AOD550 at 8o increases to 1.6-1.7 at 18o – 184

21oN corresponding to a mean difference of about 1.0 or 140% (Fig. 4b) from the long-term 185

mean. It is characteristic that the AOD exhibits its highest increase about 4o-6o southern from the 186

north Arabian Sea coast suggesting extensive continental outflow and accumulation of dust at 187

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about 400-500 km south of the Pakistan coast. In synopsis, the analysis revealed that the very 188

high aerosol loading during June 2008 is associated with enhanced values over nearly the whole 189

Arabian Sea and not only limited over its northern part. This suggests a large dynamic for long-190

range transport of the dusty continental air masses from the northern arid regions, which was not 191

seen in the other years. 192

193

3.2 Sistan meteorology and dust storms during June 2008 194

The Landsat ETM+L1T false color composite images (bands 4, 3, and 2) show a small water 195

coverage in the Hamoun lakes on 5 June 2008 (Fig. 5), which have been absolutely dried by the 196

end of June (right image). The dry-bed lakes are then composed by a saline clay alluvial material 197

(Rashki et al., 2013c), which is easily eroded by the strong Levar wind, resulting in significant 198

dust uplift and massive dust outbreaks, especially during the second half of June 2008. 199

Therefore, one of the critical reasons for the high aerosol loading over southwest Asia and the 200

consequent outflow over Arabian Sea during June 2008 is the dryness of the Hamoun lakes and 201

the enhancement in dust activity over the Sistan basin. The visibility recordings at Zabol 202

meteorological station showed that 18 out of the 30 days in June 2008 were considered as dust 203

storms with horizontal visibility less than 1 km. More specifically, from 16 June to 1 July the 204

visibility was always below 1 km and on some days (16-17, 27-30 June), it fell down to 100 m 205

corresponding to severe dust/sand storms, as the station is very close to the dust-source region. 206

Aqua-MODIS true color images over Arabian Sea on several days during the second half of June 207

2008 (Fig. 6) reveal high turbid atmospheres and significant amount of dust transported over the 208

marine environment. The Sistan/Hamoun basin seems to be very active in dust-storm outflows 209

on all days, except 24 June. The dust plumes follow an anti-clockwise direction forming a giant 210

“U” (see the arrows), which has been highlighted in previous studies (Alam et al., 2011; Rashki 211

et al., 2012, 2013b, c). The dust storms originated from Sistan are initially moving southwards 212

driven by the strong northern Levar wind and, then, are progressively shifting towards east-213

northeast affecting mostly the northernmost eastern part of Arabian Sea and south-central 214

Pakistan. Furthermore, the MODIS observations show that the dust plumes from the northern 215

arid continents strongly affect a large part of the Arabian Sea, while another significant dust 216

pathway is revealed along the Indus basin, affecting the northeastern part of the Arabian Sea and 217

the northwestern Indian coast (see arrows on 16-19 June and 28-30 June). On several cases, the 218

strong Levar wind seems to activate (but in a much lesser degree) other dust sources along the 219

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Makran mountains affecting Oman Sea, while the contribution of the southern Arabian Peninsula 220

could not be ignored (dust storms on 17-21 June). A strong SW flow dominates over central-221

western parts of the Arabian Sea along the southern edge of the Arabian Peninsula and the horn 222

of Africa, which also contributes to dust transport over Arabian Sea, as the arrows show. The 223

dust-plume pathways and travelling altitude over Arabian Sea are controlled by the concurrent 224

flow of the north Levar and the southwesterly monsoonal winds (Rashki et al., 2014). In general, 225

these two oppose wind regimes shift the dusty air masses originated from Sistan towards eastern 226

directions after reaching the northernmost part of the Arabian Sea. The Indian summer thermal 227

low and its variations in turbulence, vorticity, convergence, may also affect the long-range 228

transport and the altitudinal variation of the dust plumes over Arabian Sea (Aloysius et al., 2011; 229

Prijith et al., 2013). 230

However, during June 2008 the dusty air masses originated from Sistan, except of the 231

northernmost eastern part of the Arabian Sea, seem to affect the central and western parts as 232

well, and considering the numerous (18) dust storms during that month, the high dust-aerosol 233

loading over Arabian Sea can be explained. Figure 7 shows that the dusty air masses originated 234

from Sistan are mostly transported within the lower boundary layer over the arid terrain in 235

southwestern Pakistan and when they reach over Arabian Sea they are progressively increasing 236

in altitude to above 2-3.5 km. CALIPSO profiles of extinction coefficient and volume 237

depolarization ratio revealed increased dust occurrence at this altitude over northern part of 238

Arabian Sea progressively decreasing in intensity towards the south (Prijith et al., 2013). In 239

synopsis, the current analysis reveals that the abnormal high dust-aerosol loading over Arabian 240

Sea during June 2008 is attributed to intense dust activity and several dust-storm exposures from 241

Sistan basin. The absolute dryness of the Hamoun lakes during the second-half of June 2008 242

favored the occurrence of intense and persistent dust storms, which lowered the visibility over 243

the source region at less than 1 km for 17 consecutive days (16 June – 1 July 2008). The soil 244

moisture at 0-10 cm, which is a crucial parameter for dust erosion (Goudie and Middleton, 245

2001), was found to be lower (11.2 kgm-2; MERRA 2D observations over Sistan basin) during 246

June 2008 compared to the summer (June-September 2000-2013) mean of 11.6 kgm-2. The 247

dryness of the soil was continued during July-September 2008 (10.8 kgm-2), but the dust activity 248

was much lower (less than 8 dust storms per month) due to weakening of the Levar. During 16 – 249

30 June the intensity of the Levar wind over Hamoun dry-bed lakes was significantly increased 250

(mean of 22.5±4.3 ms-1), which is much larger than the climatological (1963-2010) June mean of 251

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12.5 ms-1. It should be noted that in long-term (2001-2012) basis, the dust-storms originated 252

from Sistan present their highest frequency in July (111 episodes) rather than June (93 episodes). 253

However, in the year 2008, the dust storms in June (18 episodes) clearly dominate those in July 254

(8 episodes) and August (6 episodes), thus contributing in the high aerosol loading over Arabian 255

Sea. Prijith et al. (2013) also found larger values of AOD over Arabian Sea during June 2008 256

instead of July 2008. It is worth to be noted that 2008 was the only year that the June AOD 257

dominated that of July over Arabian Sea, supporting that the enhanced dust activity over Sistan is 258

the main reason for the very high AOD. 259

Another important finding is that the wind speed at Zabol during the second half of June 2008 260

was 2.7 ms-1 higher, on average, than that observed during 93 dust-storm events in June during 261

2001-2012 (unpublished data). In this respect, Prijith et al. (2013) estimated larger continental 262

aerosol outflow from southwest Asia to Arabian Sea during June 2008, which justifies the high 263

dust aerosol loading. The whole analysis suggests that this enhanced continental outflow is 264

mainly attributed to the intensity in the Levar winds blowing over Iran – Afghanistan borders. It 265

should be noted that the “Shamal” winds referred by Prijith et al. (2013) do not contribute so 266

much on transportation of dust over Arabian Sea, since they blow along the Tigris-Euphrates 267

basin in Iraq and over the eastern part of the Arabian desert (Karimi et al., 2013; Rezazadeh et 268

al., 2013) without obvious connection with Levar winds (Najafi et al., 2013). 269

According to NOAA Climate Prediction Center June 2008 was the last month of a persistent 270

ENSO (El-Niño Southern Oscillation) cold phase started from August 2007. The cold phase 271

corresponds to cold episodes based on a threshold of +/- 0.5oC for the Oceanic Niño Index (ONI) 272

[3 month running mean of ERSST.v3b Sea Surface Temperature anomalies in the Niño 3.4 273

region (5oN-5oS, 120o-170oW)], characteristic of La Nina years. It should be noted that the peak 274

of the extreme drought over Iran in 1999-2001 (Rashki et al., 2013c) was related to prolonged 275

duration of the La Nina phase (ONI values below -0.5 during the 3-years period, summer 1998 – 276

spring 2001), contributing to the deficit of precipitation over southwest Asia. Similar conditions 277

occurred from August 2007 to June 2008 resulting in deficit of precipitation, Helmand river run 278

off and dryness of the Hamoun lakes. La Nina was found to be usually associated with positive 279

precipitation anomalies over the Indian Ocean and negative ones over the central and southwest 280

Asia (Mathew et al., 2002), while its association with Sistan dust storms has not been evaluated 281

so far. 282

283

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3.4 Synoptic meteorological conditions during June 2008 284

Previous studies (Alizadeh Choobari et al., 2013; Rashki et al., 2014) highlighted the major role 285

of the local and regional topography and meteorological dynamics in controlling the dust activity 286

over southwest Asia. However, when studying dust storms, the synoptic conditions cannot be 287

ignored, since they can be associated to meso-scale or even micro-scale atmospheric phenomena 288

(Kaskaoutis et al., 2012a; Nastos, 2012). 289

Apart of the important role of the local-scale meteorological dynamics discussed in the previous 290

section, the synoptic conditions over south Asia in June 2008 are also examined. The 291

NCEP/NCAR composite means of geopotential heights (gpm) at lower tropospheric levels (1000 292

hP, 850 hPa, 700 hPa) over south Asia in June 2008 (Fig. 8, upper graphs) reveal the presence of 293

a cyclonic circulation at 1000 hPa and 850 hPa extended from northwestern arid India to 294

Pakistan, southern Afghanistan, Iran and eastern Arabian Peninsula. Furthermore, the northern 295

Arabian Sea is under the strong influence of the cyclonic circulation. These synoptic conditions 296

imply a strong SW air flow pattern towards Arabian Sea, reaching 15 ms-1 to 18 ms-1 at the 297

southwestern parts, with respect to the isobaric levels at 1000 hPa and 850 hPa, respectively (Fig. 298

9, composite mean winds). In this point, it is worthy to mention that the SW air flow has been 299

enriched by continental air masses advected from northern arid regions towards northern Arabian 300

Sea. At the 700 hPa level a ridge is extending from east Africa through the Arabian Peninsula, up 301

to Iran and Afghanistan, while a trough is dominant over India, extending over northeastern 302

Arabian Sea. At this isobaric level the air flow comes from west directions (11 ms-1) at the 303

southern parts of Arabian Sea against north air stream over the northern Arabian Sea (6 ms-1). At 304

a first glance this situation resembles the typical atmospheric circulation over south Asia during 305

the Indian summer monsoon. However, the anomalies patterns are characterized by pronounced 306

negative anomalies in the geopotential height field from 1000 hPa up to 700 hPa, reaching up -20 307

to -30 gpm over southeastern Iran and northern Arabian Sea (Fig. 8, lower graphs). The negative 308

anomalies imply that during June 2008 the Indian Low was deeper than usual and expanded 309

towards the northern Arabian Sea. This resulted in the enhancement of the turbulent conditions 310

over the study region, which favored increased dust entrainment into the atmosphere. On the 311

other hand, the expansion of the cyclonic circulation over northern Arabian Sea led to the 312

reinforcement of the dusty continental air masses outflow towards this region, which in 313

combination with the dryness of the Hamoun lakes and the enhancement of the Levar wind, 314

resulted to frequent dust-storms over Arabian Sea. The negative composite anomalies of 315

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geopotential heights at 1000 hPa and 850 hPa practically form an enhancement of the trough that 316

allows the continental air masses to move further to the south, thus affecting central Arabian Sea. 317

This was evident from the air-mass trajectories (Fig. 7), which travel more to the south allowing 318

Sistan dust storms to affect central and western parts of the Arabian Sea and not only the 319

northernmost eastern part as shown from previous studies (e.g. Alam et al., 2011). Furthermore, 320

the negative composite anomalies of geopotential heights mostly at 850 hPa are linked with the 321

level (~1500 m) of higher dust presence over north Arabian Sea as observed via CALIPSO 322

profiles (Prijith et al., 2013). In synopsis, the abnormal atmospheric circulation over south Asia 323

in June 2008, characterized by the deeper and more expanded Indian low, enhances the 324

continental outflow and the movement of dusty air-masses far within the marine environment of 325

Arabian Sea. 326

327

3.5 SPRINTARS model simulations 328

This section provides an insight in SPRINTARS simulations of AOD550 and surface dust 329

concentration over south Asia and examines the anomalies of June 2008 against the decadal 330

(2001-2010) means. Except of checking the model’s capability to detect the abnormal high AOD 331

and dust outflow over Arabian Sea during June 2008, there is a compelling need for improving 332

the dust aerosol inventories over the region in order to make realistic assessment of the dust 333

impacts on radiative forcing and the south Asian monsoon. The AOD550 and surface dust 334

concentration (in µgm-3) values for June 2001-2010, June 2008 as well as the differences 335

between June 2008 and the decadal (2001-2010) means in June are shown in Fig. 10. Both 336

simulations reveal enhanced values of AOD550 and dust concentration along western Arabian 337

Peninsula and Red Sea and in parts of southeastern Iran and southwestern Pakistan. It is worth to 338

be noticed that the dust concentration over Arabian Sea is low, (< 50 µgm-3) even at its northern 339

parts. The dust simulations in the model are based, except of the dust-particle size, on 340

meteorological-atmospheric parameters, mainly surface wind speed for the dust emission, wind 341

profile and prevailing direction for the dust-plume transport, as well as on the moisture of the 342

soil and roughness of the surface (Gilletee, 1978; Takemura et al., 2009; Goto et al., 2011). 343

Therefore, the enhanced dust concentration over eastern Iran, western Afghanistan and 344

southwestern Pakistan suggest increase in dust activity (mostly from the Sistan basin as the 345

major source), which is associated with stronger Levar winds and dryness of the Hamoun lakes. 346

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Despite the different spatial resolution between SPRINTARS and MODIS, and the different 347

periods that considered for the retrieval of the anomalies (Figs. 4 and 10), the model simulations 348

are in general agreement with satellite observations. The simulated AOD550 is larger during June 349

2008 over nearly the whole Arabian Sea and most regions of southwest Asia with the larger 350

positive anomalies (60 - 120%) to be detected over the downwind to Sistan regions, like 351

southeastern Iran and gulf of Oman, suggesting increase in dust activity during June 2008. 352

According to SPRINTARS, the AOD550 over Arabian Sea was about 75% higher during June 353

2008 compared to the decadal-mean June value, which is in agreement with the MODIS 354

observations. Similarly, the dust concentration in June 2008 is shown to be much higher (~50 355

µgm-3) than the decadal mean over the arid regions of Iran and Afghanistan confirming the 356

Prijith et al.’s (2013) approach of enhanced continental outflow over Arabian Sea from northern 357

directions. However, some areas in southern Pakistan show decrease in dust concentration in 358

June 2008, while the model does not simulate pronounced differences (only a slight increase) 359

over the northern parts of the Arabian Sea. 360

361

4. Association between Sistan dust storms and Arabian Sea aerosols 362

The current analysis showed that the air masses originated from Sistan during the dust-storm 363

days were transporting further to the south affecting central Arabian Sea on certain days. Long-364

term investigation (not shown) of numerous (356) dust storms over Sistan during the summer 365

months (June-September) of the period 2001-2012 revealed that the dusty air masses originated 366

from Sistan affect the northernmost eastern part of the Arabian Sea in the vast majority (>80-367

85%) of the cases. In this respect, many studies (Alam et al., 2011; Rashki et al., 2012, 2013b; 368

Ekhtesasi and Gohari, 2013) revealed that the dust outflow from Sistan/Hamoun basin follows a 369

giant “U” affecting mostly the arid-land areas of southwest Asia. This dust-transport pathway is 370

strongly affected by the Indian summer monsoon, and the southwesterly flow over Arabian Sea 371

prevents the northern dusty air masses to significantly affect the central and southern parts of the 372

Arabian Sea, shifting them to northeastern directions. 373

The more southward movement of the Sistan dusty air masses and the wider spreading of the 374

dust plumes over central-south Arabian Sea during June 2008 (Figs. 6, 7) is an important factor 375

that explains the high-abnormal AOD over the oceanic region on that month. In this respect, 376

Prijith et al. (2013) noted enhanced continental outflow at lower tropospheric levels from the arid 377

regions northerly of Arabian Sea within the marine environment. The composite anomalies of the 378

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synoptic weather patterns (Fig. 8) favor the dusty air masses to travel further to the south over 379

Arabian Sea and to significantly affect its northwestern part as well. Strong variations in aerosol 380

loading over Arabian Sea maybe associated with changes in monsoon circulation and intensity 381

(Vinoj et al., 2014). The study by Rahul et al. (2008) showed that higher aerosol loading over 382

Arabian Sea in July occurred during periods with normal-to-surplus of rainfall over India, while 383

the weakening of the Indian summer monsoon and the drought conditions in 2002 and 2004 were 384

associated with lower dust loading over Arabian Sea, limited over the northernmost eastern part. 385

Satellite observations showed that the abnormal high AOD in June 2008 was not limited only 386

over Arabian Sea, but expanded over the Indo-Gangetic Plains (Gautam et al., 2009; Kaskaoutis 387

et al., 2011), which seem to be mostly affected by Thar rather than Sistan dust storms. However, 388

it has not been examined if the dust activity over Sistan and Thar deserts can be associated or 389

even interlinked, since each region has its own characteristics, wind regimes and weather 390

conditions. 391

The current analysis revealed that the statement by Prijith et al. (2013) “the abnormal 392

enhancement in the observed AOD during June 2008 was primarily caused by a distinct increase 393

in dust storms over the northern continents and subsequent transport into the Arabian Sea” 394

corresponds to enhanced dust activity and numerous (18) dust-storm exposures from the 395

Sistan/Hamoun dry-bed basin. Furthermore, the SPRINTARS simulations of AOD and surface 396

dust concentration justified and supports the Prijith et al.’s (2013) notification that “The 397

anomalously large increase in aerosol loading over the Arabian Sea observed in June 2008 is 398

found to be mainly controlled by the enhanced mineral dust loading at the continental regions in 399

the NoAS (e.g., Iran, Afghanistan and the northwestern parts of the Indian subcontinent) and the 400

aerosol transport through the northern boundary of the Arabian Sea”. 401

402

4. Conclusions 403

The present study examined the factors that favored the abnormal high aerosol loading over 404

Arabian Sea during June 2008. Long-term MODIS observations showed an increase of 97% 405

(78.2%) of the AOD550 over Arabian Sea in June 2008 compared to the monthly mean during 406

2000-2010 (2000-2013). Prijith et al. (2013) attributed this increase to enhanced outflow of 407

continental aerosols (dust) from the arid and semi-arid regions located northerly of the Arabian 408

Sea, without emphasizing on a specific source or on the meteorological conditions favored the 409

dust exposure. The present work covered these issues by providing analysis of satellite imagery 410

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and dataset (Landsat, MODIS), meteorological regimes (Zabol meteorological records, 411

NCEP/NCAR database), air-mass trajectories (HYSPLIT model) and model (SPRINTARS) 412

simulations. The main findings are summarized in the followings: 413

1) Analysis of the visibility recordings at Zabol meteorological station, located in Sistan, 414

southeastern Iran and very close to Hamoun dry-bed lakes, showed enhanced occurrence (18) of 415

dust storms (days with vis< 1km) during June 2008, which were mostly detected at the second 416

half of the month. The dust activity over the region was abnormal in June 2008 compared to the 417

climatological mean scenario in June. 418

2) Landsat images over Sistan have shown that the ephemeral Hamoun lakes had been 419

completely dried during the second half of June 2008, leaving an alluvial silt material easily 420

eroded by the strong Levar winds that blow over the region from northern directions. The 421

blowing of strong winds over the dry-bed lakes favored the formation of frequent and massive 422

dust storms that were easily detected by MODIS imagery covering the southern parts of Iran, 423

Pakistan and the largest part of the Arabian Sea. 424

3) 5-day air-mass trajectories that originated from Sistan basin revealed transport of the dusty air 425

masses towards northern parts of the Arabian Sea and gulf of Oman. The synoptic conditions 426

revealed the presence of low-pressure system over southwest arid Asia, favoring the uplift of 427

dust and its transportation over Arabian Sea. The dust continental outflow seemed to be 428

enhanced during June 2008 by examining the composite anomalies of the geopotential heights at 429

lower tropospheric levels from the mean (1981-2010) June climatological conditions. The 430

negative composite anomalies of geopotential heights from 1000 hPa to 700 hPa levels enhanced 431

the cyclonic circulation towards Arabian Sea allowing the dusty air masses originated from 432

Sistan to move further to the south and affect the north and central parts of the marine 433

environment. Thus, the role of meteorology (at regional to synoptic scales), the dryness of the 434

Hamoun lakes (at local scale) and the enhancement of the northern Levar wind constitute 435

important factors for the increase in dust activity over Sistan and the transport of dust air masses 436

towards Arabian Sea. 437

4) In close agreement with satellite observations, SPRINTARS model simulations revealed 438

enhancement in the AOD550 and dust concentration over the arid regions of southwest Asia, 439

especially over Sistan and downwind areas, supporting the findings that the abnormal high 440

aerosol loading over Arabian Sea during June 2008 was mostly attributed to the enhanced dust 441

activity and frequent outflow of dust storms from the Sistan basin. 442

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443

444

Acknowledgements 445

Analyses and visualizations used in this study were produced with the Giovanni online data 446

system, developed and maintained by the NASA GES DISC. We also acknowledge the MODIS 447

mission scientists and associated NASA personnel for the production of the data used in this 448

research effort. The authors gratefully acknowledge the NOAA Air Resources Laboratory (ARL) 449

for the provision of the HYSPLIT transport and dispersion model and/or READY website 450

(http://www.ready.noaa.gov) used in this publication as well as the Landsat scientific team for 451

providing the imagery. The NCEP/NCAR Reanalysis team is also gratefully acknowledged for 452

providing the meteorological maps, as well as the NOAA Climate Prediction Center for the 453

Oceanic Niño Index values. 454

455

456

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Figure Captions 600

Figure 1: Terra MODIS AOD550 values in June over Arabian Sea (8-26oN, 54-75oE) during the 601

period 2000-2013 in box and whisker chart show. Each box contains the 50% of the values (from 602

25% to 75%), the mean value is defined by the solid line and the median by the square. 603

Figure 2: Spatial distribution of Terra-MODIS AOD550 over Arabian Sea during June 2000-2013 604

(a) and June 2008 (b). 605

Figure 3: Spatial distribution of the AOD550 anomalies (%) over Arabian Sea in June 2008 with 606

respect to the long-term means (2000-2013). 607

Figure 4: Latitudinal cross section of the longitude-averaged (54-75oE) AOD550 values over 608

Arabian Sea during June 2008 and long-term (2000-2013) June mean (a). Latitudinal cross 609

section of the absolute and percentage (%) AOD550 anomalies in June 2008 with respect to the 610

long-term mean (2000-2013) (b). 611

Figure 5: Landsat (path/row: 157/38) images over Sistan region and Hamoun dry-bed lakes on 5 612

June 2008 and 21 June 2008. 613

Figure 6: Aqua MODIS true color images over Arabian Sea on 12 days during the second half 614

of June 2008. The arrows show the main pathways of the dust plumes from the arid continents to 615

the marine environment, mostly emphasizing on dust storms originated from Sistan. 616

Figure 7: 5-day forward air mass trajectories starting from Sistan basin at 500 m agl during the 617

18 dust storms in June 2008. The altitudinal variation of the dusty air masses is shown in the 618

colored scale. 619

Figure 8: NCEP/NCAR composite means of geopotential heights at 1000 hPa, 850 hPa and 700 620

hPa over south Asia during June 2008 (upper row) and anomalies from the mean June 621

climatology during 1981-2010 (lower row). 622

Figure 9: Composite mean wind vectors (ms-1) at 1000 hPa, 850 hPa and 700 hPa from 623

NCEP/NCAR reanalysis over south Asia during June 2008. 624

Figure 10: SPRINTARS simulations of surface dust concentration (µgm-3) (upper row) and 625

AOD550 (bottom row) for June 2001-2010, June 2008 and their % difference over southwest 626

Asia. 627

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Highlights

The high AOD over Arabian Sea in June 2008 is mostly attributed to Sistan dust storms

The role of the Sistan basin in dust aerosol loading over Arabian Sea

The Hamoun lakes and the Levar wind play a major role in enhancement of dust activity

The intensity of the cyclonic circulation over Arabian Sea favored the dust exposure